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Journal of Physics B Atomic Molecular and Optical Physics

High densities and optical collisions in a two-colour magneto-optical trap for metastable helium

Jeroen C. J. Koelemeij, A. S. Tychkov, T. Jeltes, W. Hogervorst, W. Vassen

Published Aug 25, 2004• 7 citations
Publisher

Abstract

We have studied a cloud of cold metastable helium (He*) atoms interacting with near-resonant light at 1083 nm and 389 nm. The 1083 nm light allows for efficient loading of a large magneto-optical trap (MOT) and the 389 nm light is subsequently used to increase the density and reduce the temperature of the He* cloud during a brief compression stage. Cold collisions in the cloud yield ions and fast metastables which are monitored separately using calibrated microchannel plate (MCP) detectors. We thus measure absolute production rates of ions and fast metastables escaping from the MOT during the various stages of the experiment. We observe that 389 nm optical collisions, apart from Penning ionization, produce a relatively large flux of fast metastables, which we relate to the short-range behaviour of the molecular potentials involved. Furthermore, by rapidly switching between 389 nm and 1083 nm the ratio between the respective two-body loss rate constants is determined. Using these values, together with the observed time dependence of the cloud size, the temporal behaviour of the absolute ion production rate during the compression stage is well reproduced.

DOI
10.1088/0953-4075/37/17/007

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This thesis describes the work done over the past three and a half years on the new metastable helium experiment at the Institut d'Optique in Palaiseau. In the first chapter it describes a study to improve both the efficiency and the accuracy of the Microchannel Plate (MCP) detection system. We have experimented with adding a gold layer on the top of the input plate, something that we have found increases the efficiency but also decreases the accuracy. The addition of a voltage between the two stacked plates has been shown to both raise the efficiency and improve the accuracy in non-coated MCPs.The second chapter is devoted to the construction of the experimental apparatus. Here the excitation of ground state helium to its metastable state is described, as well as the subsequent collimation and cooling by Zeeman slower of the resulting hot atomic beam. The slowed beam is then captured in a Magneto-Optical Trap, in which we have captured 8x108 atoms.In the third chapter an original study on three-dimensional Doppler cooling in a red-detuned molasses and in the Magneto-Optical trap is presented. The metastable helium system is unique as there is no multiple scattering of photons and there are no sub-Doppler effects. This allows for a never before seen experimental realisation of pure Doppler cooling theory. The fourth chapter describes a study on collisions in a magneto-optical trap of metastable helium. Light-induced Penning collisions are responsible for high trap losses at high intensities and at frequencies close to the transition frequency. We measure the constant rate coefficient to Ksp = 2.8 ± 0.4 x 10-7cm3/s.

