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Journal of Quantitative Spectroscopy and Radiative Transfer

Laser-linewidth effects on the interference spectra of a two-level atom

Constantine Mavroyannis

Published Oct 1, 1995• 0 citations
Publisher
DOI
10.1016/0022-4073(95)00100-y

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The effect of the laser linewidth on the resonance fluorescence spectrum of a two-level atom is revisited. The novel spectral features, such as hole-burning and dispersive profiles at line centre of the fluorescence spectrum are predicted when the laser linewidth is much greater than its intensity. The unique features result from quantum interference between different dressed-state transition channels. c # 1999 Elsevier Science B.V. PACS : 42.50.Hz; 32.80.-t Keywords: Resonance fluorescence; Laser linewidth; Quantum interference The study of resonance fluorescence spectra has provided much fundamental insight into the subject of atom1light interactions. It is well known that for weak laser field excitation, the spectrum exhibits a Lorentzian lineshape, whereas it develops into the Mollow triplet for strong field excitation [1]. The latter is a direct signature of stimulated emissions and absorptions of the atom during the time interval for one spontaneous decay. Recently, considera...
We have considered the interference spectra arising from the competition between a spontaneous process and one induced by a laser field in a two-level atom. Expressions for the spectral functions have been derived describing the spectra of the excited and ground states of the atom in the low- and high-intensity limit of the laser field. For the excited-state spectra in the low-intensity limit, the frequency profiles of the two peaks, which arise from the spontaneous and the induced processes, cancel each other out completely near the center of the line, while for the ground state the induced process dominates. For finite values of the detuning, the spectra of the excited state consist of two peaks, which have positive and negative frequency profiles, respectively. The computed spectra have been graphically presented and discussed. In the high-intensity limit, the dynamic Stark effect dominates the spectra of the excited and ground states of the atom. Expressions for the correlation functions have been derived that describe the emission or the absorption of a laser photon at two different times. The derived expressions for the corresponding delay functions in the low- and high-intensity limits have been found to be identical to those recently proposed in the literature. The laser field has been treated as a classical as well as a quantized entity.
The resonance fluorescence spectra of a laser-driven four-level closed-loop diamond-shape atomic system are investigated in this paper. The four decay channels in the system interfere with each other in different ways according to several distinct arrangements of the two intermediate atomic levels, and hence produce the spontaneously generated coherence (SGC) effects. The numerical calculation shows that the amplitude, the linewidth and the number of sidebands of the resonance fluorescence spectrum are deeply modified by the SGC effects; accordingly, interesting effects such as the spectral-line narrowing, spectral-line suppression, spectral-line enhancement and even the complete quenching of fluorescence are generated under certain conditions. Moreover, we propose a new kind of level structure, the seesaw structure, in which the SGC effect can also be attained without the rigorous conditions of degenerate levels. In the end, we discuss the possibility of demonstrating our scheme in real atomic systems and summarize our results.