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Physical Review Letters

Specular Reflection of Very Slow Metastable Neon Atoms from a Solid Surface

Fujio Shimizu

Published Feb 5, 2001• 296 citations
Publisher

Abstract

An ultracold narrow atomic beam of metastable neon in the 1s3[(2s)(5)3p:1P0] state is used to study specular reflection of atoms from a solid surface at extremely slow incident velocity. The reflectivity on a silicon (1,0,0) surface and a BK7 glass surface is measured at the normal incident velocity between 1 mm/s and 3 cm/s. The reflectivity above 30% is observed at about 1 mm/s. The observed velocity dependence is explained semiquantitatively by the quantum reflection that is caused by the attractive Casimir-van der Waals potential of the atom-surface interaction.

DOI
10.1103/physrevlett.86.987

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An ultracold narrow atomic beam of metastable neon in the 1s3[(2s)(5)3p:1P0] state is used to study specular reflection of atoms from a solid surface at extremely slow incident velocity. The reflectivity on a silicon (1,0,0) surface and a BK7 glass surface is measured at the normal incident velocity between 1 mm/s and 3 cm/s. The reflectivity above 30% is observed at about 1 mm/s. The observed velocity dependence is explained semiquantitatively by the quantum reflection that is caused by the attractive Casimir-van der Waals potential of the atom-surface interaction.
We observed quantum reflection of ultracold atoms from the attractive potential of a solid surface. Extremely dilute Bose-Einstein condensates of 23Na, with peak density 10(11)-10(12) atoms/cm(3), confined in a weak gravitomagnetic trap were normally incident on a silicon surface. Reflection probabilities of up to 20% were observed for incident velocities of 1-8 mm/s. The velocity dependence agrees qualitatively with the prediction for quantum reflection from the attractive Casimir-Polder potential. Atoms confined in a harmonic trap divided in half by a solid surface exhibited extended lifetime due to quantum reflection from the surface, implying a reflection probability above 50%.
The specular reflectivity of slow, metastable neon atoms from a silicon surface was found to increase markedly when the flat surface was replaced by a grating structure with parallel narrow ridges. For a surface with ridges that have a sufficiently narrow top, the reflectivity was found to increase more than two orders of magnitude at the incident angle of 10 mRad from the surface. The slope of the reflectivity vs the incident angle near zero was found to be nearly an order of magnitude smaller than that of a flat surface. A grating with 6.5% efficiency for the first-order diffraction was fabricated by using the ridged surface structure.
A cold beam of He∗(23S1){\mathrm{He}}^{*}\phantom{\rule{0.3em}{0ex}}(2\phantom{\rule{0.2em}{0ex}}^{3}S_{1})He∗(23S1​) atoms is used at grazing incidence to study the quantum reflection on a flat polished silicon surface. We measure the reflectivity as a function of the normal incident velocity component between 3 and 30cm∕s30\phantom{\rule{0.3em}{0ex}}\mathrm{cm}∕\mathrm{s}30cm∕s. Our result is in reasonable agreement with a calculation of the attractive van der Waals surface potential using the dielectric function of Si and the dipole polarizability of He∗{\mathrm{He}}^{*}He∗. We discuss the influence of the conductivity and of a thin oxide layer on the potential. By comparing our data to those previously measured with Ne∗{\mathrm{Ne}}^{*}Ne∗ atoms, we are also able to confirm the scaling of the reflectivity with atomic mass.
Recent developments in atom optics have brought Bose-Einstein condensates within 1 μm of solid surfaces where the atom-surface interactions can no longer be ignored. At longrange, the atom-surface interaction is described by the weakly attractive Casimir-Polder potential which is classically predicted to accelerate an incident atom toward the surface where it will interact strongly with the internal modes of the surface, lose energy, and land in a bound state of the surface. When the incident atom is very cold, on the order of a few nanokelvin, however, the acceleration of the atomic wavefunction is so abrupt that the atom may partially reflect from the attractive tail in a process known as quantum reflection. This work presents experimental evidence for quantum reflection from a solid surface at normal incidence. Using atoms from a 23Na BEC, cooled to a few nanokelvin in a recently demonstrated single-coil trap, controlled collisions were induced between atoms and solid silicon surface. A maximum reflection probability of ∼ 12% was observed for an incident velocity of 1 mm/s. Atoms confined against the surface at low density exhibited an enhanced lifetime due to quantum reflection. A surprising aspect of quantum reflection is that nano-structured surfaces are predicted to exhibit enhanced quantum reflection due to the reduction of the atom-surface interaction from reduced density surfaces. Using a pillared surface with an density reduced to 1% of bulk density, we observe an enhancement of the reflection probability to ∼ 60%. At velocities from 2-25 mm/s, predicted threshold dependence of the reflection probability was observed. At velocities below 2 mm/s, the reflection probability was observed to saturate. We develop a simple model which predicts the saturation as a result of mean-field interactions between atoms in the incident Bose-Einstein condensate. Thesis Supervisor: Wolfgang Ketterle Title: John D. MacAurthur Professor of Physics Thesis Supervisor: David E. Pritchard Title: Cecil and Ida Green Professor of Physics For the parents in my life,
The coherent reflection of ultra-cold neon and helium atoms from silicon surfaces and surface structures is measured and analyzed. When the silicon surface is flat, the reflection is explained by the quantum reflection due to van der Waals attractive potential near the silicon surface. When the silicon surface is modified to form a grating structure, the reflectivity increases dramatically. For certain ranges of surface structure parameters, the reflection may be interpreted as a coherent summation of Fresnel diffraction of the atomic wave at the ridges of the grating structure.