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Physics Letters A

Quantum jumps in a single atom; Prolonged darkness in the fluorescence of a resonantly driven cascade

THOMAS ERBER, Seth Putterman

Published Oct 1, 1989• 1 citation
Publisher
DOI
10.1016/0375-9601(89)90442-8

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Physical Review A•Jan 1, 1987•270 citations
Correlations between the emission of photons from an excited three-level atom with one transition more strongly driven than the other are studied. Antibunching, anticorrelation, and superbunching are exhibited in the four possible configurations: ``vee'' (V), ``lambda'' (\ensuremath{\Lambda}), and two cascades with the upper or lower transition strongly driven. We pay particular attention to the projection of the atom into particular states by the measurement of fluorescence, and its significance for detecting quantum jumps in the weak transition by observing the fluorescence from the strong transition. For incoherent excitation we find that cross antibunching (the anticorrelation between emissions of different types of photons) manifests itself as prolonged periods of darkness. For the V and the cascade configuration with a strongly driven lower transition, these periods herald the emission of a weak-transition photon; for the other cascade and the \ensuremath{\Lambda} configuration the periods are heralded by the emission of a weak-transition photon. For on-resonance coherent excitation, dark periods are extremely infrequent for the former two configurations, and are extremely long or infinite for the latter two.
We consider a three-level atomic system driven strongly on one transition and weakly on the other. The excited state on the weak transition is assumed to be metastable. We give an analysis of the fluorescence from the strong transition in terms of the elementary probability density p[0{p}_{[0}p[0​,t)(t1{\mathrm{t}}_{1}t1​,t2{t}_{2}t2​,..., tn{t}_{n}tn​) which gives us the probability density that exactly n photons are emitted at times t1{t}_{1}t1​,t2{t}_{2}t2​,...,tn{t}_{n}tn​ by the atom in the time interval [0,t). We show that p[0{p}_{[0}p[0​,t) essentially factorizes into products of conditional densities c\ifmmode \tilde{}\else \~{}\fi{}(\ensuremath{\tau}) that, given a photon is emitted at time zero, the next photon emission occurs at time \ensuremath{\tau}. This enables a simulation of the individual photon emissions to be given which shows directly the existence of prolonged dark windows in the fluorescence corresponding to the shelving of the electron in the metastable state or ``quantum jumps.''