In this thesis we study the generation of randomness from quantum mechanical sources: quantum random number generators (QRNGs). Such devices are thought to provide a better quality of randomness than is possible with classical devices, but the issue is in need of more rigorous study. In Chapter 1 we provide the necessary background for the thesis from both computability and probability theory. We then present and extend some recent results providing a more theoretical grounding for the indeterminism in quantum mechanics. In particular, we show that sequences of quantum random bits are incomputable in the strongest sense: no bit can be provably computed in advance. In Chapter 2 we study in detail the use of von Neumann normalisation for QRNGs producing both finite strings and infinite sequences of bits; such normalisation methods are necessary in order to counter for experimental imperfections. We show that, in the case of a constantly biased source, this normalisation gives the desired uniform distribution. The effect of this normalisation on the (in)computability of the generated sequences is studied, and it is shown that algorithmic randomness and Borel normality are preserved, but e-randomness (and thus incomputability) is, in general, not. Experimental bounds for the extent of departure from the uniform distribution in the non-ideal case of a slowly drifting bias are derived. In Chapter 3 we propose a new QRNG which uses entangled photon pairs and is certified to produce incomputable bits by value indefiniteness; this is the first QRNG with explicit certification by a physical principle. The effects of various experimental imperfections are discussed in detail, and care is taken to make the proposed QRNG as robust as is possible to these. A robust method based on XORing the produced bitstrings together is proposed to further improve the quality of the distribution produced by the QRNG. Various improvements and optimisations to this scheme are discussed.
We construct a class of three-dimensional photonic quantum random number generators (QRNGs) and prove that each of them generates maximally unpredictable digits via measurements that are robust to errors. This shows that every sequence generated is strongly incomputable; hence its quality is provably better than that of every pseudo-random sequence. These results suggest that incomputability in physics is real and practically applicable. Finally, we present photonic implementations of three-dimensional QRNGs and discuss device independence.
Room-temperature MASERs (Microwave Amplification by Stimulated Emission of Radiation) are coherent sources that exploit stimulated emission to amplify electromagnetic waves at microwave frequencies. Here we report the first demonstration of an LED-pumped maser based on photo-excited triplet states of pentacene in p-terphenyl. The LED light is brightness enhanced and guided using a Cerium-doped Yttrium Aluminium Garnet luminescent crystal that uses light recycling to reach record luminance and power levels. We observe stable maser emission at 1.45 GHz using LED pumping at a much lower pump threshold power. This new maser is cost-effective, safe, and environmentally friendly, and hence ensures a wide variety of potential uses, including more sensitive magnetic resonance body scanners, quantum optical coherence tomography, advanced quantum computer components, portable atomic clocks, and better radio astronomy devices for deep space exploration.