•Oct 3, 2014•0 citations
We have studied a cloud of cold metastable helium (He*) atoms interacting with near-resonant light at 1083 nm and 389 nm. The 1083 nm light allows for efficient loading of a large magneto-optical trap (MOT) and the 389 nm light is subsequently used to increase the density and reduce the temperature of the He* cloud during a brief compression stage. Cold collisions in the cloud yield ions and fast metastables which are monitored separately using calibrated microchannel plate (MCP) detectors. We thus measure absolute production rates of ions and fast metastables escaping from the MOT during the various stages of the experiment. We observe that 389 nm optical collisions, apart from Penning ionization, produce a relatively large flux of fast metastables, which we relate to the short-range behaviour of the molecular potentials involved. Furthermore, by rapidly switching between 389 nm and 1083 nm the ratio between the respective two-body loss rate constants is determined. Using these values, together with the observed time dependence of the cloud size, the temporal behaviour of the absolute ion production rate during the compression stage is well reproduced.
We have studied the optical collisions of cold, metastable helium atoms in a magneto-optical trap. We have detected the rate of Penning and associative ionization of two metastable helium atoms at a temperature of 1 mK with and without nearly resonant light. We find that the associative ionization rate is increased with more than a factor 20 due to the presence of the light field. We present a simple, semiclassical model, which accounts for all the observed features, and which agrees, also on an absolute scale, with our experimental results.
About 10 4 triplet metastable helium atoms have been trapped in a magneto-optical trap, based on the 2 3 S 1 –2 3 P 2 transition at 1.083 μm (volume 0.1 mm 3 , temperature 1 mK). The losses of the trap are analysed by monitoring the ion current due to Penning collisions either with background gases, or between trapped atoms. The rate coefficient for these collisions between trapped metastable helium atoms has been found to be unusually large, and the crucial role of the quasi-resonant laser light has been experimentally demonstrated. The rate coefficient of the dominant process (He*(2 3 S 1 ) + He*(2 3 P 2 ) Penning collisions) has been measured by two different methods, and found to be K sp ≃ 10 -7 cm 3 s -1 within an estimated factor of 4. The corresponding cross-section is 6 · 10 6 Å 2 .
We describe a powerful scheme which combines laser cooling on two transitions of metastable helium to obtain a high phase-space density. By running a sequence of a large 1083nm1083\phantom{\rule{0.3em}{0ex}}\text{nm}1083nm magneto-optical trap (MOT) and a compressed 389nm389\phantom{\rule{0.3em}{0ex}}\text{nm}389nm MOT, a density increase of more than one order of magnitude is achieved within 5ms5\phantom{\rule{0.3em}{0ex}}\text{ms}5ms. After compression, $8\ifmmode\times\else\texttimes\fi{}{10}^{8}$ atoms at a central density of $5\ifmmode\times\else\texttimes\fi{}{10}^{10}\phantom{\rule{0.3em}{0ex}}{\text{cm}}^{\ensuremath{-}3}$ remain, while the temperature of the cloud has been reduced from 1mK1\phantom{\rule{0.3em}{0ex}}\text{mK}1mK to 0.4mK0.4\phantom{\rule{0.3em}{0ex}}\text{mK}0.4mK. The resulting phase-space density $(4.1\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}6})$ is more than one order of magnitude higher than what we achieved by 1083nm1083\phantom{\rule{0.3em}{0ex}}\text{nm}1083nm laser cooling only.
We have constructed a magneto-optical trap (MOT) for metastable triplet helium atoms utilizing the $2{}^{3}{S}_{1}\ensuremath{\rightarrow}3{}^{3}{P}_{2}$ line at 389 nm as the trapping and cooling transition. The far-red-detuned MOT (detuning $\ensuremath{\Delta}=\ensuremath{-}41\mathrm{MHz})$ typically contains few times 107{10}^{7}107 atoms at a relatively high $(\ensuremath{\sim}{10}^{9}{\mathrm{cm}}^{\ensuremath{-}3})$ density, which is a consequence of the large momentum transfer per photon at 389 nm and a small two-body loss rate coefficient $(2\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}10}{\mathrm{cm}}^{3}/\mathrm{s}<\ensuremath{\beta}<1.0\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}9}{\mathrm{cm}}^{3}/\mathrm{s}).$ The two-body loss rate is more than five times smaller than in a MOT on the commonly used $2{}^{3}{S}_{1}\ensuremath{\rightarrow}2{}^{3}{P}_{2}$ line at 1083 nm. Furthermore, laser cooling at 389 nm results in temperatures somewhat lower than those achieved using 1083 nm. The 389-nm MOT exhibits small losses due to two-photon ionization, which have been investigated as well.
We report loading of $1.5\ifmmode\times\else\texttimes\fi{}{10}^{9}$ metastable triplet helium atoms in a large magneto-optical trap, using far-red-detuned laser beams. We fully characterized this trap by measuring trap losses and absorption of a probe beam. From the highly nonexponential trap decay we derive Penning ionization loss rate coefficients for two detunings: $5.3(9)\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}9}{\mathrm{cm}}^{3}/\mathrm{s}$ at $\ensuremath{-}35\mathrm{MHz}$ and $3.7(6)\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}9}{\mathrm{cm}}^{3}/\mathrm{s}$ at $\ensuremath{-}44\mathrm{MHz}.$ Also, we find that the loss rate is maximum at $\ensuremath{-}5\mathrm{MHz}$ detuning, where the rate is $1.3(3)\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}8}{\mathrm{cm}}^{3}/\mathrm{s},$ much larger than recent theoretical and experimental values. In the absence of light the $S\ensuremath{-}S$ ionization rate constant is measured to be $1.3(2)\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}10}{\mathrm{cm}}^{3}/\mathrm{s}.$
This thesis describes the work done over the past three and a half years on the new metastable helium experiment at the Institut d'Optique in Palaiseau. In the first chapter it describes a study to improve both the efficiency and the accuracy of the Microchannel Plate (MCP) detection system. We have experimented with adding a gold layer on the top of the input plate, something that we have found increases the efficiency but also decreases the accuracy. The addition of a voltage between the two stacked plates has been shown to both raise the efficiency and improve the accuracy in non-coated MCPs.The second chapter is devoted to the construction of the experimental apparatus. Here the excitation of ground state helium to its metastable state is described, as well as the subsequent collimation and cooling by Zeeman slower of the resulting hot atomic beam. The slowed beam is then captured in a Magneto-Optical Trap, in which we have captured 8x108 atoms.In the third chapter an original study on three-dimensional Doppler cooling in a red-detuned molasses and in the Magneto-Optical trap is presented. The metastable helium system is unique as there is no multiple scattering of photons and there are no sub-Doppler effects. This allows for a never before seen experimental realisation of pure Doppler cooling theory. The fourth chapter describes a study on collisions in a magneto-optical trap of metastable helium. Light-induced Penning collisions are responsible for high trap losses at high intensities and at frequencies close to the transition frequency. We measure the constant rate coefficient to Ksp = 2.8 ± 0.4 x 10-7cm3/s.