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Journal of Physics B Atomic Molecular and Optical Physics

Sum-frequency generation in an ultracold atomic gas due to collective atomic recoil

Gordon R. M. Robb, Brian W J McNeil

Published Oct 27, 2006• 1 citation
Publisher

Abstract

We describe a method for sum-frequency generation via non-degenerate four-wave mixing in classical (thermal) and quantum ultracold atomic gases (BEC). An integral part of the sum-frequency generation process is a collective instability which spontaneously generates a periodic density modulation in the atomic gas with a period comparable to the wavelength of the generated high-frequency optical field. Due to the generation of this density modulation, phase matching between the pump and generated fields is not a necessary initial condition for this sum-frequency generation process to occur: rather the density modulation acts to 'self-phase-match' the fields during the course of the sum-frequency generation process. We describe a one-dimensional model of this process, and suggest a proof-of-principle experiment to demonstrate a regime where the sum-frequency generation process evolves quantum mechanically, with discrete emission of sum-frequency photons. This experiment would involve pumping ultracold Cs atoms in a high-finesse unidirectional cavity with three infrared pump fields to produce blue light as a series of hyperbolic secant pulses.

DOI
10.1088/0953-4075/39/22/004

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We describe a method for sum-frequency generation via non-degenerate four-wave mixing in classical (thermal) and quantum ultracold atomic gases (BEC). An integral part of the sum-frequency generation process is a collective instability which spontaneously generates a periodic density modulation in the atomic gas with a period comparable to the wavelength of the generated high-frequency optical field. Due to the generation of this density modulation, phase matching between the pump and generated fields is not a necessary initial condition for this sum-frequency generation process to occur: rather the density modulation acts to 'self-phase-match' the fields during the course of the sum-frequency generation process. We describe a one-dimensional model of this process, and suggest a proof-of-principle experiment to demonstrate a regime where the sum-frequency generation process evolves quantum mechanically, with discrete emission of sum-frequency photons. This experiment would involve pumping ultracold Cs atoms in a high-finesse unidirectional cavity with three infrared pump fields to produce blue light as a series of hyperbolic secant pulses.
We describe a method for nondegenerate four-wave-mixing in a cold sample of four-level atoms. An integral part of the four-wave-mixing process is a collective instability which spontaneously generates a periodic density modulation in the cold atomic sample with a period equal to half of the wavelength of the generated high-frequency optical field. Because of the generation of this density modulation, phase matching between the pump and scattered fields is not a necessary initial condition for this wave-mixing process to occur; rather the density modulation acts to "self-phase match" the fields during the course of the wave-mixing process. We describe a one-dimensional model of this process, and suggest a proof-of-principle experiment which would involve pumping a sample of cold Cs atoms with three infrared pump fields to produce blue light.
Collective scattering of light due to atomic recoil, also known as collective atomic recoil lasing (CARL), occurs when a gas of atoms coherently scatters light from a pump laser via a collective instability. The scattering process can become unstable due to the atoms in the gas recoiling under the influence of the dynamic optical forces which arise due to the interference of the pump and scattered fields. The atoms move to form a spatially periodic density grating, which in turn amplifies the scattered field. This paper presents a theoretical analysis of CARL phenomena in degenerate ultracold gases of bosons and fermions. In the case of bosons i.e. in a Bose-Einstein Condensate (BEC),the effect of atom-atom interactions due to collisions on the CARL instability in the case of both attractive and repulsive condensates, is investigated. In the case of fermionic gases, the effect of Fermi pressure, is also presented. The linear and nonlinear evolution of the optical field and the atomic momentum distribution are considered for both cases.
