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The Journal of Physical Chemistry A

On the Quenching of Rovibrationally Excited Molecular Oxygen at Ultracold Temperatures

N. Balakrishnan, A. Dalgarno

Published Feb 10, 2001• 41 citations
Publisher

Abstract

We report quantum mechanical scattering calculations of zero temperature quenching rate coefficients for vibrationally and rotationally excited O 2 in collisions with 3 He. It is found that vibrational energy is channeled into more specific rotational levels in the ultracold regime than at thermal energies where a broad range of rotational levels are populated. The influence of the van der Waals interaction on the low-temperature quenching rate coefficients and the possibility of trapping vibrationally excited O 2 by the buffer gas cooling technique are also discussed.

DOI
10.1021/jp0034224

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We report quantum mechanical scattering calculations of zero temperature quenching rate coefficients for vibrationally and rotationally excited O 2 in collisions with 3 He. It is found that vibrational energy is channeled into more specific rotational levels in the ultracold regime than at thermal energies where a broad range of rotational levels are populated. The influence of the van der Waals interaction on the low-temperature quenching rate coefficients and the possibility of trapping vibrationally excited O 2 by the buffer gas cooling technique are also discussed.
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We discuss the formation of molecular oxygen in ultracold collisions between hydroxyl radicals and atomic oxygen. A time-independent quantum formalism based on hyperspherical coordinates is employed for the calculations. Elastic, inelastic, and reactive cross sections as well as the vibrational and rotational populations of the product O2{\mathrm{O}}_{2}O2​ molecules are reported. A JJJ-shifting approximation is used to compute the rate coefficients. At temperatures T=10−−100mKT=10--100\phantom{\rule{0.3em}{0ex}}\mathrm{mK}T=10−−100mK for which the OH molecules have been cooled and trapped experimentally, the elastic and reactive rate coefficients are of comparable magnitude, while at colder temperatures, T<1mKT<1\phantom{\rule{0.3em}{0ex}}\mathrm{mK}T<1mK, the formation of molecular oxygen becomes the dominant pathway. The validity of a classical capture model to describe cold collisions of OH and O is also discussed. While very good agreement is found between classical and quantum results at T=0.3KT=0.3\phantom{\rule{0.3em}{0ex}}\mathrm{K}T=0.3K, at higher temperatures, the quantum calculations predict a larger rate coefficient than the classical model, in agreement with experimental data for the O+OH\mathrm{O}+\mathrm{O}\mathrm{H}O+OH reaction. The zero-temperature limiting value of the rate coefficient is predicted to be about $6\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}12}\phantom{\rule{0.3em}{0ex}}{\mathrm{cm}}^{3}\phantom{\rule{0.2em}{0ex}}{\text{molecule}}^{\ensuremath{-}1}\phantom{\rule{0.2em}{0ex}}{\mathrm{s}}^{\ensuremath{-}1}$, a value comparable to that of barrierless alkali-metal atom-dimer systems and about a factor of five larger than that of the tunneling dominated F+H2\mathrm{F}+{\mathrm{H}}_{2}F+H2​ reaction.
A quantum-mechanical investigation of the vibrational deactivation of ${}^{14}{\mathrm{N}}_{2}(\ensuremath{\nu}=1,{j}_{\mathrm{rot}}=j)$ in the ultracold collisions with 3He{}^{3}\mathrm{He}3He atoms is presented. Ab initio potential-energy calculations are carried out at BCCD(T) level and a global three-dimensional potential-energy surface is obtained by fitting ab initio points within the reproducing kernel Hilbert space method. Close coupling scattering calculations are performed at collision energy ranging from ${10}^{\ensuremath{-}6}$ to 2000 ${\mathrm{cm}}^{\mathrm{\ensuremath{-}}1}$. It is shown that the potential-energy surface supports a series of shape and Feshbach resonances. Their influence on the behavior of elastic and inelastic cross sections and quenching rate coefficients is discussed. It is demonstrated that, similar to the ${\mathrm{H}\mathrm{e}\ensuremath{-}\mathrm{O}}_{2}$ system, the rate coefficients exhibit three different regimes: Wigner regime at very low temperatures, van der Waals regime at intermediate temperatures due to series of resonances, and the usual rovibration--translation energy transfer regime at high temperatures.
We discuss the formation of molecular oxygen in ultracold collisions between hydroxyl radicals and atomic oxygen. A time-independent quantum formalism based on hyperspherical coordinates is employed for the calculations. Elastic, inelastic and reactive cross sections as well as the vibrational and rotational populations of the product O{sub 2} molecules are reported. A J-shifting approximation is used to compute the rate coefficients. At temperatures T = 10--100 mK for which the OH molecules have been cooled and trapped experimentally, the elastic and reactive rate coefficients are of comparable magnitude, while at colder temperatures, T < 1 mK, the formation of molecular oxygen becomes the dominant pathway. The validity of a classical capture model to describe cold collisions of OH and O is also discussed. While very good agreement is found between classical and quantum results at T = 0.3 K, at higher temperatures, the quantum calculations predict a higher rate coefficient than the classical model, in agreement with experimental data for the O + OH reaction. The zero-temperature limiting value of the rate coefficient is predicted to be about 6 x 10{sup -12} cm{sup 3} s{sup 01}, a value comparable to that of barrierless alkali metal atom-dimer systems and about a factor of five larger than that of the tunneling dominated F + H{sub 2} reaction.
The study of molecular inelastic collision processes at cold and ultracold temperatures is of considerable interest as schemes are currently being developed to efficiently cool and trap neutral polar molecules. In this work, quantum-mechanical scattering calculations are presented for the quenching of rotationally excited CO due to collisions with H, He and H 2 for collision energies between 10 −5 and 10 cm −1 . The calculations were performed using the close-coupling approach and the coupled-states approximation. Cross sections for the quenching of the j = 1–10, 20, 30 and 40 levels of CO are presented and mechanism and trends of energy transfer in these systems are discussed.