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Optics Communications

Ground state Zeeman coherence effects in an optically pumped cesium beam

G. Théobald, N. Dimarcq, V. Giordano, P. Cérez

Published Jun 1, 1989• 48 citations
Publisher
DOI
10.1016/0030-4018(89)90004-7

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We investigate the population differences between ground-state hyperfine levels (5S1/2,F=2{5S}_{1/2},F=25S1/2​,F=2 and 5S1/2,{5S}_{1/2},5S1/2​, F=1F=1F=1) of an optically pumped 87Rb{}^{87}\mathrm{Rb}87Rb beam in a static magnetic field, taking into account the various kinds of atomic coherence (Zeeman, hyperfine, and optical). The pumping lasers are monochromatic and in resonance with the ${(5S}_{1/2},F=1\ensuremath{\leftrightarrow}{5P}_{1/2}{,F}^{\ensuremath{'}}=1)$ transition. By varying the polarization configuration of the pumping lasers, we find that the pumping efficiency is substantially enhanced when a $\ensuremath{\sigma}$-polarized laser and a $\ensuremath{\pi}$-polarized laser are counterpropagating. In this case, the pumping efficiency remains high even in a weak magnetic field, which explains qualitatively experimental data reported previously from a cesium beam experiment.
Two-laser optical pumping schemes show great promise for atom preparation since they can act as a nearly perfect state selector. This paper presents a new theoretical model to evaluate the pumping efficiency of two-laser pumping schemes, taking into account optical, ground and excited states hyperfine and Zeeman coherences, neighboring transitions, and fluctuating laser fields. The model is used to predict the optical pumping efficiency of two lasers with Lorentzian spectral profiles on a beam of cesium atoms. The particular laser intensities and linewidths that optimize the optical pumping efficiency and rate are calculated.
We report an experimental study on the ground-state magnetic resonances of optically pumped cesium vapors at lower temperatures of about 30°C–40°C. A longitudinal static magnetic field is applied along the single laser beam to control the splitting of the Zeeman sublevels of the ground state. When the laser frequency is set to the cesium D1 spectral line (F=3→F′=4), by modifying the transverse radio frequency field, we find that the unusual weaker-absorption and zero-dip resonance phenomena occur in the optical-magnetic resonance (OMR) effects, which is called the cesium optical-RF resonance line reversals and doubling in this paper. We explore a theoretical description for these phenomena by using density matrix equations, and our calculated results are in approximate agreement with the experimental results.