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Optics and Spectroscopy

Effects of inversionless lasing in two-level media from the point of view of specificities of the spatiotemporal propagation dynamics of radiation

Mikhail V. Arkhipov, Rostislav M. Arkhipov, S. A. Pulkin

Published Jun 1, 2013• 6 citations
Publisher

Abstract

We report the results of computer simulation of the emission of radiation by an extended two-level medium in a ring cavity. The cases of using strong external monochromatic, quasi-monochromatic, and biharmonic radiation for pumping the two-level medium are analyzed. It is shown that the emission of radiation with spectral content different from that of the pump radiation, which is interpreted as the inversionless oscillation, is the result of the spatiotemporal dynamics of light propagation in an extended two-level medium imbedded in a cavity. The appearance of this radiation is not related to known resonances of amplification of a weak probe field in a thin layer of the two-level system (the effect of inversionless oscillation) induced by strong resonance monochromatic or biharmonic field, as was thought before.

DOI
10.1134/s0030400x13060015

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We report the results of computer simulation of the emission of radiation by an extended two-level medium in a ring cavity. The cases of using strong external monochromatic, quasi-monochromatic, and biharmonic radiation for pumping the two-level medium are analyzed. It is shown that the emission of radiation with spectral content different from that of the pump radiation, which is interpreted as the inversionless oscillation, is the result of the spatiotemporal dynamics of light propagation in an extended two-level medium imbedded in a cavity. The appearance of this radiation is not related to known resonances of amplification of a weak probe field in a thin layer of the two-level system (the effect of inversionless oscillation) induced by strong resonance monochromatic or biharmonic field, as was thought before.
We report a theoretical study on the possibility of amplification and generation of radiation by an inversionless two-level system in the ‘red’ wing of its spectral line under resonant diode pumping. The two-level system is used to simulate atoms of an active gas, while it is in the atmosphere of a high-pressure buffer gas. The effect results from the fact that the probability of stimulated emission in the ‘red’ wing of the spectral line exceeds the probability of absorption if the homogeneous broadening due to the interaction of particles with the buffer gas significantly exceeds the natural one (at high pressures of the buffer gas). It is found that the higher the buffer gas pressure and the higher the pump radiation intensity, the greater the inversionless amplification. It is shown that the gain in a two-level system in the ‘red’ wing of its spectral line can reach 0.011 cm −1 when the radiation intensity and the width of the radiation spectrum of pump diodes are 5 kW cm −2 and 4 cm −1 , respectively. The use of transverse diode pumping of an active medium placed in an optical cavity will make it possible to obtain lasing with frequency tuning and thereby solve the problem of converting incoherent broadband radiation into a coherent laser light in a gas of two-level active particles.
Amplification of probe radiation by an inversionless two-level system in the 'red' wing of its spectral line is studied theoretically during the resonance absorption of intense cw laser radiation. The effect is caused by the inequality of the spectral densities of the Einstein coefficients for absorption and stimulated emission outside the absorption line under conditions when homogeneous broadening, due to the interaction of particles with the buffer gas, significantly exceeds the natural broadening (at high pressures of the buffer gas). It is found that the larger the inversionless gain, the higher the buffer gas pressure and the pump radiation intensity. It is established that at high enough pump intensity, the probe field is amplified along the entire region of the 'red' wing of the line (at any negative detunings of the probe field frequency).
Generation of coherent multifrequency optical radiation by means of excitation of mechanical vibration (acoustical oscillation) of a medium along the propagation of resonant laser radiation is proposed. At the same time the vibrating medium becomes transparent for the incident resonant radiation (acoustically induced transparency). We show, that generation of multifrequency radiation takes place in the absence of inversion in two-level quantum system for any energy distribution among the spectral components of the incident (multifrequency in general) field and any amplitude of vibration. Amplitude of vibration determines efficiency of the normal wave generation. Mechanism of the effect is destructive interference of different spectral harmonics of the field components appearing in the frame of vibrating atoms.
The transmission spectra of inversionless amplification are investigated. Propagation of a weak probe optical beam through a three-level medium pumped with a microwave strong beam is numerically modeled. Three various schemes of transitions under the conditions providing the amplification of the probe field without inversion are taken to calculate the atomic polarization, which enters the paraxial wave equations. Diffraction and self-action ofbeams due to nonlinear absorption and refraction are properly taken into account. These effects together with linear absorption and refraction form a complex distribution of gain across the beams. As a result the amplified beam acquires ring transverse patterns and slight asymmetry in the frequency characteristics.
We consider a three-level medium with low-frequency separation between the two upper levels. The medium interacts with an external field that induces a coherence between the two upper levels. We analyze the amplification condition for the probe monochromatic optical field in a general nonresonant case. We show that amplification without population inversion arises either at line center or at the sidebands, depending on the sign of the population difference between the upper sublevels. This amplification occurs in a limited range of the coherent pump intensity.