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Journal of the Optical Society of America B

Nonlinear pulse deceleration using photorefractive four-wave mixing

Boris I. Sturman, P. Mathey, Riadh Rebhi, Hans Rudolf Jauslin

Published Sep 24, 2009• 11 citations
Publisher

Abstract

We investigate the possibilities of the backward four-wave coupling based on the nonlocal photorefractive response for the nonlinear deceleration of light pulses. The presence of an additional external variable parameter—the pump intensity ratio—allows to improve the output characteristics of the decelerated pulses compared to those typical of the two-wave coupling. In particular, large delay times of the output pulses can be achieved without their strong amplification. This positive distinctive feature of the pulse deceleration occurs far from threshold of the mirrorless optical oscillation.

DOI
10.1364/josab.26.001949

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We investigate the possibilities of the backward four-wave coupling based on the nonlocal photorefractive response for the nonlinear deceleration of light pulses. The presence of an additional external variable parameter—the pump intensity ratio—allows to improve the output characteristics of the decelerated pulses compared to those typical of the two-wave coupling. In particular, large delay times of the output pulses can be achieved without their strong amplification. This positive distinctive feature of the pulse deceleration occurs far from threshold of the mirrorless optical oscillation.
A slowing down of light pulses using backward-wave four-wave mixing is achieved in photorefractive crystals with different coupling strength. The delay and width of the output pulse are studied as a function of the input pulse width and pump intensity ratio for the amplified transmitted beam and for the phase-conjugated beam. The delay characteristics are compared with those of the two-beam coupling. It is demonstrated that the four-wave mixing process ensures a larger slowing down of short pulses (pulses with width shorter than the photorefractive response time) as compared to the photorefractive two-beam coupling scheme and guarantees the elimination of forerunners. The delay of long pulses in the four-wave mixing configuration is almost the same as the one that can be reached with two-beam coupling. The effect of absorption on the nonlinear shape transformation of the output pulses is discussed qualitatively.
We theoretically study the effect of light deceleration in photorefractive nonlinear media. This includes consideration of different types of the photorefractive nonlinear response, different wave interaction schemes, and an analysis of the influence of the input parameters, such as the input temporal pulse width and the coupling strength, on the output pulse characteristics: the time delay, the propagation velocity, the amplification factor, and the output width. We show that photorefractive light deceleration has numerous advantages over other known techniques. It works already at low intensities, at room temperature, and within wide spectral ranges and offers a vast variety of handles for manipulating light pulses. An analogy with the light deceleration method based on the quantum effect of electromagnetically induced transparency in ultracold resonant gases is also considered.
It is shown experimentally and theoretically that photorefractive wave coupling can be used for dramatic (< or approximately 0.025 cm/s) deceleration of light pulses whose width is larger than (or comparable with) the nonlinear response time. This classical nonlinear scheme exhibits similarities with the technique based on the quantum effect of electromagnetically induced transparency. The main distinctive feature of our scheme is amplification of the delayed output pulse. Advantages of the novel technique and its prospects for manipulation with light photons are discussed.
The slowing down of light pulses with backward-wave four-wave mixing is analyzed for photorefractive crystals with different coupling strengths. The conditions are found for which the delay of a phase-conjugate pulse decreases when the coupling strength increases and can even become negative, switching the pulse deceleration to acceleration. It is shown that for relatively low coupling strength the backward-wave four-wave mixing ensures a longer delay as compared to the two-beam-coupling technique. For coupling strengths tending to zero, the delay of long pulses approaches the response time of the medium. The conclusions of the theoretical analysis are confirmed experimentally with backward-wave four-wave mixing in barium titanate.
The nonlinear phase shift per unit length acquired by the transmitted and phase conjugate waves in backward-wave four-wave mixing may be considered as an effective refractive index. Consequently, a narrow spectrum of the nonlinear phase shift in non-degenerate frequency interaction corresponds to natural dispersion and such interaction may be used for temporal manipulation of light pulses. Analysis of the narrow spectra of the nonlinear phase shift shows high potential of the backward-wave four-wave for slowing down of light pulses. The slowing down is achieved using backward-wave four-wave mixing in media with local and nonlocal response. The delay and shape transformation of output pulses are studied and compared for the transmitted and phase conjugate channels. It is shown that the phase conjugate pulse achieves a longer delay under typical experimental conditions.
It has been shown recently (see, e.g., Nature, 397, 594, 1999; 409, 490, 2001) that light pulses can be remarkably slowed down in resonant gases under very low temperatures. We show theoretically and experimentally that a similar in nature (and stronger in value) phenomenon occurs in photorefractive nonlinear media. The pulse-maximum velocity can be reduced here to the value of thickness/response time because of the two wave coupling effect. Specific properties of pulse propagation depend on the type of the photorefractive response and also duration and shape of the input pulse. Our theoretical results for the nonlocal nonlinear response are in a good agreement with experimental data obtained with BaTiO3 and Sn2P2S6 crystals.