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Physical Review A

Spatial correlations of random potentials and the dynamics of quantum coherence

Michael R. Gallis

Published Jan 1, 1992• 15 citations
Publisher

Abstract

Several quantum open-system models have been examined recently that dynamically reduce the off-diagonal terms of the density operator in the position representation by incorporating the effects of interaction with external degrees of freedom. A recent model [M. R. Gallis and G. N. Fleming, Phys. Rev. A 42, 38 (1990)] includes explicit dependence on the spatial correlations of the decoherence rate of the off-diagonal elements (in the position representation) of the density operator. In this paper, we use influence-functional techniques to examine the effect of an external potential that randomly varies as function of position and time, which leads to a natural characterization of the decay rate of the coherence between spatially separated states in terms of the spatial correlations of the potential, and the corresponding fluctuating forces. We obtain the effective master equations for short environment relaxation time scales, and discuss the similarities and differences between the effects of random external potentials versus the effects of interactions with external degrees of freedom, such as that recently investigated by Stern, Aharonov, and Imry [Phys. Rev. A 41, 3436 (1990)].

DOI
10.1103/physreva.45.47

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Several quantum open-system models have been examined recently that dynamically reduce the off-diagonal terms of the density operator in the position representation by incorporating the effects of interaction with external degrees of freedom. A recent model [M. R. Gallis and G. N. Fleming, Phys. Rev. A 42, 38 (1990)] includes explicit dependence on the spatial correlations of the decoherence rate of the off-diagonal elements (in the position representation) of the density operator. In this paper, we use influence-functional techniques to examine the effect of an external potential that randomly varies as function of position and time, which leads to a natural characterization of the decay rate of the coherence between spatially separated states in terms of the spatial correlations of the potential, and the corresponding fluctuating forces. We obtain the effective master equations for short environment relaxation time scales, and discuss the similarities and differences between the effects of random external potentials versus the effects of interactions with external degrees of freedom, such as that recently investigated by Stern, Aharonov, and Imry [Phys. Rev. A 41, 3436 (1990)].
The challenge of making nano-scale quantum systems experimentally accessible is being overcome for an increasing diversity of systems by improved fabrication techniques and experimental control. Despite rapid progress, one of the main hindrances in all experiments is the difficulty of isolating the quantum system from the surrounding environment and its fluctuations. This experimental “noise” perturbs the quantum system, a process that is generally referred to as decoherence: the system slowly loses its distinguishing quantum features. In this thesis the effects of spatial correlations in the noise environment with a finite correlation length are investigated. The consequences for the experimental design of controlled quantum systems as well as the dynamics of solid state systems are presented. We utilize the Bloch-Redfield formalism, a Markovian master equation approach, which gives a close connection to the underpinning system-environment model. We show how to use this formalism to model any spatial correlation function of the noise environment. Using microscopic environmental models, several correlation functions are derived and their properties connected to the environmental parameters. Several phenomenological correlation functions are also studied and a mapping to the Lindblad master equation is presented, which provides a test of positivity for phenomenological models. For quantum transport through spin chains and networks, noise is generally detrimental. Spatial correlations however reduce the effect of dephasing noise and can reinstate the transport dynamics. The critical correlation length proves to be closely connected to the maximal packet width of one excitation in the transfer process. For dissipation noise, relaxation-free states emerge with spatial correlations. The decay of an excitation is therefore fundamentally modified into a fast decay towards an intermediate relaxation-reduced state and a subsequent decay to the ground state on a much longer time scale. In quantum metrology noise correlations have been observed in experiments with trapped ions, in which they limit the use of such experiments for metrology. Quantum advantage, i.e. a better precision scaling than the standard quantum limit has been proven impossible in the presence of uncorrelated Markovian noise only. We show that for certain optimized states the best possible quantum advantage, Heisenberg scaling, can be achieved in the presence of noise with a finite spatial decay of correlations. We furthermore identify how dephasing effects change and a topology dependence arises in strength with increasing correlation length for entangled states in a general way. Biological photosynthetic complexes have recently been found to potentially include quantum coherent dynamics, particularly in the process of transmitting an exciton from the point of creation to the reaction centre. We show how the formalism of spatially correlated decoherence adapts to this significantly different energy regime. Typical effects of decoherence in this field are presented and we show how the light-harvesting efficiency is influenced by spatial correlations in the noise. This thesis highlights the fundamental relevance of noise correlations to several fields of quantum physics and the importance of the efficient and comprehensive modelling techniques presented.
