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IEEE Journal of Quantum Electronics

Coherent two-photon propagation and self-induced transparency of different frequency optical pulses through three-level system in potassium

N. Tan-no, Kenichi Yokoto, Humio Inaba

Published Jun 1, 1972• 2 citations
Publisher
DOI
10.1109/jqe.1972.1077028

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For pt.I see ibid., vol.8, no.3, 339 (1975). The transient behaviour of two short optical pulses in two-photon coherent propagation is obtained by calculating numerically the coherent propagation equations which couple the two electromagnetic pulses and the atomic system in self-consistent fashion. The coherent interaction of the two different frequency pulses gives rise to lossless propagation in the absorptive medium. This description is characterized by a two-photon area theorem. Novel coherent propagation effects of peak amplification and multiple pulse breakup are found. These effects are ascribed to two-photon self-induced transparency analogous to that of a one-photon transition in a two-level system. A difference of input intensity between the two different frequency pulses yields curious modulation effects involving sharp peak amplification and marked pulse breakup for the low-intensity input. In contrast, the high-intensity input pulse displays a smooth variation with distance and time. Low-loss pulse transmission above threshold, and pulse advance and delay are found for the present case in contrast to that for one-photon self-induced transparency.

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Coherent and phase-sensitive phenomena of ultrashort laser pulses propagating in three-level Λ -type systems studied with the finite-difference time-domain method

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Propagation of single- and two-color hyperbolic secant femtosecond laser pulses in a three-level $\ensuremath{\Lambda}$-type quantum system is investigated by solving the Maxwell and density matrix equations with the finite-difference time-domain and Runge-Kutta methods. As a first study of our modeling, we simulate pulse self-induced transparency (SIT) in two-level systems and see how this phenomenon can be controlled by manipulating the initial relative phase between the SIT pulse and a second control pulse, provided the ratio between both pulse frequencies obeys the relation ${\ensuremath{\omega}}_{1}∕{\ensuremath{\omega}}_{2}=3$. We then examine frequency down-conversion processes that are observed with single- and two-color pulses the envelope area of which is equal to or a multiple of $2\ensuremath{\pi}$, for pulse frequencies close to resonance with the transitions of a three-level $\ensuremath{\Lambda}$ medium. Also, phase-sensitive phenomena are discussed in the case of two-color $\ensuremath{\omega}\text{\ensuremath{-}}3\ensuremath{\omega}$ pulses propagating resonantly in the three-level system. In particular, possibilities for such coherent control are found for frequency down-conversion processes when the ratio of the frequencies of optical transitions is ${\ensuremath{\omega}}_{13}∕{\ensuremath{\omega}}_{12}=3$. The conditions for quantum control of four-wave mixing processes are also examined when the pulse frequencies of two-color $\ensuremath{\omega}\text{\ensuremath{-}}3\ensuremath{\omega}$ pulses are far from any resonance of the three-level system. We demonstrate the possibility to cancel the phase sensitivity of the four-wave coupling in a $\ensuremath{\Lambda}$-type system by competition effects between optical transitions.

Physical Review A•Jun 8, 2006•23 citations
For pt.I see ibid., vol.8, no.3, 339 (1975). The transient behaviour of two short optical pulses in two-photon coherent propagation is obtained by calculating numerically the coherent propagation equations which couple the two electromagnetic pulses and the atomic system in self-consistent fashion. The coherent interaction of the two different frequency pulses gives rise to lossless propagation in the absorptive medium. This description is characterized by a two-photon area theorem. Novel coherent propagation effects of peak amplification and multiple pulse breakup are found. These effects are ascribed to two-photon self-induced transparency analogous to that of a one-photon transition in a two-level system. A difference of input intensity between the two different frequency pulses yields curious modulation effects involving sharp peak amplification and marked pulse breakup for the low-intensity input. In contrast, the high-intensity input pulse displays a smooth variation with distance and time. Low-loss pulse transmission above threshold, and pulse advance and delay are found for the present case in contrast to that for one-photon self-induced transparency.
Propagation of single- and two-color hyperbolic secant femtosecond laser pulses in a three-level $\ensuremath{\Lambda}$-type quantum system is investigated by solving the Maxwell and density matrix equations with the finite-difference time-domain and Runge-Kutta methods. As a first study of our modeling, we simulate pulse self-induced transparency (SIT) in two-level systems and see how this phenomenon can be controlled by manipulating the initial relative phase between the SIT pulse and a second control pulse, provided the ratio between both pulse frequencies obeys the relation ${\ensuremath{\omega}}_{1}∕{\ensuremath{\omega}}_{2}=3$. We then examine frequency down-conversion processes that are observed with single- and two-color pulses the envelope area of which is equal to or a multiple of $2\ensuremath{\pi}$, for pulse frequencies close to resonance with the transitions of a three-level $\ensuremath{\Lambda}$ medium. Also, phase-sensitive phenomena are discussed in the case of two-color $\ensuremath{\omega}\text{\ensuremath{-}}3\ensuremath{\omega}$ pulses propagating resonantly in the three-level system. In particular, possibilities for such coherent control are found for frequency down-conversion processes when the ratio of the frequencies of optical transitions is ${\ensuremath{\omega}}_{13}∕{\ensuremath{\omega}}_{12}=3$. The conditions for quantum control of four-wave mixing processes are also examined when the pulse frequencies of two-color $\ensuremath{\omega}\text{\ensuremath{-}}3\ensuremath{\omega}$ pulses are far from any resonance of the three-level system. We demonstrate the possibility to cancel the phase sensitivity of the four-wave coupling in a $\ensuremath{\Lambda}$-type system by competition effects between optical transitions.