A new kind of quantum interference between Raman scattering and single-photon absorption is predicted theoretically, which gives an expanded view of quantum interference. Its potential application is also proposed.
We report on the observation of a new magic frequency within the hyperfine structure of the D2 line of 87Rb atoms at which the scattering of light into a high-finesse cavity is suppressed by an interplay between quantum interference and the strong collective coupling of atoms to the cavity. Scattering from a cloud of laser-driven cold atoms into the cavity was measured in a polarization sensitive way. We have found that both the Rayleigh and Raman scattering processes into the near-resonant cavity modes are extinguished at 185 MHz below the F=2↔F'=3 transition frequency. This coincidence together with the shape of the observed spectral dip imply that the effect relies on a quantum interference in the polariton excitations of the strongly coupled combined atom-photon system. We have also demonstrated the existence of a magic frequency around -506 MHz, where only the Raman scattering is suppressed due to a quantum interference effect at the single-atom level.
This Letter reports all-optically tunable and highly indistinguishable single Raman photons from a driven single quantum dot spin. The frequency, linewidth, and lifetime of the Raman photons are tunable by varying the driving field power and detuning. Under continuous-wave excitation, subnatural linewidth single photons from off-resonant Raman scattering show an indistinguishability of 0.98(3). Under π pulse excitation, spin- and time-tagged Raman fluorescence photons show an almost vanishing multiphoton emission probability of 0.01(2) and a two-photon quantum interference visibility of 0.95(3). Lastly, Hong-Ou-Mandel interference is demonstrated between two single photons emitted from remote, independent quantum dots with an unprecedented visibility of 0.87(4).