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Il Nuovo cimento della Società italiana di fisica. B/Il Nuovo cimento B

π/2 pulse shaping via analytic inversion of Bloch equations

Chang Jae Lee

Published Nov 1, 1993• 0 citations
Publisher
DOI
10.1007/bf02741281

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Journal of the Optical Society of America B•Jan 1, 1989•4 citations
An exact analytic solution to the time-dependent Schrödinger equation is presented for a two-state quantum system coherently driven by a nonresonant pulsed external field. The pulse has a hyperbolic-secant shape, with a sign jump (i.e. a phase step of π) at its maximum, which nullifies the overall pulse area. It is shown that off resonance, for detunings larger than the pulse bandwidth, the transition probability approaches unity as the field intensity increases. The population inversion is robust against small-to-moderate variations in the detuning and the intensity, a feature reminiscent of adiabatic passage. The population inversion, however, is not of adiabatic nature; it is induced by δ-function-shaped nonadiabatic coupling with an area of nearly π. An estimate of the required experimental resources shows that implementation with shaped femtosecond pulses is feasible.
The generation of an optical breather in coherent, resonant pulse propagation is studied. The initial field envelope is assumed to be in the form of a hyperbolic secant, with one half inverted so that the total area of the pulse is equal to zero. The Maxwell–Bloch equations for an inhomogeneously broadened atomic line are solved by the inverse-scattering method for all values of the independent variables x and t. The scattering amplitudes are found for any value θ of the absolute area of the initial pulse. For θ = 2πn the reflection coefficients are rational functions of the spectral parameter, and the inverse problem can be solved exactly. It is shown that the x-dependent poles of the reflection coefficients are responsible for the transient pulse shape. Such poles appear only in the presence of inhomogeneous broadening. The threshold for transparency is found at θ = 2π. At this value of the area, a breatherlike decaying solution is obtained. At θ = 4π a breather appears. Its energy amounts to approximately 70% of the initial pulse energy. For θ = 2π and 0 = 4π the solutions are analyzed in detail.