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Physical Review A

Brownian Motion of a Quantum Oscillator

G. S. Agarwal

Published Aug 1, 1971• 208 citations
Publisher

Abstract

The theory of Brownian motion of a quantum oscillator is developed. The Brownian motion is described by a model Hamiltonian which is taken to be the one describing the interaction between this oscillator and a reservoir. Use is made of the master equation recently derived by the author, to obtain the equation of motion for the various reduced phase-space distribution functions that are obtained by mapping the density operator onto $c$-number functions. The equations of motion for the reduced phase-space distribution functions are found to be of the Fokker-Planck type. On transforming the Fokker-Planck equation to real variables, it is found to have the same form as the Fokker-Planck equation obtained by Wang and Uhlenbeck to describe the Brownian motion of a classical oscillator. The Fokker-Planck equation is solved for the conditional probability (Green's function) which is found to be in the form of a two-dimensional Gaussian distribution. This solution is then used to obtain various time-dependent quantum statistical properties of the oscillator. Next, the entropy for a quantum oscillator undergoing Brownian motion is calculated and we show that this system approaches equilibrium as $t\ensuremath{\rightarrow}\ensuremath{\infty}$. Finally we show that in the weak-coupling limit the Fokker-Planck equation reduces to the one obtained by making the usual rotating-wave approximation.

DOI
10.1103/physreva.4.739

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The theory of Brownian motion of a quantum oscillator is developed. The Brownian motion is described by a model Hamiltonian which is taken to be the one describing the interaction between this oscillator and a reservoir. Use is made of the master equation recently derived by the author, to obtain the equation of motion for the various reduced phase-space distribution functions that are obtained by mapping the density operator onto ccc-number functions. The equations of motion for the reduced phase-space distribution functions are found to be of the Fokker-Planck type. On transforming the Fokker-Planck equation to real variables, it is found to have the same form as the Fokker-Planck equation obtained by Wang and Uhlenbeck to describe the Brownian motion of a classical oscillator. The Fokker-Planck equation is solved for the conditional probability (Green's function) which is found to be in the form of a two-dimensional Gaussian distribution. This solution is then used to obtain various time-dependent quantum statistical properties of the oscillator. Next, the entropy for a quantum oscillator undergoing Brownian motion is calculated and we show that this system approaches equilibrium as t\ensuremath→\ensuremath∞t\ensuremath{\rightarrow}\ensuremath{\infty}t\ensuremath→\ensuremath∞. Finally we show that in the weak-coupling limit the Fokker-Planck equation reduces to the one obtained by making the usual rotating-wave approximation.
The theory of Brownian motion of a quantum oscillator is presented. The equation of motion for the density operator of the oscillator is obtained by a model Hamiltonian which characterizes the interaction between this oscillator and a reservoir. By applying iteration methods the equation of motion is solved and the time development of the density operator is obtained. The solution is then used to write the normally ordered generating functional for the field of the oscillator executing Brownian motion. This field appears to be the superposition of a thermal field in equilibrium with the reservoir, a chaotic field, and a field statistically similar to the one before the interaction. Next, it is shown that for large times the oscillator approaches equilibrium; moreover, it is shown that, if the reservoir is at zero temperature and initially the state of the oscillator is a coherent state, then it remains in a coherent state for later time. In order to obtain by differentiation two-time modal densities, a suitable two-time generating functional is introduced. This functional allows two-time averages to be computed from one-time averages before the interaction. Finally, some time-dependent statistical properties of the oscillator are studied.
Recent progress in our understanding of quantum effects on the Brownian motion in an external potential is reviewed. This problem is ubiquitous in physics and chemistry, particularly in the context of decay of metastable states, for example, the reversal of the magnetization of a single domain ferromagnetic particle, kinetics of a superconducting tunnelling junction, etc. Emphasis is laid on the establishment of master equations describing the diffusion process in phase space analogous to the classical Fokker-Planck equation. In particular, it is shown how Wigner's [E. P. Wigner, Phys. Rev., 1932, 40, 749] method of obtaining quantum corrections to the classical equilibrium Maxwell-Boltzmann distribution may be extended to the dissipative non-equilibrium dynamics governing the quantum Brownian motion in an external potential V(x), yielding a master equation for the Wigner distribution function W(x,p,t) in phase space (x,p). The explicit form of the master equation so obtained contains quantum correction terms up to o(h(4)) and in the classical limit, h --> 0, reduces to the classical Klein-Kramers equation. For a quantum oscillator, the method yields an evolution equation coinciding in all respects with that of Agarwal [G. S. Agarwal, Phys. Rev. A, 1971, 4, 739]. In the high dissipation limit, the master equation reduces to a semi-classical Smoluchowski equation describing non-inertial quantum diffusion in configuration space. The Wigner function formulation of quantum Brownian motion is further illustrated by finding quantum corrections to the Kramers escape rate, which, in appropriate limits, reduce to those yielded via quantum generalizations of reaction rate theory.
Chandrasekhar's phenomenological theory of brownian motion is transcribed to the quantum regime. The statistics used is that of Boltzmann but the free particle was treated, in addition, with Fermi-Dirac statistics followed by some discussion relating to the measurements of low temperatures. Difficulties arising from the dissipative processes involved are by-passed with the aid of a new methodology enabling one to obtain a propagator in configuration space, which embraces single-particle dissipative forces. This sort of propagator is in turn used for the construction of a type of a nonequilibrium density matrix for the quantum brownian particle. Exact nonequilibrium density matrices for the free and the harmonically bound brownian particles under the influence of external time dependent forces are obtained. Finally, a quantum Fokker-Planck type equation for the general brownian particle is derived. The analysis proceeds via functional integration.
It has long been recognized that the dynamics of linear quantum systems is classical in the Wigner representation. Yet many conceptually important linear problems are typically analyzed using such generally applicable techniques as influence functionals and Bogoliubov transformations. In this Letter we point out that the classical equations of motion provide a simpler and more intuitive formalism for linear quantum systems. We examine the important problem of Brownian motion in the independent oscillator model, and show that the quantum dynamics is described directly and completely by a c-number Langevin equation. We are also able to apply recent insights into quantum Brownian motion to show that the classical Fokker-Planck equation is always local in time, regardless of the spectral density of the environment.
The quantum theory of damping is presented and illustrated by means of a driven damped harmonic oscillator. The theory is formulated in the coherent state representation which illustrates very vividly the nearly classical nature of the problem. In this representation the reduced system density operator equation becomes a Fokker-Planck equation. Green's function solutions are found for the damped oscillator in closed form and as an eigenfunction expansion. In addition, a quantum regression theorem due to Lax is derived in the coherent state representation. The theorem allows two-time averages to be computed from one-time averages.