Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Physical Review Letters

Quantum State Holography

C. Leichtle, Wolfgang P. Schleich, Ilya Sh. Averbukh, M. Shapiro

Published Feb 16, 1998• 98 citations
Publisher

Abstract

We introduce a method for reconstructing quantum superposition states excited in molecules or atoms by short laser pulses. The technique is based on mixing the unknown object state with a known reference state generated in the same system by an additional delayed laser pulse, and detecting the total time- and frequency-integrated fluorescence as a function of the delay. We demonstrate the feasibility of the method by reconstructing various vibrational wave packets in sodium dimers.

DOI
10.1103/physrevlett.80.1418

Related papers

Reconstructing wave packets by quantum-state holography

Ilya Sh. Averbukh, M. Shapiro, C. Leichtle +1 more

We analyze and further develop our method of quantum-state holography for reconstructing quantum superposition states in molecules or atoms [Phys. Rev. Lett. 80, 1418 (1998)]. The technique is based on mixing the unknown object state with a known reference state generated in the same system by two delayed laser pulses, and detecting the total time- and frequency-integrated fluorescence as a function of the delay. The feasibility of the method is demonstrated by reconstructing various vibrational wave packets in sodium dimers. Both the cases of completely controlled and noisy relative phase between the laser pulses are considered. In the latter case, we use the technique of coherence observation by interference noise to recover the interference component of the fluorescence signal. Our results clearly demonstrate the robustness of quantum-state holography and the high quality of reconstruction even in the presence of the external noise.

Physical Review A•Mar 1, 1999•38 citations

Heterodyne measurement of vibrational wave packets of diatomic molecules

A. Zucchetti, W. Vogel, D.‐G. Welsch +1 more

A method is presented for reconstructing the quantum state of vibrational wave packets in diatomic molecules by a heterodyne experiment. After the preparation of a wave packet, a femtosecond laser pulse interferes with the induced polarization and the resulting signal is frequency filtered and measured by a photodetector. The conditions are analyzed under which the resulting time- and frequency-resolved photocurrent contains the information needed to recover the quantum state of the prepared wave packet. It is shown that the vibrational wave function in the excited electronic state can be measured directly without the need of involved numerical reconstruction. Simulations of the proposed experiment are performed for sodium dimers.

Physical Review A•Oct 1, 1999•14 citations

Reconstructing vibrational states in warm molecules using four-wave mixing with femtosecond laser pulses

Anders S. Mouritzen, Olga Smirnova, Stefanie Gräfe +2 more

We propose a method to reconstruct the vibrational quantum state of molecules excited by a general excitation laser pulse. Unlike existing methods, we do not require the molecules before excitation to be in a pure state, allowing us to treat the important case of initially thermally excited molecules. Even if only a single initial level is appreciably populated, initial levels with small populations can still give major contributions to the unknown vibrational state, making it essential to take them into account. In addition to the excitation pulse, the method uses two incident, short laser pulses in a non-co-linear geometry to create four-wave mixing in the molecules. The measurements used in the reconstruction are spectra of the outgoing four-wave mixing pulse at different time delays of the excitation laser pulse. An important point is that the method does not require detailed knowledge of molecular transition moments between excited states nor of any of the incoming laser pulses, but circumvents this requirement by using one or more calibration laser pulses in a separate experiment either before or after the main data are recorded. The only requirements for the calibration laser pulses are that the constant parts of their spectrums should together cover the spectral range of the excitation laser pulse, and the constant part of each should have sufficient spectral overlap with one other calibration pulse to populate two of the same levels. Finally, we discuss the extension of the reconstruction method in this paper to more general situations, hereby presenting the new idea of quantum state reconstruction through perturbations with calibration.

arXiv:0706.1452•Jun 11, 2007•0 citations

Coherent control of electronic and vibrational wave packets using phase-locked optical pulses

