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AIP conference proceedings

Quantum Coherence in Nano-and Micro-Photonics

Salvatore Savasta, Dmitry N. Chigrin

Published Jan 1, 2011• 0 citations
Publisher

Abstract

The principle of complementarity refers to the ability of quantum entities to behave as particles or waves under different experimental conditions. I discuss a recently proposed device enabling the ultrafast all optical control of the wave‐particle duality of light. It is constituted by a three‐level quantum emitter strongly coupled to a microcavity and can be realized by exploiting a great variety of systems ranging from atomic physics and semiconductor quantum dots to intersubband polaritons and Cooper pair boxes. Control pulses with specific arrival times, performing which‐path and quantum‐eraser operations, are able to destroy and recover interference almost instantaneously. I will also discuss quantum coherence effects and more generally the optical properties of ultracompact (with dimensions below the diffraction limit) hybrid structures, composed of metallic nanoparticles and a single quantum dot. The coupling between a single quantum emitter and a metallic nanoparticle can give rise to a Fano interference effect which strongly influences the quantum statistical properties of the scattered photons.

DOI
10.1063/1.3644210

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The principle of complementarity refers to the ability of quantum entities to behave as particles or waves under different experimental conditions. I discuss a recently proposed device enabling the ultrafast all optical control of the wave‐particle duality of light. It is constituted by a three‐level quantum emitter strongly coupled to a microcavity and can be realized by exploiting a great variety of systems ranging from atomic physics and semiconductor quantum dots to intersubband polaritons and Cooper pair boxes. Control pulses with specific arrival times, performing which‐path and quantum‐eraser operations, are able to destroy and recover interference almost instantaneously. I will also discuss quantum coherence effects and more generally the optical properties of ultracompact (with dimensions below the diffraction limit) hybrid structures, composed of metallic nanoparticles and a single quantum dot. The coupling between a single quantum emitter and a metallic nanoparticle can give rise to a Fano interference effect which strongly influences the quantum statistical properties of the scattered photons.
Recently a device enabling the ultrafast all-optical control of the wave-particle duality of light was proposed [Ridolfo et al., Phys. Rev. Lett. 106, 013601 (2011)]. It is constituted by a three-level quantum emitter strongly coupled to a microcavity and can be realized by exploiting a great variety of systems ranging from atomic physics and semiconductor quantum dots to intersubband polaritons and Cooper pair boxes. Control pulses with specific arrival times, performing which-path and quantum-eraser operations, are able to destroy and recover interference almost instantaneously. Here we show that the coherence sudden death implies the sudden birth of a higher order correlation function storing coherence. Such storing enables coherence rebirth after the arrival of an additional suitable control pulse. We derive analytical calculations describing the all-optical control of the wave-particle duality and the entanglement-induced switch-off of the strong coupling regime. We also present analytical calculations describing a homodynelike method exploiting pairs of phase locked pulses with precise arrival times to probe the optical control of wave-particle duality of this system. Within such a method the optical control of wave-particle duality can be directly probed by just detecting the photons escaping the microcavity.
The principle of complementarity refers to the ability of quantum entities to behave as particles or waves under different experimental conditions. We present a proposal for the experimental observation of the ultrafast all-optical control of the wave-particle duality of light. The device is constituted by a three-level quantum emitter strongly coupled to a microcavity (MC) and can be realized by exploiting a great variety of systems, ranging from atomic physics and semiconductor quantum dots to intersubband polaritons and Cooper pair boxes. The wavelike or particlelike behavior of MC photons can be probed by simply measuring the cavity output photon rate after excitation with pairs of phase-locked weak pulses with precise arrival times.
ABSTRACT. We study theoretically the quantum optical properties of hybrid artificial molecules composed of an individual quantum emitter and a metallic nanoparticle. The coupling between the two systems can give rise to a Fano interference effect which strongly influences the quantum statistical properties of the scattered photons: a small frequency shift of the incident light field may cause changes in the intensity correlation function of the scattered field of orders of magnitude. The system opens a good perspective for applica-tions in active metamaterials and ultracompact single-photon devices. We also demonstrate with accurate scattering calculations that a system constituted by a single quantum emitter (a semiconductor quantum dot) placed in the gap between two metallic nanoparticles can display the vacuum Rabi splitting. 1.
We study theoretically the quantum optical properties of hybrid molecules composed of an individual quantum dot and a metallic nanoparticle. We calculate the resonance fluorescence of this composite system. Its incoherent part, arising from nonlinear quantum processes, is enhanced by more than 2 orders of magnitude as compared to that of the dot alone. The coupling between the two systems gives rise to a Fano interference effect which strongly influences the quantum statistical properties of the scattered photons: a small frequency shift of the incident light field may cause changes in the intensity correlation function of the scattered field of orders of magnitude. The system opens a good perspective for applications in active metamaterials and ultracompact single-photon devices.
Optically controlled dipole-dipole interaction at submicrometers and subwavelength scales leads to many interesting phenomenon and remarkable potential applications in quantum optics, condensed matter physics, and today’s micro-devices. In this dissertation, we study the applications of quantum optical coherence to nano-optics in the following systems and aspects. On the one hand, chiral metamaterials has been previously reported as excellent candidates to realize both attractive and repulsive Casimir forces, where the existence of a repulsive Casimir force depends upon the strength of the chirality. On the other hand, nanoscale integration of metal nanoparticles and semiconductors is particularly interesting because the strengths of both materials are combined in such a hybrid system. In the first part of this work, we proposed a technical scheme to coherently control of the Casimir interaction energy with two identical chirality mediums. We took explicit caution regarding the requirements of passivity and causal response of the materials, since these requirements are essential for the application of the Lifshitz formula. The rare-earth metals’ atomic species, for instance, dysprosium, is proposed as an applicable medium for the forthcoming studies of possible experimental implementation of our technique. Secondly, we fully investigated the coherent control of the quantum optical properties of spontaneous emission spectra of a semiconductor quantum dot coupled to a metallic nanoparticle. The properties of the spontaneous emission spectra of such a system are studied in detail with and without involving the coherent field. The Rabi splitting effect in the spectrum emitted by the quantum dot under particular conditions is predicted for different sizes of the metal nanoparticles. We show that the spontaneous emission spectra of the transition coupled to surface plasmons may be further modified by adjusting the external coherent control on the adjacent transitions. In the third part, we propose a robust protocol to study the entanglement generation in a hybrid structure consisting of two quantum dots in the proximity of a metallic nanoshell. The entanglement arises impulsively due to common coupling to the plasmonic nanostructure, without demanding postselective measurement or mediating the dissipative environment. The long-lived entangled states can be created deterministically by optimizing the shell thickness as well as the ratio of the distances between the quantum dots and the surface of the shell. The loss of the system is greatly reduced even when the quantum dots are ultraclose to the shell, which signifies a slow decay rate of the coherence information and longtime entanglement preservation.
We discuss the optical bistability and multistability properties of incident light on a unidirectional ring cavity consisting of a hybrid semiconductor quantum dot-metal nanoparticle system driven by coupling and incoherent pumping fields. We consider the quantum dot system as a three-level V-type configuration which is placed near the metallic nanoparticle. We realize that the threshold of optical bistability and optical multistability can be controlled by tuning the center-to-center distance between quantum dots and metallic nanoparticles. Moreover, the effect of incoherent pumping field on optical bistability and optical multistability has been discussed for different distances between quantum dots and metallic nanoparticles.