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Optics Communications

Near-resonant Rayleigh scattering and collision-induced fluorescence

John L. Carlsten, A. Szöke

Published Jul 1, 1976• 1 citation
Publisher
DOI
10.1016/0030-4018(76)90622-2

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Light scattered from strontium vapor near its 460.73-nm ($^{1}{P}_{1}^{\ensuremath{\circ}}\ensuremath{-}^{1}S_{0}$) resonance transition was resolved into its three spectral components: Rayleigh scattering, collision-induced fluorescence, and three-photon scattering. The saturation behavior of the central (Rayleigh) component and the intensity and ac Stark shift of the three-photon component were studied as a function of detuning and laser intensity. Good agreement is obtained with theoretical predictions.
Light scattered from strontium vapor near its 460.73-nm ($^{1}{P}_{1}^{\ensuremath{\circ}}\ensuremath{-}^{1}S_{0}$) resonance transition was resolved into its three spectral components: Rayleigh scattering, collision-induced fluorescence, and three-photon scattering. The saturation behavior of the central (Rayleigh) component and the intensity and ac Stark shift of the three-photon component were studied as a function of detuning and laser intensity. Good agreement is obtained with theoretical predictions.
Strontium vapour was irradiated by a dye laser tuned near the 460.73 nm ( 1 P 1 0 - 1 S 0 ) resonance transition. Collision-induced fluorescence at the resonance frequency and Rayleigh scattering at the laser frequency were studied as a function of detuning Delta over a range of about 30 nm (1500 cm -1 ). The Rayleigh component was found to vary as Delta -2 , as expected, whereas the collision-induced fluorescence was markedly asymmetric. This experiment constitutes a direct measurement of the redistribution function.