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Journal of Physics A Mathematical and Theoretical

Amplitudes for multiphoton quantum processes in linear optics

Jesús Urı́as

Published Jun 30, 2011• 4 citations
Publisher

Abstract

The prominent role that linear optical networks have acquired in the engineering of photon states calls for physically intuitive and automatic methods to compute the probability amplitudes for the multiphoton quantum processes occurring in linear optics. A version of Wick's theorem for the expectation value, on any vector state, of products of linear operators, in general, is proved. We use it to extract the combinatorics of any multiphoton quantum processes in linear optics. The result is presented as a concise rule to write down directly explicit formulae for the probability amplitude of any multiphoton process in linear optics. The rule achieves a considerable simplification and provides an intuitive physical insight about quantum multiphoton processes. The methodology is applied to the generation of high-photon-number entangled states by interferometrically mixing coherent light with spontaneously down-converted light.

DOI
10.1088/1751-8113/44/30/305303

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The prominent role that linear optical networks have acquired in the engineering of photon states calls for physically intuitive and automatic methods to compute the probability amplitudes for the multiphoton quantum processes occurring in linear optics. A version of Wick's theorem for the expectation value, on any vector state, of products of linear operators, in general, is proved. We use it to extract the combinatorics of any multiphoton quantum processes in linear optics. The result is presented as a concise rule to write down directly explicit formulae for the probability amplitude of any multiphoton process in linear optics. The rule achieves a considerable simplification and provides an intuitive physical insight about quantum multiphoton processes. The methodology is applied to the generation of high-photon-number entangled states by interferometrically mixing coherent light with spontaneously down-converted light.
Advances in the production of multiple-photon states with a broadband spectrum and its subsequent processing through linear optical systems demand simple rules to automate the calculation of probability amplitudes. A methodology to write down directly the probability amplitude of any broadband multi-photon process in linear optics is proved. A physically intuitive notion of multi-photon paths is derived from Wick's theorem and amplitudes are formulated as sums over paths. Every permutation of the out-state photon frequencies over the photon occupation indices that the in-state wavepacket assigns to the inports contributes a path. A simple general rule is provided to compute them. Broadband two-photon processes in the interferometers by Hong, Ou and Mandel (HOM) and by Mach and Zehnder (MZ) are considered. We provide a rigorous description of the HOM interferometer as a probe of the amount of frequency entanglement contained in some two-photon wavepackets, establishing an integral transform between the interference profile and the spectral density of frequency-entangled photon pairs. For the MZ interferometer, our method provides the exact rate of coincidence counts for a broadband two-photon process that is relevant for pairs produced with a wide two-dimensional spectral bandwidth by spontaneous parametric downconversion.
Abstract We have developed a theory for accessing quantum coherences in mutually unbiased bases associated with generalized Pauli operators in multiphoton multimode linear optics networks (LONs). We show a way to construct complementary Pauli measurements in multiphoton LONs and establish a theory for evaluation of their photonic measurement statistics without dealing with the computational complexity of Boson samplings. This theory extends characterization of complementary properties in single-photon LONs to multiphoton LONs employing convex-roof extension. It allows us to detect quantum properties such as entanglement using complementary Pauli measurements, which reveals the physical significance of entanglement between modes in bipartite multiphoton LONs.
Entangled photons are a crucial resource for linear optical quantum communication and quantum computation. Besides the remarkable progress of photon state engineering using atomic memories (Kimble (2008); Yuan et al. (2008)) the majority of current experiments is based on the production of photon pairs in the process of spontaneous parametric down-conversion (SPDC), where the entangled photon pair is concluded from post-selection of randomly occurring coincidences. Here we present new insights into the heralded generation of photon states (Barz et al. (2010); Wagenknecht et al. (2010)) that are maximally entangled in polarization (Schrodinger (1935)) with linear optics and standard photon detection from SPDC (Kwiat et al. (1995)). We utilize the down-conversion state corresponding to the generation of three pairs of photons, where the coincident detection of four auxiliary photons unambiguously heralds the successful preparation of the entangled state (Śliwa & Banaszek (2003)). This controlled generation of entangled photon states is a significant step towards the applicability of a linear optics quantum network (Nielsen & Chuang (2000)), in particular for entanglement distribution (Bennett et al. (1996)), entanglement swapping (Kaltenbaek et al. (2009); Pan et al. (1998)), quantum teleportation (Bouwmeester et al. (1997)), quantum cryptography (Bennett & Brassard (1984); Ekert (1991); Jennewein et al. (2000)) and scalable approaches towards photonics-based quantum computing schemes (Browne & Rudolph (2004); Gottesman & Chuang (1999); Knill et al. (2001)).
