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Frontiers in Optics

Alignment Dynamics of Slow Light Diffusion in Ultracold Atomic 85Rb

Salim Balik, R. G. Olave, Charles I. Sukenik, Mark D. Havey, V. M. Datsyuk, Igor M. Sokolov, Dmitriy V. Kupriyanov

Published Jan 1, 2005• 2 citations
Publisher

Abstract

We report experimental and theoretical study of time-and polarization-dependent propagation of light in ultracold atomic Rb. Strong variations of the time-dependent electronic alignment in the vicinity of atomic resonance is measured.
DOI
10.1364/fio.2005.jwa87

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A combined experimental and theoretical investigation of time- and alignment-dependent propagation of light in an ultracold atomic gas of atomic 85Rb^{85}\mathrm{Rb}85Rb is reported. Coherences among the scattering amplitudes for light scattering off excited hyperfine levels produce strong variations of the light polarization in the vicinity of atomic resonance. Measurements are in excellent agreement with Monte Carlo simulations of the multiple scattering process.
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Probing the alignment of ultracold spin-polarized Rb2\textrm{Rb}_2Rb2​ molecules
We demonstrate a method to probe the alignment of the molecular axis of spin-polarized ultracold dimers. Diatomic 87^{87}87Rb2_22​ molecules are held in the lowest Bloch band of a far-off resonance 3D optical lattice. Using lattice modulation spectroscopy we measure the molecular polarizabilities, which are directly linked to the alignment, along each of the xxx-, yyy-, and zzz-directions of the lab coordinate system. In contrast to nonrotating molecules, we observe that rotating molecules have an anisotropic orientation of the molecular axis. Furthermore, we derive the dynamical polarizabilities for a laser wavelength of 1064.5 nm parallel and orthogonal to the molecular axis of the dimer, α∥=(8.9±0.9)×103 a.u.\alpha_\parallel=(8.9 \pm 0.9)\times10^3\:\textrm{a.u.}α∥​=(8.9±0.9)×103a.u. and α⊥=(0.9±0.4)×103 a.u.\alpha_\perp=(0.9 \pm 0.4)\times10^3\:\textrm{a.u.}α⊥​=(0.9±0.4)×103a.u., respectively.
We report a combined experimental and theoretical simulation of multiply scattered light dynamics in an ultracold gas of 85Rb atoms. Measurements of the spectral dependence of the time-decay of the scattered light intensity, following pulsed excitation with near resonance radiation, reveals that the decay for long times is nearly exponential, with a decay constant that is largely independent of detuning from resonance. Monte Carlo simulations of the multiple scattering process show that, for large detunings, near resonance scattering of Fourier components of the excitation pulse plays a significant role in the effect. This interpretation is supported by the observations, and successful modelling, of beating between Rayleigh scattered light at the excitation carrier frequency with the Fourier components of the excitation pulse that overlap significantly with the atomic resonance.
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