An ensemble of periodically ordered atoms coherently scatters the light of an incident laser beam. The scattered and the incident light may interfere and give rise to a light intensity modulation and thus to optical dipole forces which, in turn, emphasize the atomic ordering. This positive feedback is at the origin of the collective atomic recoil laser (CARL). We demonstrate this dynamics using ultracold atoms confined by dipole forces in a unidirectionally pumped far red‐detuned high‐finesse optical ring cavity. Under the influence of an additional dissipative force exerted by an optical molasses the atoms, starting from an unordered distribution, spontaneously form a density grating moving at constant velocity. Additionally, steady state lasing is observed in the reverse direction if the pump laser power exceeds a certain threshold. We compare the dynamics of the atomic trajectories to the behavior of globally coupled oscillators, which exhibit phase transitions from incoherent to coherent states if the coupling strength exceeds a critical value.
We investigate the effect of a phase-modulated pump beam on collective backscattering [also termed collective atomic recoil lasing (CARL)] by a cold, collisionless atomic gas. We show using a numerical analysis that different regimes can be identified in which the atomic dynamics evolves in a qualitatively different manner during the light-atom interaction, depending on the magnitude of the pump modulation frequency. Our results also demonstrate that phase-modulating the pump field can substantially enhance the backscattered field intensity relative to the case of a monochromatic pump which has been used in CARL experiments to date.
Lasing [1, 2] and superradiance [3‐5] phenomena are currently enjoying a renaissance as research topics in atomic physics. Fundamentally based on the interaction of matter with an electromagnetic (light) field, the atomic dipoles in a “lasing medium” collectively emit into selected modes of the electromagnetic field and thereby create an amplified and coherent source of light. Present-day lasers use di erent types of gain media and cover a wide range of output frequencies for application in both, fundamental research and industry. A recent string of papers has reported on superradiance [6, 7] and lasing-type instabilities using Bose gases of various type (thermal atoms [8, 9], photon gases [10] and Bose-Einstein condensed atoms [11‐14]) in optical cavities. Buoyed by experimental control over essentially single excitation quanta of atoms and photons [15‐19] in cavity quantum electrodynamics, these works o er intriguing prospects for the next wave of experiments on strongly interacting light-mattter systems including a new regime where unexpected many-body and quantum fluctuation e ects of the lasing medium may become visible. Bohnet et al. [20] recently operated a superradiant “bad-cavity” laser in the few-photon regime based on coherent oscillations of the inter-atomic, collective dipole of the ultracold atoms in the cavity [21]. In this paper, we point out that a quantum degenerate Fermi gas has remarkable features as a lasing medium in a transversally driven cavity as sketched in Fig. 1. We show that the quantum statistics of the Fermi gas puts the coupled cavity+atoms system generically close to superradiance threshold as a consequence of the Pauli exclusion principle (“Pauli pressure”). Physically, this arises from enhanced scattering of fermions between di erent points on the Fermi surface with radiusjkFj by exchanging relatively large photon momenta Q from the cavity as illustrated in Fig. 1. By changing the power of the pump laser at a given density of the Fermi gas, the lasing transition is concomitant with the spontaneous formation of a charge density wave oscillating with 1=Q in real space. Tuning the ratiojkFj=jQj allows to generate a cavity spectrum with “broadband light” in certain spectral ranges or, for energies outside the particle-hole continuum of the fermions, light with relatively narrow linewidth. The normal mode splitting of the cavity by a single atom is completely replaced by many-body Ω |kF| Q
Subradiance, i.e., the cooperative inhibition of spontaneous emission by destructive interatomic interference, can be realized in a cold atomic sample confined in a ring cavity and lightened by a two-frequency laser. The atoms, scattering the photons of the two laser fields into the cavity mode, recoil and change their momentum. Under proper conditions the atomic initial momentum state and the first two momentum recoil states form a three-level degenerate cascade. A stationary subradiant state is obtained after the scattered photons have left the cavity, leaving the atoms in a coherent superposition of the three collective momentum states. Both a semiclassical description of the process and the quantum subradiant state with its Wigner function are given. Antibunching, quantum correlations, and entanglement between the atomic modes of the subradiant state are demonstrated.