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Journal of Molecular Structure

Anticorrelation effects in raman scattering

Przemyslaw Szlachetka, S. Kielich, Jan Peřina, Vlasta Peřinová

Published Jan 1, 1980• 2 citations
Publisher
DOI
10.1016/0022-2860(80)85148-9

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Photon-photon and photon-phonon anticorrelation effects in Raman scattering are studied theoretically. The Heisenberg equations of motion describing Raman scattering are solved in the short-time approximation. The laser, Stokes, anti-Stokes and phonon modes are quantised. The joint normally ordered characteristic functions are evaluated for modes exhibiting anticorrelation effects. The problem of existence of a Glauber-Sudarshan quasi-distribution function related to anticorrelation effects is considered. The magnitude of the anticorrelation effects depends on the initial statistical properties of the photon and phonon modes.
The quantum theory of the statistical properties and the photocount statistics of intense radiation in Raman scattering are presented making use of the coherent-state techniques. Both the Heisenberg-Langevin and Fokker-Planck equations approaches are developed. The existence of the conditional Glauber-Sudarshan quasi-distribution is also discussed. The time dependences of the photocount distribution and its factorial moments are demonstrated in the case of stimulated scattering and anticorrelation and antibunching of scattered photons are found.