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Optics Communications

Absorption coefficient of luminescent bodies in the emission band

A. Aleksić, K. Nikolić, J. Burić, D. Magnant, H. Payen de la Garanderie

Published Feb 1, 1982• 0 citations
Publisher
DOI
10.1016/0030-4018(82)90361-3

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Journal of the Physical Society of Japan•Feb 1, 1984•17 citations
We propose a multiple beam illumination scheme to control the intensity of the light emitted by a thin luminescent layer. The experiment is designed to get as close as possible to the condition of Coherent Perfect Absorption (CPA) at a wavelength at which the absorption coefficient of the luminescent layer is low, and it is realized by externally acting on the phase difference between the incident beams. We elucidate experimental limitations that prevent the achievement of CPA in these slabs. Nevertheless, we are able to demonstrate that when the two beams destructively interfere outside the luminescent layer, the incident light is more efficiently absorbed by the luminescent layer and the intensity of the emitted light is phase-modulated.
Nonradiative relaxation and photoluminescence quenching in nanocrystalline powders doped with rare-earth elements are of interest in optical bistability, random laser, and other optoelectronic applications. Here, the luminescence quenching of a one-dimensional random medium made of multilayer nanoparticles (Y2O3) doped with rare-earth elements (Yb3+) is analyzed by considering the transport, transition, and interaction of the fundamental energy carriers. The nonradiative decay and luminescence quenching in random media are enhanced compared to single crystals, due to multiple scattering, enhanced absorption, and low thermal conductivity. The coherent wave treatment is used to calculate the photon absorption, allowing for field enhancement and photon localization. The luminescent and thermal emission is considered as incoherent. The size-dependent absorption coefficient and penetration depth are observed. The nonradiative decay is identified as a multiphonon relaxation process, and is found to be enhanced compared to bulk materials. The luminescence quenching and nonlinear thermal emission, occurring with increasing irradiation intensity, are predicted.
Under the off-resonant excitation at the slightly higher energy side of the giant two-photon absorption band (GTA) for the direct generation of excitonic molecules (EM) in CuCl, new narrow emission bands designated as X T and X L have been found in the energy region of the M T and M L broad bands, respectively. Their photon energies increase with the decrease of the pump photon energy from the higher-energy side of the resonance and finally, at the on-resonant excitation, their bands merge into M T 0 and M L 0 bands, respectively, previously reported by Mita et al. Based on the detailed studies on these bands, it is found that there exists a certain kind of transverse relaxation process which acts on the EM just after their generation by the GTA and brings about the X emission as a hot luminescence.