Photons are natural carriers of quantum information due to their ease of distribution and long lifetime. This thesis concerns various related aspects of quantum information processing with single photons. Firstly, we demonstrate N-photon entanglement generation through a generalised N X N symmetric beam splitter known as the Bell multiport. A wide variety of 4-photon entangled states as well as the N-photon W-state can be generated with an unexpected non-monotonic decreasing probability of success with N. We also show how the same setup can be used to generate multiatom entanglement. A further study of multiports also leads us to a multiparticle generalisation of the Hong-Ou-Mandel dip which holds for all Bell multiports of even number of input ports. Next, we demonstrate a generalised linear optics based photon filter that has a constant success probability regardless of the number of photons involved. This filter has the highest reported success probability and is interferometrically robust. Finally, we demonstrate how repeat-until-success quantum computing can be performed with two distant nodes with unit success probability using only linear optics resource. We further show that using non-identical photon sources, robustness can still be achieved, an illustration of the nature and advantages of measurement-based quantum computation. A direct application to the same setup leads naturally to arbitrary multiphoton state generation on demand. Finally, we demonstrate how polarisation entanglement of photons can be detected from the emission of two atoms in a Young's double-slit type experiment without linear optics, resulting in both atoms being also maximally entangled.
This thesis presents results under the topics of quantum correlations and quantum information processing using linear-optical networks. The first part of this thesis concerns with quantum correlations, specially in Gaussian states, which play a central role as resource in quantum protocols. The second part is about quantum information processing using linear-optical networks that are of great practical interest due to their simple physical realization. In the first part, we present a measurement-based method for verifying nonzero quantum discord, a measure of quantum correlations, in bipartite systems that can be used for both continuous and discrete-variable systems. Based on this method, we show that the only bipartite Gaussian states with zero quantum discord are product states. We also present a simple and efficient experimental method for verifying quantum correlations in Gaussian states using homodyne measurements. Moreover, we introduce an operational measure for quantifying quantum correlations in Gaussian states that is purely based on Gaussian measurements. We then illustrate the operational significance of the measure in terms of a Gaussian quantum protocol. In the second part, we present results on linear quantum-optics experiments, specifically boson sampling, an intermediate model of quantum computation that can be implemented using single-photon states, linear-optical networks, and photodetectors. We first present an efficient experimental method for characterization of linear-optical networks, which is essential for practical implementation of boson sampling. We show that using coherent states one can directly measure all the nontrivial phases and moduli of the matrix describing the network. Next, we consider the problem of boson sampling with Gaussian states. We derive a general formula for calculating the output photon-counting probabilities. We show that for input thermal states, sampling from the output probability distribution can be efficiently classically simulated. Using this, we find that permanents of positive-semidefinite Hermitian matrices can be approximated to within a multiplicative error in BPPNP. We also discuss boson sampling with squeezed vacuum states. Finally, we provide a sufficient condition for the efficient classical simulation of the general sampling problem using linear-quantum optics, which involves a multimode input quantum state to a linear-optical network and set of measurements at the output. This condition is based on the phase-space quasiprobability distributions, and suggests that negativity is a quantum resource. We apply this condition to implementations of boson sampling using single-photon or spontaneous parametric down-conversion sources. We show that above some threshold for loss and noise in the experiment, boson sampling is classically simulatable.