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Physical Review A

Recoil-induced optical Faraday rotation

B. Dubetsky, P. R. Berman

Published Oct 1, 1995• 10 citations
Publisher

Abstract

It is shown that, as a result of recoil during spontaneous emission, optical activity in a vapor can be induced under the action of resonant pump and probe fields. For field geometries that exclude other mechanisms for rotation of the probe field's plane of polarization, the recoil accompanying spontaneous emission provides the needed coupling between the spatial and internal atomic degrees of freedom to produce an optically active medium. A transition between ground and excited states, each having angular momentum $J=\frac{1}{2}$, is analyzed in detail. The effect can be interpreted as the result of pump field scattering off a spatial polarization grating of ground-state Zeeman coherence.

DOI
10.1103/physreva.52.r2519

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It is shown that, as a result of recoil during spontaneous emission, optical activity in a vapor can be induced under the action of resonant pump and probe fields. For field geometries that exclude other mechanisms for rotation of the probe field's plane of polarization, the recoil accompanying spontaneous emission provides the needed coupling between the spatial and internal atomic degrees of freedom to produce an optically active medium. A transition between ground and excited states, each having angular momentum J=12J=\frac{1}{2}J=21​, is analyzed in detail. The effect can be interpreted as the result of pump field scattering off a spatial polarization grating of ground-state Zeeman coherence.
We investigate an all-optical, pump-probe scheme for the polarization rotation of linearly polarized light in an atomic medium. A circularly polarized control light is shown to play the role of a static magnetic field via a Zeeman-like ac Stark interaction and to induce the optical Faraday rotation (OFR) of the probe light. As a model system, we consider a stationary atom with $nS\text{\ensuremath{-}}nP\text{\ensuremath{-}}nD$ level scheme without electronic or nuclear spin. In addition to OFR, we find that electromagnetically induced transparency for the three-level atom and circular dichroism also contribute to the polarization change. We characterize these three effects over different frequency ranges through an explicit calculation of the fractional transmission and the output polarization of the probe light. Our results are compared with the $nS\text{\ensuremath{-}}nP\text{\ensuremath{-}}(n+1)S$ scheme, which has been previously studied both theoretically and experimentally. We also compare the optically induced Faraday effect with the Faraday effect from a static magnetic field. We propose an experimental situation to test the theory and address the possibility of producing an atomic medium that is both optically active and transparent.
Theoretical calculations are presented for the probe absorption spectra of atoms having magnetically degenerate ground states which are subjected to weak pump fields that produce spatial polarization gradients. Apart from the Raman resonance contribution to the spectrum which has been observed experimentally, we predict that additional resonant structures should appear as a result of the atomic recoil that occurs during the absorption or emission of radiation by the atoms. The width of the atomic recoil resonances is directly related to the Doppler width associated with the driven transition. For sub-Doppler cooled atoms, the width can be much narrower than the optical pumping rate that determines the width of the Raman signal.
We demonstrate a type of chiral effect of an atomic medium. Polarization rotation of a probe beam is observed only when both a magnetic field and a linearly polarized coupling beam are present. We compare it with other chiral effects like optical activity, the Faraday effect, and the optically induced Faraday effect from the viewpoint of spatial inversion and time reversal transformations. As a theoretical model we consider a five-level configuration involving the cesium D2D2D2 transition. We use spin-polarized cold cesium atoms trapped in a magneto-optical trap to measure the polarization rotation versus probe detuning. The result shows reasonable agreement with a calculation from the master equation of the five-level configuration.
A theory of pump-probe spectroscopy is developed in which optical fields drive two-photon Raman transitions between ground states of an ensemble of three-level atoms. Effects related to the recoil the atoms undergo as a result of their interactions with the fields are fully accounted for in this theory. The linear absorption coefficient of a weak probe field in the presence of two pump fields of arbitrary strength is calculated. For subrecoil cooled atoms, the spectrum consists of eight absorption lines and eight emission lines. In the limit that ${\ensuremath{\chi}}_{1}\ensuremath{\ll}{\ensuremath{\chi}}_{2},$ where ${\ensuremath{\chi}}_{1}$ and ${\ensuremath{\chi}}_{2}$ are the Rabi frequencies of the two pump fields, one recovers the absorption spectrum for a probe field interacting with an effective two-level atom in the presence of a single pump field. However, when ${\ensuremath{\chi}}_{1}\ensuremath{\gtrsim}{\ensuremath{\chi}}_{2},$ new interference effects arise that allow one to selectively turn on and off some of these recoil-induced resonances.
Results of a fairly straightforward experiment on resonant magneto-optical rotation by rubidium-87 atoms revealed strong time-dependence of the polarization plane of light emerging from atomic vapors following a sudden irradiation with a laser beam. The rotation of the plane appears as a not direct consequence of the influence of the magnetic field on atoms. Reported measurements conducted using a vapor cell without any buffer gas or an anti-relaxation wall coating show that transmitted light has initially the same (linear) polarization as the incident one. Rotation of the polarization plane caused by an axial magnetic field develops in time scales similar to the pace of establishing the optical pumping/relaxation equilibrium in the atomic ensemble. The traditional passive Faraday rotation picture providing working description for the resonant magneto-optical effects in steady-state conditions does not explain the observed sequence of evolution of the polarization. The picture has to be augmented with analysis of time dependence in the spatial distribution of relevant quantum states within the atomic ensemble as well as longitudinal and transversal intensity profiles of the light beam. Isolation of external effects caused by the optical pumping and relaxation processes from consequences of internal atomic coherences should uncover more details of mechanisms of the latter in the presence of magnetic field. Plentitude of data available from time-dependent polarization measurements provides strong incentives for further development and tests of comprehensive models of coherent interactions of atomic ensembles with radiation and possibly a base for additional advance in understanding and applications of these phenomena.
We demonstrate a pump-probe scheme in which an atomic vapor is optically pumped with circularly polarized light and probed with a vector vortex beam. The pump induces a macroscopic magnetization in the medium, which gives rise to frequency-dependent circular dichroism and birefringence. The vortex probe, characterized by spatially varying polarization, maps this optical activity onto the spatial structure of the transmitted light, thereby generating correlations between the frequency, polarization, and spatial degrees of freedom. Measuring the intensity profile in a suitable polarization component then allows us to perform spatially resolved polarization spectroscopy. We demonstrate the translation of frequency shifts into an image rotation, observing on resonance a rotation in the order of 98 mrad per MHz. These findings may find applications in high-precision spectroscopy, magnetometry, and the generation of hybrid entanglement.