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Physical Review B

Exciton states and their entanglement in coupled quantum dots

Jia‐Lin Zhu, Weidong Chu, Zhensheng Dai, Dong Xu

Published Oct 28, 2005• 22 citations
Publisher

Abstract

Exciton states and optical spectra in a pair of vertically stacked $\mathrm{InGaAs}∕\mathrm{GaAs}$ quantum dots are studied with a proposed variation-diagonalization technique. The spectra obtained are in good agreement with experiments. The tunnel coupling and the exciton entanglement are also investigated. It is found that at short barrier widths, the entanglement is small due to the coupling between the intradot and interdot orbitals. At large barrier widths, large entanglement appears in coupled identical quantum dots; however, such an entanglement can be easily destroyed by the broken symmetry because of the weak tunneling of the hole.

DOI
10.1103/physrevb.72.165346

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Exciton states and optical spectra in a pair of vertically stacked InGaAs∕GaAs\mathrm{InGaAs}∕\mathrm{GaAs}InGaAs∕GaAs quantum dots are studied with a proposed variation-diagonalization technique. The spectra obtained are in good agreement with experiments. The tunnel coupling and the exciton entanglement are also investigated. It is found that at short barrier widths, the entanglement is small due to the coupling between the intradot and interdot orbitals. At large barrier widths, large entanglement appears in coupled identical quantum dots; however, such an entanglement can be easily destroyed by the broken symmetry because of the weak tunneling of the hole.
We calculate the excitonic structure of pairs of GaAs/AlGaAs quantum dots forming lateral molecules and obtain the entanglement of exciton states. The following advantages of the lateral geometry over the vertical one are found: (1) The energy structures of the dots forming a molecule can be in principle identical. (2) Comparable tunneling of electrons and holes ensures a high entanglement of antisymmetric excitons. A drawback of existing structures are very low tunneling energies, which make the entanglement vulnerable against differences in the sizes and shapes of both dots.
Currently there is strong interest in realizing implementations of quantum computation and quantum cryptography in a solid state environment. One of the systems that are actively studied are semiconductor quantum dots (QDs). Due to their discrete energy level structure, they are often called artificial atoms, and they attract immediately interest of quantum information science since they allow to mimic the design developed for atomic physics systems such as ions in traps or atoms in cavities. However, despite of the similarities, one has to keep in main that any elementary excitation in a QD has a generic many-body character. An essential building block of a quantum processor is a quantum gate which entangles the states of two quantum bits. Recently it has been proposed that a pair of vertically aligned QDs could be used as an optically driven quantum gate: The quantum bits are individual carriers either on dot zero or dot one. The different dot indices play the same role as a "spin," therefore we term them "isospin." Quantum mechanical tunneling between the dots rotates the "isospin" and leads to superposition of two quantum dot states. The quantum gate is built when two different particles, an electron and a hole, are created optically. The two particles form entangled isospin states. The entanglement can be controlled by application of an electric field along the heterostructure growth direction. Here we present spectroscopic studies on single quantum dot molecules (QDMs) with different vertical separation between the dots that support the feasibility of this proposal. The comparison of the evolution of the excitonic recombination spectrum with the results of calculations allows us to demonstrate coherent tunneling of electrons and holes across the separating barrier and the formation of entangled exciton states. For a given barrier width, we find only small variations of the tunneling induced splitting between the entangled states demonstrating a good homogeneity within the obtained QDM ensembles.
Recently a pair of vertically aligned quantum dots has been suggested as optically driven quantum gate. The later is built when two different particles, an electron and a hole, are created optically. The two particles form entangled states. We study theoretically the dynamics of a single heavy hole exciton confined in a small vertically coupled quantum dot. We use harmonic potentials to model the confining of electrons and holes and calculate the exciton's energy spectrum using the Hund-Mulliken approach, and including the Coulomb interaction. The entanglement may be controlled by the application of external electric field. At certain times of dynamical evolution one can generate a maximally entangled coherent exciton state by initially preparing the quantum dots in a superposition of coherent state. In ideal situations, entangled quantum states would not decohere during processing and transmission of quantum information. However, a real quantum system is inevitably influenced by its environment. Since, we study the decoherence effect caused by the interaction of the confined carriers with the acoustic phonon effects. (© 2004 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim)
Exciton-biexciton coherent coupling effects are examined in semiconductor quantum dots. The exciton absorption spectrum is measured with the microphotoluminescence excitation technique in a single InGaAs quantum dot. The spectrum changes from a Lorenztian-type line shape to an unusual dip-shaped line shape with increasing excitation intensities in a higher exciton state where there is a large oscillator strength between the exciton and biexciton states. The intensity dependence of the dip energy width clearly indicates that coherent Rabi oscillation occurs between the exciton and biexciton states. The absorption properties with excitation light of different polarizations show that the dip-shaped spectra only appear when there is a large biexciton state population with linear polarization. A theoretical analysis undertaken with the density matrix method agrees well with experimental results. This agreement reveals that exciton-biexciton coherent interactions lead to unusual absorption spectra and contribute crucially to the optical properties of quantum dots. The exciton-biexciton coherent effects provide a scheme for controlling four distinguishable states, which can be applied to a demonstration of quantum gate operations.