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Physical Review E

Decay of a metastable state induced by a spin bath

Sudarson Sekhar Sinha, Arnab Ghosh, Deb Shankar Ray

Published Oct 11, 2011• 9 citations
Publisher

Abstract

The spin-bath induced decay of a quantum system out of a metastable state, which can tunnel and undergo thermal activation, is considered. The treatment is based on the c-number description of bath degrees of freedom and a canonical thermal distribution of the associated c-number variables. We show that, apart from the usual frequency prefactor and its dynamical modification in the spatial diffusion-limited regime, i.e., the Grote-Hynes factor, the rate coefficient contains two other factors. One is a quantum correction to the dynamical factor resulting from quantum transmission and reflection of the particle at the finite barrier. This term exhibits exponential rate enhancement at low temperature. The other one is a quantum corrected Arrhenius factor, which incorporates the effect of thermal saturation. At 0 K, dissipation due to tunneling multiplies the tunneling probability by a factor that gets exponentially damped by friction, implying that, at this temperature, the behavior of spin bath is almost identical to that of a harmonic bath.

DOI
10.1103/physreve.84.041113

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The spin-bath induced decay of a quantum system out of a metastable state, which can tunnel and undergo thermal activation, is considered. The treatment is based on the c-number description of bath degrees of freedom and a canonical thermal distribution of the associated c-number variables. We show that, apart from the usual frequency prefactor and its dynamical modification in the spatial diffusion-limited regime, i.e., the Grote-Hynes factor, the rate coefficient contains two other factors. One is a quantum correction to the dynamical factor resulting from quantum transmission and reflection of the particle at the finite barrier. This term exhibits exponential rate enhancement at low temperature. The other one is a quantum corrected Arrhenius factor, which incorporates the effect of thermal saturation. At 0 K, dissipation due to tunneling multiplies the tunneling probability by a factor that gets exponentially damped by friction, implying that, at this temperature, the behavior of spin bath is almost identical to that of a harmonic bath.
The Kramers factor is the key nonequilibrium contribution to the decay rate of a metastable state of a system in contact with a thermal bath. In the 1980s Wolynes introduced a quantum equilibrium correction to the overall rate. This is responsible for tunnelling and quantum enhancement of rate at low temperature. Based on a quantum formulation of a system–reservoir model and a Wigner canonical thermal distribution function for the harmonic oscillator bath we suggest a generalization of the quantum equilibrium factor and a consequent rate expression which are valid in the deep tunnelling region.
This chapter considers one important physical example of that kind, quantum dissipative decay of a metastable state. It demonstrates how to evaluate the quantum decay rate of a metastable state for a quantum particle in the presence of dissipation. In the presence of phase fluctuations, however, such current states become unstable and decay simply because the “particle” can escape from the local potential minimum either by thermal activation or by quantum tunneling. The chapter also considers sufficiently low temperatures in which case the decay is due to quantum tunnelling. Classical process of thermally activated decay of supercurrent in Josephson junctions was first demonstrated in 1974, and the results turned out to be in a good agreement with theoretical predictions. Later experiments allowed to quantitatively verify a number of important theoretical predictions, for example, ones concerning the effect of temperature and damping on the quantum decay rate.
Usually one finds that dissipation tends to make a quantum system more classical in nature. We study the effect of momentum dissipation on a quantum system. The momentum of the particle is coupled bi-linearly to the momenta of a harmonic oscillator heat bath. For a harmonic oscillator system we find that the position and momentum variances for momentum coupling are, respectively, identical to momentum and position variances for spatial friction. This implies that momentum coupling leads to an increase in the fluctuations in position as the temperature is lowered, exactly the opposite of the classical-like localization of the oscillator, found with spatial friction. For a parabolic barrier, momentum coupling causes an increase in the unstable normal mode barrier frequency, as compared to the lowering of the barrier frequency in the presence of purely spatial coupling. This increase in the frequency leads to an enhancement of the thermal tunneling flux, which below the crossover temperature becomes exponentially large. The crossover temperature between tunneling and thermal activation increases with momentum friction so that quantum effects in the escape are relevant at higher temperatures.
Usually one finds that dissipation tends to make a quantum system more classical in nature. In this paper we study the effect of momentum dissipation on a quantum system. The momentum of the particle is coupled bilinearly to the momenta of a harmonic oscillator heat bath. For a harmonic oscillator system we find that the position and momentum variances for momentum coupling are respectively identical to momentum and position variances for spatial friction. This implies that momentum coupling leads to an increase in the fluctuations in position as the temperature is lowered, exactly the opposite of the classical like localization of the oscillator, found with spatial friction. For a parabolic barrier, momentum coupling causes an {\it increase} in the unstable normal mode barrier frequency, as compared to the lowering of the barrier frequency in the presence of purely spatial coupling. This increase in the frequency leads to an enhancement of the thermal tunneling flux, which below the crossover temperature becomes exponentially large. The crossover temperature between tunneling and thermal activation {\it increases} with momentum friction so that quantum effects in the escape are relevant at higher temperatures.
The problem of metastability due to quantum and thermal fluctuations in a weakly damped system is treated within Feynman's influence-functional theory. It is shown that quite generally the nonequilibrium density matrix may be written as a single path integral. For a cubic metastable potential it has the form of a Feynman propagator with a complex Lagrangian containing second-order derivatives in time and terms noninvariant under time reversal. Dissipative tunneling and thermal activation emerge together as different solutions of the associated Lagrange equations. The low-temperature correction to the exponent of the tunneling rate behaves as Tn+1{T}^{n+1}Tn+1 for a spectrum of bath excitations vanishing as ${\ensuremath{\omega}}^{n}$. It is shown, moreover, how this result may be understood in terms of environment-assisted tunneling. Thus the low-temperature behavior of the tunneling rate provides a method to measure the dissipation mechanism in the quantum regime.