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Journal de Physique Lettres

Detection of optical resonances by observation of fluorescence light emitted from a fast atomic beam when optical pumping occurs

H. T. Duong, Jean Vialle

Published Jan 1, 1980• 1 citation
Publisher

Abstract

The sensitivity of the method of detection of optical resonances by observation of the fluorescence light emitted from a fast beam excited by a laser in collinear geometry is often limited by the optical pumping. In our method, we propose to take advantage of the optical pumping process to detect optical resonances by using a second laser beam in almost collinear geometry which acts as a detector of optical pumping.

DOI
10.1051/jphyslet:019800041017040700

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The sensitivity of the method of detection of optical resonances by observation of the fluorescence light emitted from a fast beam excited by a laser in collinear geometry is often limited by the optical pumping. In our method, we propose to take advantage of the optical pumping process to detect optical resonances by using a second laser beam in almost collinear geometry which acts as a detector of optical pumping.
The detection of optical resonances by observation of the fluorescence light emitted from a fast atomic beam of Na interacting with a collinear laser beam is limited in sensitivity by optical pumping processes. In the experiment reported here, we take advantage of the optical pumping by using a second collinear laser beam, achieving then a gain in fluorescence signal. The effects of the lasers power and polarization on line shapes have been studied in the single laser excitation case as well as in the two laser beams one.
The use of highly monochromatic light permits the selective excitation of atoms in vapors if excitation and detection of the fluorescence is carried out collinearly. The atoms capable of absorbing light then form an atomic beam of well-defined velocity along the direction of the laser beam, but no velocity selection occurs perpendicular to it. The potential of the technique for Doppler-free atomic spectroscopy and for the study of excited atom collisions is demonstrated by using the Na D1 line as an example.
The use of highly monochromatic light permits the selective excitation of atoms in vapors if excitation and detection of the fluorescence is carried out collinearly. The atoms capable of absorbing light then form an atomic beam of well-defined velocity along the direction of the laser beam, but no velocity selection occurs perpendicular to it. The potential of the technique for Doppler-free atomic spectroscopy and for the study of excited atom collisions is demonstrated by using the Na D1 line as an example.
An apparatus has been constructed to produce well-characterized fast beams of rare gas metastable atoms for subsequent scattering experiments. Optical pumping by a collinear laser beam can be used to selectively remove either of the two metastable components from the beam. Laser-induced-fluorescence (LIF) techniques can be used to determine the original beam composition and to monitor composition changes resulting from optical absorption. These techniques have been successfully applied to a metastable neon beam produced by near-resonant charge transfer of Ne+ in Na. A simple model has been developed which accurately reproduces the observed LIF lineshape generated by tuning the laser throught the optical transition frequency.