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Journal of Applied Physics

Absence of Ordering in Certain Isotropic Systems

Michael F. Thorpe

Published Mar 15, 1971• 30 citations
Publisher

Abstract

The method of Mermin and Wagner [Phys. Rev. Lett. 17, 1133 (1966)] is used to show that one- and two-dimensional spin systems interacting with a general isotropic interaction H=12 ∑ ijn Iij(n) (Si·Sj)n,where the exchange interactionsIij(n) are of finite range, cannot order in the sense that 〈Oi〉=0for all traceless operators Oi defined at a single site i. Mermin and Wagner have proved the above for the case n = 1 with Oi = Si, i.e., for the Heisenberg Hamiltonian. The proof allows us to rule out the possibility that a small isotropic biquadratic exchange (Si·Sj)2 could induce ferromagnetism or antiferromagnetism in a two-dimensional Heisenberg system.

DOI
10.1063/1.1660265

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The method of Mermin and Wagner [Phys. Rev. Lett. 17, 1133 (1966)] is used to show that one- and two-dimensional spin systems interacting with a general isotropic interaction H=12 ∑ ijn Iij(n) (Si·Sj)n,where the exchange interactionsIij(n) are of finite range, cannot order in the sense that 〈Oi〉=0for all traceless operators Oi defined at a single site i. Mermin and Wagner have proved the above for the case n = 1 with Oi = Si, i.e., for the Heisenberg Hamiltonian. The proof allows us to rule out the possibility that a small isotropic biquadratic exchange (Si·Sj)2 could induce ferromagnetism or antiferromagnetism in a two-dimensional Heisenberg system.
It is rigorously proved that at any nonzero temperature, a one- or two-dimensional isotropic spin-SSS Heisenberg model with finite-range exchange interaction can be neither ferromagnetic nor antiferromagnetic. The method of proof is capable of excluding a variety of types of ordering in one and two dimensions.
Some measurements have shown that the second-order exchange interaction is non-negligible in ferromagnetic compounds whose microscopic interactions are described by means of half-odd integer quantum spins. In these spin systems the ground state is either ferromagnetic or antiferromagnetic when the bilinear exchange interaction is dominant. Instead, in ferromagnetic systems characterized by bilinear and biquadratic exchange interactions of comparable magnitude, the energy minimum occurs when spins are in a canting ground-state. To this aim, a one-dimensional (1D) quantum spin chain and a two-dimensional (2D) lattice of quantum spins subjected to periodic boundary conditions are modeled via the generalized quantum Heisenberg Hamiltonian containing, in addition to the isotropic and short-range bilinear exchange interaction of the Heisenberg type, a second-order interaction, the isotropic and short-range biquadratic exchange interaction between nearest-neighbors quantum spins. For these 1D and 2D quantum systems a generalization of the Mermin–Wagner–Hohenberg theorem (also known as Mermin–Wagner–Berezinksii or Coleman theorem) is given. It is demonstrated, by means of quantum statistical arguments, based on Bogoliubov’s inequality, that, at any finite temperature, (1) there is absence of long-range order and that (2) the law governing the vanishing of the order parameter is the same as in the bilinear case for both 1D and 2D quantum ferromagnetic systems. The physical implications of the absence of a spontaneous spin symmetry breaking in 1D spin chains and 2D spin lattices modeled via a generalized quantum Heisenberg Hamiltonian are discussed.
The Mermin-Wagner theorem is strengthened so as to rule out magnetic long-range order at T>0T>0T>0 in one- or two-dimensional Heisenberg and XY systems with long-range interactions decreasing as ${R}^{\ensuremath{-}\ensuremath{\alpha}}$ with a sufficiently large exponent $\ensuremath{\alpha}$. For oscillatory interactions, ferromagnetic long-range order at T>0T>0T>0 is ruled out if $\ensuremath{\alpha}\ensuremath{\ge}1(D\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}1)$ or $\ensuremath{\alpha}>5/2(D\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}2)$. For systems with monotonically decreasing interactions, ferro- or antiferromagnetic long-range order at T>0T>0T>0 is ruled out if $\ensuremath{\alpha}\ensuremath{\ge}2D$.
We look at the general SU(2) invariant spin-1 Heisenberg model. This family includes the well-known Heisenberg ferromagnet and antiferromagnet as well as the interesting nematic (biquadratic) and the largely mysterious staggered-nematic interaction. Long range order is proved using the method of reflection positivity and infrared bounds on a purely nematic interaction. This is achieved through the use of a type of matrix representation of the interaction making clear several identities that would not otherwise be noticed. Using the reflection positivity of the antiferromagnetic interaction one can then show that the result is maintained if we also include an antiferromagnetic interaction that is sufficiently small.