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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Suboptical wavelength atomic gratings generated in a time-domain interferometer

Andrey V. Turlapov, Dmitry Strekalov, Anantharaman Kumarakrishnan, Sydney B. Cahn, Andreas Karpf, Tycho Sleator

Published Jul 19, 1999• 0 citations
Publisher

Abstract

We have studied sub-optical wavelength atomic gratings generated by the interference of atomic de Broglie waves in a time-domain interferometer. Three short optical standing- wave pulses, detuned from resonance with a cloud of approximately 100 (mu) K 85Rb atoms, act as phase gratings for atomic matter waves. Shortly after the first pulse, a modulation in the atomic density containing spatial harmonics of period (lambda) /2N appears ((lambda) is the optical wavelength, and N is any integer) and then rapidly vanishes due to the atomic thermal motion. The cloud maintains phase memory of this modulation, however, and the second pulse (applied at time T after the first one) results in a temporal sequence of atomic density gratings of periods (lambda) /2N. The appearance of a grating is referred to as an echo. The third pulse (and a subsequent traveling wave pulse) is used to detect these gratings. By this technique, we have created and detected in real time a grating with period (lambda) /4 at time 1.5T after the first pulse and observed new types of `echoes' caused by interaction of the de Broglie waves with all three phase gratings. This ability to produce sub-wavelength structures makes our techniques applicable to atomic beam lithography.

