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Optica Acta International Journal of Optics

Effect of Detuning on Squeezing in Two-atom Resonance Fluorescence

Thomas Richter

Published Sep 1, 1984• 8 citations
Publisher

Abstract

The exact steady-state solution is presented for the reduced atomic density operator describing the cooperative resonance fluorescence from a system of two atoms separated by an arbitrary distance in an off-resonance laser field, with the dipole-dipole near-field interaction between the atoms included. It is shown that the destructive effect of the dipole-dipole interaction on the formation of squeezing in two-atom resonance fluorescence found recently by Ficek et al. can be compensated to a very large extent by an appropriate choice of the detuning between the laser frequency and the single-atom transition frequency.

DOI
10.1080/713821613

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Resonance fluorescence of a two-level atom in an off-resonance squeezed vacuum

Z. Ficek, Barry C. Sanders

The authors present analytical and numerical results for resonance fluorescence produced by a two-level atom damped by a broad-band squeezed vacuum. Previous theoretical analyses of this model have assumed that the laser frequency and the carrier frequency of the squeezed vacuum are equal. The authors introduce a non-zero detuning between the laser frequency and the carrier frequency while maintaining resonance between the laser frequency and atomic resonance. In the absence of the driving field there is a squeezing threshold: above threshold the decay rate of the atomic polarization can be reduced, and below threshold a squeezing-induced two peak spectrum and frequency shift, which is analogous to the Bloch-Siegert shift, are predicted. In the presence of the driving field, the spectrum is asymmetric for Rabi frequencies smaller or comparable to the detuning of the squeezed vacuum. A symmetric spectrum is obtained for large Rabi frequencies. An interpretation is predicted by means of a dressed-state analysis. The authors find that for not too large Rabi frequencies a remarkably large population inversion can be induced in the dressed states, even at exact resonance of the driving field, provided that the laser frequency and carrier frequency are detuned. Moreover, for detection times larger than the inverse detuning, the spectrum is insensitive to the phase between the driving field and the squeezed vacuum, in marked contrast to the case of no detuning.

Journal of Physics B Atomic Molecular and Optical Physics•Feb 28, 1994•21 citations
The exact steady-state solution is presented for the reduced atomic density operator describing the cooperative resonance fluorescence from a system of two atoms separated by an arbitrary distance in an off-resonance laser field, with the dipole-dipole near-field interaction between the atoms included. It is shown that the destructive effect of the dipole-dipole interaction on the formation of squeezing in two-atom resonance fluorescence found recently by Ficek et al. can be compensated to a very large extent by an appropriate choice of the detuning between the laser frequency and the single-atom transition frequency.
The cooperative resonance fluorescence radiation from two atoms separated by an arbitrary distance and driven by a coherent laser field is studied, taking into account the dipole-dipole near-field interaction. The steady-state total scattering intensity, as a function of laser frequency and field strength, differs considerably from the single-atom one for sufficiently small distances. Photon bunching and antibunching occur in the scattered radiation depending on the laser frequency. Practically a full antibunching effect is found, especially if the laser is tuned to resonance with a transition frequency of the two-atom system. This is in contrast to a recent result of Agarwal et al., who studied the two-atom system but neglected the frequency splitting due to the dipole-dipole near-field interaction.
The equal-time intensity correlation function and variances of the in-phase and out-of-phase components of the electric field radiated by a system of two interacting atoms in the process of resonance fluorescence are calculated analytically for arbitrary values of the field strength, interatomic interaction, and detuning and are illustrated graphically. It is shown that not only photon antibuching but also squeezing can occur in two-atom resonance fluorescence. The influence of dipole-dipole interaction between the atoms on both nonclassical effects is discussed. It is shown that a considerable amount of photon antibunching and squeezing can be obtained for finite detuning of the laser frequency from atomic resonance, especially when the detuning and dipole-dipole interaction parameters cancel out mutually. The maximum value of squeezing for interacting atoms is shown to be less, however, than that for noninteracting atoms. Very strong dipole-dipole interaction reduces the squeezing effect to zero.
In this Comment we study the resonance fluorescence of a system of two atoms separated by an arbitrary distance RRR in an on-resonance laser field. The steady-state spectrum is calculated in the strong-field limit both for negligible and for non-negligible dipole-dipole interaction. The singlet state of the system is included throughout, even for small interatomic separations. We show that the so-called "scaling factor," or the enhancement of the integrated fluorescence by NNN atoms (above the expected factor of NNN), predicted in the literature by many authors, does not, in fact, exist.
The influence of the dipole-dipole interaction on the final atomic state of a two-atom system driven by a coherent laser field and damped by a broad-band squeezed vacuum is discussed. It is shown that in the absence of a coherent laser field the final atomic state is independent of the dipole-dipole interaction and can be the pure two-atom squeezed state only if detuning of the squeezed vacuum field from atomic resonance is equal to zero. In the presence of a coherent laser field, the final atomic state depends on the dipole-dipole interaction. As the latter increases, the final atomic state shifts from a mixed state to the pure two-atom squeezed state. However, this happens only if the driving field and the squeezed field frequencies are tuned to the atomic transition frequency. For the driving field and the squeezed vacuum field frequencies detuned from atomic resonance the system decays into a mixed state irrespective of the dipole-dipole interaction between the atoms.
The spectrum of resonance fluorescence and the second-order correlation function are calculated for a system of two identical two-level cooperative systems interacting via the dipole-dipole interaction. The results are valid for arbitrary incident-field strengths and for atomic separations much less than the resonant wavelength. The intensity of the sidebands at the Rabi frequency is diminished by the dipole interaction, whereas that of the sidebands at twice the Rabi frequency is enhanced. Both the cooperative behavior and the dipole-dipole interaction act to diminish the photon antibunching, as shown by the second-order correlation function.
The authors present analytical and numerical results for resonance fluorescence produced by a two-level atom damped by a broad-band squeezed vacuum. Previous theoretical analyses of this model have assumed that the laser frequency and the carrier frequency of the squeezed vacuum are equal. The authors introduce a non-zero detuning between the laser frequency and the carrier frequency while maintaining resonance between the laser frequency and atomic resonance. In the absence of the driving field there is a squeezing threshold: above threshold the decay rate of the atomic polarization can be reduced, and below threshold a squeezing-induced two peak spectrum and frequency shift, which is analogous to the Bloch-Siegert shift, are predicted. In the presence of the driving field, the spectrum is asymmetric for Rabi frequencies smaller or comparable to the detuning of the squeezed vacuum. A symmetric spectrum is obtained for large Rabi frequencies. An interpretation is predicted by means of a dressed-state analysis. The authors find that for not too large Rabi frequencies a remarkably large population inversion can be induced in the dressed states, even at exact resonance of the driving field, provided that the laser frequency and carrier frequency are detuned. Moreover, for detection times larger than the inverse detuning, the spectrum is insensitive to the phase between the driving field and the squeezed vacuum, in marked contrast to the case of no detuning.