Elizabeth Durrell Boleat

Experimental and theoretical work is presented on the control of wave packet dynamics in atomic and molecular systems. Using sequences of phase-locked optical pulses, the link between optical phase and quantum mechanical phase is explored in the Na atom and Naj dimer, representing a step towards the logical engineering of quantum states in more complicated systems. A novel apparatus, constructed to study and control the vibrational dynamics of vibrational wave packets on the Na ionic potential surface, is described in chapter 3. Theoretical simulations for proposed experiment are presented in chapter 4. Control is achieved by exploiting the phase-evolution of the constituent vibrational quantum states within the wave packet superposition. The phase relationship and the accumulated phase difference between the various components of the wave packet is determined, and a sequence of phase-locked optical pulses is employed to selectively enhance or depopulate specific vibrational states, or sets of vibrational states. The quantum state composition of the resulting wave packet, and the efficiency of the control scheme, is determined by calculating the multi-pulse response of the time-dependent vibrational state populations. In chapter 5, the quantum interference between Rydberg electron wave packets in the Na atom is investigated using pairs of phase-locked wave packets, allowing manipulation of the total orbital angular momentum of Na Rydberg atoms. Initially the wave packet is composed of a superposition of s and d Rydberg series. Exploitation of the difference between the quantum defects of the two series allows specific angular momentum compositions within the resultant wave packet to be engineered. Experimentally, this final quantum state distribution is analysed in the frequency domain using state selective field ionisation, and in the time domain using the optical Ramsey method. The theoretical calculations show how the phase difference between pairs of optical pulses is linked to the corresponding Rydberg frequency spectrum, therefore enabling the control of the quantum state composition of the wave packets.

•Jan 1, 2005•0 citations

Observation of a vibrational-wave-packet-induced photon echo

Thomas J. Dunn, John N. Sweetser, Czesław Radzewicz +1 more

Most experiments that study the dynamics of vibrational wave packets in small molecules utilize geometries in which propagation plays little or no role.1 In contrast, we have developed an apparatus for performing time-resolved fluorescence upconversion from an extended sample of sodium dimers that are excited by a resonant short optical pump pulse, with a temporal resolution of about 70 fs.

Annual Meeting Optical Society of America•Jan 1, 1992•0 citations

Atom-optics holograms

Alexander Soroko

The temporal evolution of atomic wave packets interacting with object and reference electromagnetic waves is investigated, and an analytical solution for the off-resonant density matrix is presented. It is shown that, under certain physical conditions, the diffraction of an ultracold atomic beam by an inhomogeneous laser field can be interpreted as if the beam passes through a three-dimensional hologram. We show that high diffraction efficiencies can be realized if one restricts the extent of the atomic hologram in the time domain rather than in space. The hologram, thus, can work in a pulsed regime pumping atoms from the beam or from the initial wave packet into the reconstructed matter wave. The suggested regime is well compatible with the Raman cooling methods and the recent realization of an atom laser, which are capable of repeatedly reproducing coherent, or almost coherent, atomic wave packets necessary for the actual implementation of the reading beam. It is found that the diffraction efficiency of such a hologram may reach 100% and is determined by the duration of laser pulses. On this basis, a new method for the reconstruction of the object image with matter waves is offered. The latter may have useful practical applications, ranging from atom lithography, to the manufacturing of microstructures, and quantum microfabrication.