DOI
10.1117/12.354726

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•Jan 1, 2014•0 citations
We have studied sub-optical wavelength atomic gratings generated by the interference of atomic de Broglie waves in a time-domain interferometer. Three short optical standing- wave pulses, detuned from resonance with a cloud of approximately 100 (mu) K 85Rb atoms, act as phase gratings for atomic matter waves. Shortly after the first pulse, a modulation in the atomic density containing spatial harmonics of period (lambda) /2N appears ((lambda) is the optical wavelength, and N is any integer) and then rapidly vanishes due to the atomic thermal motion. The cloud maintains phase memory of this modulation, however, and the second pulse (applied at time T after the first one) results in a temporal sequence of atomic density gratings of periods (lambda) /2N. The appearance of a grating is referred to as an echo. The third pulse (and a subsequent traveling wave pulse) is used to detect these gratings. By this technique, we have created and detected in real time a grating with period (lambda) /4 at time 1.5T after the first pulse and observed new types of `echoes' caused by interaction of the de Broglie waves with all three phase gratings. This ability to produce sub-wavelength structures makes our techniques applicable to atomic beam lithography.
We have studied suboptical wavelength atomic gratings, generated by the interference of atomic de Broglie waves in a time-domain interferometer. Three short optical standing- wave pulses, detuned from resonance with a cloud of approximately 100 (mu) K85 Rb atoms, act as phase gratings for atomic matter waves. The first two standing- wave pulses, separated by time T, produce a sequence of atomic density gratings of periods $lamda/4 at time 1.5T after the first pulse. The dependence of our signals on the time separation of the pulses is in good agreement with our theoretical predictions. As far as we know, this is the first time when the formation of a high order matter-wave diffraction grating was observed in real time. This demonstrated ability to produce sub-wavelength structures makes our techniques applicable to atomic beam lithography.
We have demonstrated a method of generation and real-time detection of nanostructures in a cold Rb cloud. These structures, which are periodic gratings of atomic density, appear as a result of interference of atoms diffracted by pulses of an optical standing wave of wavelength $\ensuremath{\lambda}.$ We have detected structures of period $\ensuremath{\lambda}/2$ and $\ensuremath{\lambda}/4.$ Calculations indicate that these density gratings have period $\ensuremath{\lambda}/2N$ for integer N. While the structures with the period $\ensuremath{\lambda}/2$ are easily detected by Bragg scattering of an optical probe beam, the shorter-period structures are not. For their detection we have developed a three-pulse echo method, in which the shorter-period gratings get converted into the structures with period $\ensuremath{\lambda}/2,$ readily detected in real time. Applications related to lithography are discussed.
We have demonstrated direct imaging of interference fringes of total atomic density with periods $\ensuremath{\lambda}∕4$ and $\ensuremath{\lambda}∕2$ for optical wavelength $\ensuremath{\lambda}$ that have been produced in a de Broglie wave atom interferometer. The imaging was done by means of an ``optical mask'' technique, which allowed us to observe subwavelength periodic patterns with a resolution of up to $\ensuremath{\lambda}∕16$. In addition, the dependence of the fringe pattern on the recoil phase and pulse area reveals quantum dynamics in the atomic center-of-mass motion. The behavior of the fringe patterns near the interference times distinguishes the effects of phase gratings from those of amplitude gratings.
We have used an echo-type atom interferometer that manipulates laser-cooled atoms in a single ground state to investigate the effect of light scattering from pulsed and continuous-wave light. The interferometer uses two off-resonant standing-wave pulses applied at times t=0t=0t=0 and t=Tt=Tt=T to diffract and recombine momentum states separated by $2\ensuremath{\hbar}k$ at t=2Tt=2Tt=2T. Matter wave interference is associated with the formation of a density grating with period $\ensuremath{\lambda}/2$ in the vicinity of this echo time. The grating contrast is measured by recording the intensity of coherently backscattered light. The interferometer is perturbed by an additional pulse applied at $t=2T\ensuremath{-}\ensuremath{\delta}T$ or by continuous-wave background light. If the additional pulse is a standing wave, the momentum states interfering at t=2Tt=2Tt=2T are displaced and the grating contrast can be completely recovered due to constructive interference. In this case, the contrast shows a periodic modulation at the atomic recoil frequency as a function of $\ensuremath{\delta}T$. In a recent work, it was shown that the atomic recoil frequency can be measured easily and precisely when using coherence functions to model the signal shape. This paper provides an alternative description of the signal shape through an analytical calculation of echo formation in the presence of an additional standing-wave pulse. Using this treatment, it is possible to model the effects of spontaneous emission and spatial profile of the laser beam on the signal shape. Additionally, the theory predicts scaling laws as a function of the pulse area and the number of additional standing-wave pulses. These scaling laws are investigated experimentally and can be exploited to improve precision measurements of the atomic recoil frequency. We also show that coherence functions can be used to make a direct measurement of the populations of momentum states associated with the ground state under conditions where the Doppler-broadened velocity distribution of the sample is much larger than the recoil velocity. These measurements are consistent with Monte Carlo wave-function simulations. If the additional pulse is a traveling wave, we find that the grating contrast measured as a function of $\ensuremath{\delta}T$ can be modeled by a quasiperiodic coherence function as in previous experiments that utilized atomic beams. In this work, we investigate the dependence of the photon scattering rate on the intensity and detuning of the traveling wave. We also study the effects of perturbing the interferometer with continuous-wave light and find that the dependence of the photon scattering rate on the intensity and detuning of the perturbing field is consistent with expectations.
This thesis details the experimental investigation of a new type of atom interferometer using rubidium-85 atoms in the unexplored near-resonant domain. A cold cloud of atoms, all prepared in the same hyperfine ground state, are subjected to temporally periodic pulses of near-resonant standing waves of light. The standing wave pulses are made to act like an absorption grating where only atoms located around the low intensity region about the nodes remain in the initial ground state, the rest are pumped into a dark hyperfine ground state. The output of the atom interferometer is a measure of the fraction of atoms remaining in the initial ground state after N standing wave pulses for different times between the pulses. An increased survival rate is observed for certain times between pulses due to the occurrence of a coherence echo and the matter wave Talbot effect. This feature allows us to use our atom interferometer to make measurements of the Talbot time which is an important parameter in determinations of the fine structure constant alpha.\n\nWe provide a theoretical model to describe the relevant physics behind our atom interferometer that compares well with our empirical results. Design and implementation of the apparatus are discussed along with characterisation of parameters such as pulse duration, pulse number, and frequency. Finally we include a demonstration of how, in principle, our atom interferometer could be used to make precision measurements of the Talbot time along with some of the necessary steps to bring it in line with current leading measurements.