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Physics Letters A

gJ Factors of the 6s6p 3P1 and 6s6p 1P1 states of ytterbium

M. Baumann, G. Wandel

Published Nov 1, 1968• 19 citations
Publisher
DOI
10.1016/0375-9601(68)90200-4

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We report the magneto-optical trapping of ytterbium atoms using the 6s2 1S0-6s6p 3P1 intercombination transition. The magneto-optical trap is continuously loaded from an atomic beam decelerated by a Zeeman-tuned atomic-beam slower operated at the 6s2 1S0-6s6p 1P1 transition. Among seven stable isotopes of ytterbium, six isotopes of 170Yb, 171Yb, 172Yb, 173Yb, 174Yb, and 176Yb are successfully trapped. The number and density of the trapped atoms are about 108 and 1011 cm-3, respectively. The temperature of atoms is estimated to be about 20 μK from the time-of-flight measurement. The decay time of the trapped atoms after stopping the loading of atoms is about 3 s.

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The electronic transitions of ytterbium atoms in a solid Xe matrix grown at 4.8 K are investigated. Absorption bands are detected in the regions of the gas-phase 6s2 1S0 → 4f135d6s2 and 6s2 1S0 → 6s6p 1P1 transitions. Both bands indicate that Yb atoms occupy multiple trapping sites, of which three are identified. Emission induced by the 6s2 1S0 → 6s6p 1P1 excitation is found to be concentrated entirely in the region of the 6s6p 3PJ → 6s2 1S0 decay, whereas the singlet emission is completely quenched. Multiple emission peaks are observed and the effects of annealing and prolonged irradiation on their amplitudes are found to be significant and are interpreted as a consequence of Yb population transfer from one type of site to another. Modeling of the ground-state site structure and stability predicts three Yb/Xe occupation types, substitutional (ss), tetravacancy (tv) and hexavacancy (hv), in order of decreasing stability. Their tentative associations with observed absorption and emission features are discussed. Time correlated single photon spectroscopy is used to determine the lifetimes of the individual emission bands. They are found to be different from each other with indications of a mixture of short- and long- lived 6s6p 3PJ fine-structure components and demonstrate distinct temperature dependencies. A dramatic decrease in the lifetime of the emission peak tentatively assigned to the most stable site with temperature is explained by a competition between the radiative and non-radiative decay paths of the 6s6p 3P1 state. The mechanism of the latter can be attributed to electron–phonon coupling as confirmed by a model of the temperature-dependence of the lifetime.

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An evaluation of the gJ factors of the lowest states of Rb and Cs

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We report the magneto-optical trapping of ytterbium atoms using the 6s2 1S0-6s6p 3P1 intercombination transition. The magneto-optical trap is continuously loaded from an atomic beam decelerated by a Zeeman-tuned atomic-beam slower operated at the 6s2 1S0-6s6p 1P1 transition. Among seven stable isotopes of ytterbium, six isotopes of 170Yb, 171Yb, 172Yb, 173Yb, 174Yb, and 176Yb are successfully trapped. The number and density of the trapped atoms are about 108 and 1011 cm-3, respectively. The temperature of atoms is estimated to be about 20 μK from the time-of-flight measurement. The decay time of the trapped atoms after stopping the loading of atoms is about 3 s.
HYPERFINE STRUCTURE OF THE 6s6psup3sup 3sup3Psub1sub 1sub1 STATE OF sup171sup 171sup171Yb AND sup173sup 173sup173Yb.
The electronic transitions of ytterbium atoms in a solid Xe matrix grown at 4.8 K are investigated. Absorption bands are detected in the regions of the gas-phase 6s2 1S0 → 4f135d6s2 and 6s2 1S0 → 6s6p 1P1 transitions. Both bands indicate that Yb atoms occupy multiple trapping sites, of which three are identified. Emission induced by the 6s2 1S0 → 6s6p 1P1 excitation is found to be concentrated entirely in the region of the 6s6p 3PJ → 6s2 1S0 decay, whereas the singlet emission is completely quenched. Multiple emission peaks are observed and the effects of annealing and prolonged irradiation on their amplitudes are found to be significant and are interpreted as a consequence of Yb population transfer from one type of site to another. Modeling of the ground-state site structure and stability predicts three Yb/Xe occupation types, substitutional (ss), tetravacancy (tv) and hexavacancy (hv), in order of decreasing stability. Their tentative associations with observed absorption and emission features are discussed. Time correlated single photon spectroscopy is used to determine the lifetimes of the individual emission bands. They are found to be different from each other with indications of a mixture of short- and long- lived 6s6p 3PJ fine-structure components and demonstrate distinct temperature dependencies. A dramatic decrease in the lifetime of the emission peak tentatively assigned to the most stable site with temperature is explained by a competition between the radiative and non-radiative decay paths of the 6s6p 3P1 state. The mechanism of the latter can be attributed to electron–phonon coupling as confirmed by a model of the temperature-dependence of the lifetime.