Several modifications of the Schr\"odinger equation that dynamically reduce the off-diagonal elements of the density operator in the position representation (localization) have received recent attention in the literature. Models of quantum open systems provide localization for the system of interest by considering the effects of an environment on the effective master equation that describes the dynamics of the reduced density operator for the system of interest. In contrast, localization is introduced as a fundamental modification to the Schr\"odinger equation in quantum mechanics with spontaneous localization (QMSL) [G. C. Ghirardi, A. Rhimini, and T. Weber, Phys. Rev. D 34, 470 (1986)]. We compare several environment models and discuss some of the anomalous features of the effective master equations noted by Ballentine [L. E. Ballentine, Phys. Rev. A 43, 9 (1991)] by examining the Ehrenfest relations for position, energy, and momentum. Insight is provided into the relative importance of various terms in the effective master equations for several environment models. We also briefly discuss the implications of similar anomalous features present in the QMSL master equation in light of our analysis of the open-system models.
We present a comprehensive analytical and numerical study of time-dependent decoherence in open quantum systems, focusing on a single-qubit model with time-varying Lindblad dissipation rates. Employing a master equation framework, we derive exact solutions for the evolution of off-diagonal density matrix elements and characterize the emergence of robust pointer states. Our findings reveal an initial rapid coherence decay followed by a gradual slowdown, mirroring experimental trends observed in superconducting qubits influenced by quasiparticle dynamics and in photonic cavities subject to fluctuating environments. By incorporating real experimental parameters and validating the model through quantum simulations using QuTiP, we provide a robust quantitative tool for analyzing decoherence in quantum technologies. This extended model addresses limitations in static-rate approximations, offering insights into non-Markovian effects without resolving the measurement problem, and suggests extensions to multi-qubit systems.
The interaction of a quantum system with a many degree of freedom environment entails damping and the loss of quantum coherence. In these two lectures we focus on two aspects of open quantum system dynamics. First, we present decoherence as a dynamical phenomenon and determine the corresponding time scales, discuss an experiment and the nature of robust states, and mention universal properties of short-time decoherence of macroscopic superpositions. Secondly, in analogy to the classical description of open systems in terms of Langevin equations, we present a stochastic approach to open quantum system dynamics in terms of a stochastic Schrödinger equation. We give a microscopic derivation that allows us to generalize the stochastic approach to non-Markovian situations. We discuss a convolutionless formulation of our theory and finally, we focus on the quantised version of Brownian motion as an often-employed example.
Quantum mechanics has both deepened our understanding of the physical reality and allowed development of quantum technologies beating their classical counterparts in efficiency, security, and sensitivity. As a major downside, the quantum properties behind these technologies are very sensitive to the effects the system’s interaction with its environment. The theory of open quantum systems describes how such interaction influences the system, and as a consequence, how the quantum features are lost, controlled, and possibly returned by manipulating the environment. This thesis begins with a short description of the most relevant features and results of the open quantum system theory. We continue by presenting some commonly used measures to quantify the information encoded in quantum systems and the correlations between spatially or temporally separated parties. The literature review ends with discussion of non-Markovianity and memory effects which combine the fields of open quantum systems and quantum information in a natural way. The rest of the thesis presents the main results of Publications I – VII. We study the memory effects and physicality conditions of open system dynamics described by the vast family of phase-covariant master equations. We show how the open quantum system picture can be exploited to design probing protocols to extract information without knowing how the probe and system interact. Such protocols are considered also from the point-of view of efficiently obtaining the information required in the probing, both in theory and by experimental implementation. The experiment serves also as evidence for applicability of recently developed geometric tools to design informationally incomplete measurements for solving so-called membership problems. We present and experimentally realize a protocol where control over intial correlations between polarization and frequency gives full freedom to implement any dephasing dynamics in the open system polarization, thus dictating how its information content changes in time. We study the two-qubit memory effects of dephasing dynamics and compare them to the effect of such noise in the transmission efficiency in superdense coding. Optimal noise configurations in different situations are found. Finally, we characterize the families of initial states for which the decay of quantum correlations depends or does not depend on the noise location.
This work presents an effective open-quantum-systems model for decoherence in multipartite entangled states subject to spatially correlated environmental noise. Without assuming a specific microscopic mechanism, the model characterizes collective decoherence through correlated noise terms and examines their impact on entanglement stability and decay rates. The approach is phenomenological and compatible with standard quantum dynamical frameworks, providing testable scaling behavior relevant to quantum information and foundational studies.