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Physical Review Letters

Spontaneous Emission Suppression via Quantum Path Interference in Coupled Microcavities

Marc M. Dignam, David P. Fussell, Michael J. Steel, C. Martijn de Sterke, R. C. McPhedran

Published Mar 16, 2006• 20 citations
Publisher

Abstract

We examine theoretically the spontaneous emission rate in optical microstructures with cavity resonances that overlap in both position and frequency. Using projection techniques, we show that the spontaneous emission in such structures can be accurately described by the direct emission and quantum path interference of emission into a few discrete resonant modes, even though the exact infinite-dimensional problem involves a coupling to the continuum of radiation states. Moreover, we obtain an efficient numerical time-domain method for determining the spontaneous emission rate that incorporates these effects, including the suppression of spontaneous emission into some modes.

DOI
10.1103/physrevlett.96.103902

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Enhancement or suppression of spontaneous emission by the presence of a cavity has been a subject of numerous papers [1]. The effective number of radiation modes was estimated in terms of the cavity Q. Sachdev [2] has improved on this by an exact quantum Langevin treatment of a lossy, single-mode cavity and predicted a vacuum Rabi oscillation for high-Q cavities. Cook et al. [3] included retardation effects by incorporating multiple Fabry-Perot modes and treated the coupling loss by a heuristic introduction of the mirror reflectivity. The present author [4] has considered the same problem in perturbation and Wigner-Weisskopf approximations by use of a set of continuously distributed radiation modes which describes a cavity having output coupling.

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We examine theoretically the spontaneous emission rate in optical microstructures with cavity resonances that overlap in both position and frequency. Using projection techniques, we show that the spontaneous emission in such structures can be accurately described by the direct emission and quantum path interference of emission into a few discrete resonant modes, even though the exact infinite-dimensional problem involves a coupling to the continuum of radiation states. Moreover, we obtain an efficient numerical time-domain method for determining the spontaneous emission rate that incorporates these effects, including the suppression of spontaneous emission into some modes.
We consider spontaneous emission in dielectric microcavities with multiple resonances that may overlap in both position and frequency. By projecting the Green tensor onto a set of quasimodes associated with the resonances, we derive the reduced spontaneous emission rate. To demonstrate the accuracy and computational efficiency of our approach, we model spontaneous emission in a two-dimensional photonic crystal with two coupled defects. Employing a quantum mechanical interpretation, we show that the spontaneous emission involves both direct decay into the individual quasimodes and photon transfer between the quasimodes. The quantum path interference between these different emission channels can cause the spontaneous emission rate to differ dramatically from the rate obtained by the summation over resonant line shapes. We also show how our approach can be used to determine the emission into particular quasimodes of multiple-resonance microcavities.
Starting from a quantum Maxwell equation for the vector potential operator, we study the spontaneous emission properties of a two-level atom interacting with the electromagnetic field in a lossless and inhomogeneous dielectric structure and express the spontaneous emission rate, the external quantum efficiency, and the spontaneous emission factor in terms of the classical Green function of the dielectric structure. Comparing these results with the corresponding classical results, we show that the above quantities can be calculated from the radiation field of a classical dipole. Based on this correspondence, a numerical algorithm is developed to calculate the modification of spontaneous emission in microcavities. The line shape of the emission spectrum of the light source and the decay of the cavity resonant modes are automatically taken into account in this algorithm. The approximate expressions for the spontaneous emission rate and the spontaneous emission factor are discussed.
A complete set of cavity modes in planar dielectric microcavities is presented which naturally includes guided modes. We show that most of these orthonormal fields can be derived from a coherent superposition of plane waves incoming on the stack from the air and from the substrate. Spontaneous emission of a dipole located inside the microcavity is analyzed, in terms of cavity modes. Derivation of the radiation pattern in the air and in the substrate is presented. The power emitted into the guided modes is also determined. Finally, a numerical analysis of the radiative properties of an erbium atom located in a Fabry-P\'erot multilayer dielectric microcavity is investigated. We show that a large amount of light is emitted into the guided modes of the structure, in spite of the Fabry-P\'erot resonance, which increases the spontaneous emission rate in a normal direction. \textcopyright{} 1996 The American Physical Society.
Impressive progress has been achieved in controlling the spontaneous emission rate for emitters in Nanophotonic structures, such as microcavities, photonic crystals and nano-antennas. In all cases, however, the modification of the emission is stationary in time. Thus, the emission rate is time-independent and the distribution of photon emission times are stochastic and follow an exponential distribution in the weak coupling regime. In this paper, by using fast all-optical switching of a microcavity, the cavity resonance is tuned within tens of picosesonds. This drastically changes the local optical density of states at the emission frequency within the emission lifetime of the emitters. This paper theoretically studied an ensemble of two-level sources with a time dependent decay rate and have derived the excited state population and emitted intensity as a function of time for continuous wave and pulsed excitation. Deterministic bursts of dramatically enhanced or inhibited emission intensity within short intervals. Thereby, we control the photon distribution to show behavior that strongly deviates from single exponential decay. This can be used to protect quantum information systems against decoherence and to realize non-Markovian dynamics in cavity quantum electrodynamics.
Enhancement or suppression of spontaneous emission by the presence of a cavity has been a subject of numerous papers [1]. The effective number of radiation modes was estimated in terms of the cavity Q. Sachdev [2] has improved on this by an exact quantum Langevin treatment of a lossy, single-mode cavity and predicted a vacuum Rabi oscillation for high-Q cavities. Cook et al. [3] included retardation effects by incorporating multiple Fabry-Perot modes and treated the coupling loss by a heuristic introduction of the mirror reflectivity. The present author [4] has considered the same problem in perturbation and Wigner-Weisskopf approximations by use of a set of continuously distributed radiation modes which describes a cavity having output coupling.