Optics and Spectroscopy•Sep 1, 2001•2 citations
We introduce a method for reconstructing quantum superposition states excited in molecules or atoms by short laser pulses. The technique is based on mixing the unknown object state with a known reference state generated in the same system by an additional delayed laser pulse, and detecting the total time- and frequency-integrated fluorescence as a function of the delay. We demonstrate the feasibility of the method by reconstructing various vibrational wave packets in sodium dimers.
We analyze and further develop our method of quantum-state holography for reconstructing quantum superposition states in molecules or atoms [Phys. Rev. Lett. 80, 1418 (1998)]. The technique is based on mixing the unknown object state with a known reference state generated in the same system by two delayed laser pulses, and detecting the total time- and frequency-integrated fluorescence as a function of the delay. The feasibility of the method is demonstrated by reconstructing various vibrational wave packets in sodium dimers. Both the cases of completely controlled and noisy relative phase between the laser pulses are considered. In the latter case, we use the technique of coherence observation by interference noise to recover the interference component of the fluorescence signal. Our results clearly demonstrate the robustness of quantum-state holography and the high quality of reconstruction even in the presence of the external noise.
A method is presented for reconstructing the quantum state of vibrational wave packets in diatomic molecules by a heterodyne experiment. After the preparation of a wave packet, a femtosecond laser pulse interferes with the induced polarization and the resulting signal is frequency filtered and measured by a photodetector. The conditions are analyzed under which the resulting time- and frequency-resolved photocurrent contains the information needed to recover the quantum state of the prepared wave packet. It is shown that the vibrational wave function in the excited electronic state can be measured directly without the need of involved numerical reconstruction. Simulations of the proposed experiment are performed for sodium dimers.
We propose a method to reconstruct the vibrational quantum state of molecules excited by a general excitation laser pulse. Unlike existing methods, we do not require the molecules before excitation to be in a pure state, allowing us to treat the important case of initially thermally excited molecules. Even if only a single initial level is appreciably populated, initial levels with small populations can still give major contributions to the unknown vibrational state, making it essential to take them into account. In addition to the excitation pulse, the method uses two incident, short laser pulses in a non-co-linear geometry to create four-wave mixing in the molecules. The measurements used in the reconstruction are spectra of the outgoing four-wave mixing pulse at different time delays of the excitation laser pulse. An important point is that the method does not require detailed knowledge of molecular transition moments between excited states nor of any of the incoming laser pulses, but circumvents this requirement by using one or more calibration laser pulses in a separate experiment either before or after the main data are recorded. The only requirements for the calibration laser pulses are that the constant parts of their spectrums should together cover the spectral range of the excitation laser pulse, and the constant part of each should have sufficient spectral overlap with one other calibration pulse to populate two of the same levels. Finally, we discuss the extension of the reconstruction method in this paper to more general situations, hereby presenting the new idea of quantum state reconstruction through perturbations with calibration.
Experimental and theoretical work is presented on the control of wave packet dynamics in atomic and molecular systems. Using sequences of phase-locked optical pulses, the link between optical phase and quantum mechanical phase is explored in the Na atom and Naj dimer, representing a step towards the logical engineering of quantum states in more complicated systems. A novel apparatus, constructed to study and control the vibrational dynamics of vibrational wave packets on the Na ionic potential surface, is described in chapter 3. Theoretical simulations for proposed experiment are presented in chapter 4. Control is achieved by exploiting the phase-evolution of the constituent vibrational quantum states within the wave packet superposition. The phase relationship and the accumulated phase difference between the various components of the wave packet is determined, and a sequence of phase-locked optical pulses is employed to selectively enhance or depopulate specific vibrational states, or sets of vibrational states. The quantum state composition of the resulting wave packet, and the efficiency of the control scheme, is determined by calculating the multi-pulse response of the time-dependent vibrational state populations. In chapter 5, the quantum interference between Rydberg electron wave packets in the Na atom is investigated using pairs of phase-locked wave packets, allowing manipulation of the total orbital angular momentum of Na Rydberg atoms. Initially the wave packet is composed of a superposition of s and d Rydberg series. Exploitation of the difference between the quantum defects of the two series allows specific angular momentum compositions within the resultant wave packet to be engineered. Experimentally, this final quantum state distribution is analysed in the frequency domain using state selective field ionisation, and in the time domain using the optical Ramsey method. The theoretical calculations show how the phase difference between pairs of optical pulses is linked to the corresponding Rydberg frequency spectrum, therefore enabling the control of the quantum state composition of the wave packets.
The temporal evolution of atomic wave packets interacting with object and reference electromagnetic waves is investigated, and an analytical solution for the off-resonant density matrix is presented. It is shown that, under certain physical conditions, the diffraction of an ultracold atomic beam by an inhomogeneous laser field can be interpreted as if the beam passes through a three-dimensional hologram. We show that high diffraction efficiencies can be realized if one restricts the extent of the atomic hologram in the time domain rather than in space. The hologram, thus, can work in a pulsed regime pumping atoms from the beam or from the initial wave packet into the reconstructed matter wave. The suggested regime is well compatible with the Raman cooling methods and the recent realization of an atom laser, which are capable of repeatedly reproducing coherent, or almost coherent, atomic wave packets necessary for the actual implementation of the reading beam. It is found that the diffraction efficiency of such a hologram may reach 100% and is determined by the duration of laser pulses. On this basis, a new method for the reconstruction of the object image with matter waves is offered. The latter may have useful practical applications, ranging from atom lithography, to the manufacturing of microstructures, and quantum microfabrication.