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American Journal of Physics

Some basic properties of stimulated and spontaneous emission: A semiclassical approach

Alan V. Durrant

Published Jul 1, 1976• 14 citations
Publisher

Abstract

The coherence and directional properties of stimulated and spontaneous emission can be understood without a knowledge of quantum electrodynamics. This paper presents a semiclassical description of the interaction between a free atom and a weak optical field under conditions of either a stimulated emission or a stimulated absorption resonance. It is shown that, under certain conditions, the stimulated or spontaneous radiation fields emitted from a sample of atoms will propagate in the same direction as the incident beam, will be coherent with the incident beam, and will have the correct phase to provide amplification or attenuation.

DOI
10.1119/1.10322

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Soviet Journal of Quantum Electronics•Apr 30, 1981•1 citation
The coherence and directional properties of stimulated and spontaneous emission can be understood without a knowledge of quantum electrodynamics. This paper presents a semiclassical description of the interaction between a free atom and a weak optical field under conditions of either a stimulated emission or a stimulated absorption resonance. It is shown that, under certain conditions, the stimulated or spontaneous radiation fields emitted from a sample of atoms will propagate in the same direction as the incident beam, will be coherent with the incident beam, and will have the correct phase to provide amplification or attenuation.
A semiclassical radiation theory is developed in which the spontaneous emission field of a two-level atom is a quantum entity represented by atomic operators acting in the Hilbert space of the atomic states. The theory is applied to an investigation of the coherence properties of spontaneous emission. It is found that incoherent and coherent components can be identified in the emission field, the former dominating in the early stages of the decay from the excited state and the latter dominating in the later stages or in the emission from a weakly excited atom. The single-atom coherence properties are shown to lead to well-known superradiance phenomena in the spontaneous emission from an assembly of similar atoms. The paper does not use the theory of quantum electrodynamics; it builds on knowledge at the undergraduate level of classical radiation theory and the quantum mechanics of atoms.
This chapter discusses the details of what stimulated emission of radiation is, why it is the major physical phenomenon at the heart of the laser, and how it is exploited in ways to create laser light beams. It describes the Bohr model of the atom and how electrons can only make quantized leaps in energy levels from one atomic orbital or shell to the next. The chapter considers Pauli’s Exclusion Principle and singlet, doublet, and triplet states of the atom. It also describes the interaction of light with atoms through absorption, spontaneous emission, and stimulated emission. The chapter shows that the quantum mechanical harmonic oscillator and the ground state of the universe is a nonzero electromagnetic field and therefore is the trigger for spontaneous emission. It looks at the models for absorption, spontaneous and stimulated emission, and vibrational states.
Abstract In his celebrated 1916–17 papers in which he proposed the A and B coefficients for the spontaneous and stimulated emission of energy quanta from excited atoms, Einstein conjectured that stimulated emission involves the release of individual quanta (later dubbed “photons”) along the direction of an incident photon with the same energy, momentum, phase, and polarization state as that of the incident photon. According to classical electrodynamics, of course, an oscillating dipole must radiate an azimuthally symmetric electromagnetic field around its axis of oscillation. Nevertheless, Einstein suggested that the release of stored energy from excited atoms in the form of discrete quanta (photons) must be directional, and that, in the case of stimulated emission, the direction of the emitted photon must coincide with that of the incident photon. The goal of the present paper is to show that some of the prominent features of absorption and stimulated emission emerge from Maxwellian electrodynamics in conjunction with the simple mass-and-spring model of an atom known as the Lorentz oscillator model.
The problem of induced and spontaneous emission is investigated for an atomic two-level system with incident beams of radiation which are either in a coherent state or in a stationary state (contain a definite number of photons). The treatment is fully quantum-mechanical, and is confined to the case where the frequency spectrum of the incident beam is narrow compared to the natural linewidth of the system. It is shown that, under such conditions, the spontaneous emission for frequencies within the narrow band of the incident radiation is sharply reduced compared to the prediction of the natural lineshape. It is shown that a hole is burned in the natural lineshape within the narrow frequency band, thus effectively quenching the spontaneous emission at some frequency within the band. This effect is shown to occur both for the coherent and stationary beams. Quantities proportional to the induced and spontaneous probability amplitudes and the lifetimes are computed for times comparable to and long compared to the free lifetime of the state. An expression is found for the spectrum of the emergent radiation in terms of these quantities. Its physical meaning is briefly discussed. The density operator of the field for all times is given.
Spontaneous emission competes with stimulated emission in many interactions of light with matter. In the usual analyses which describe the interaction of an atom with a coherent optical field, the spontaneous emission characteristics, e.g., probability and spectral distribution, are not determined. The spontaneous emission from an atom which interacts with a coherent light wave is considered. The competition between coherent photons and spontaneous photons is treated in detail for a system consisting of a stationary atom, an open cavity and spatial fields. In the model chosen, a multilevel atom which spontaneously decays by interacting with spatial fields has two nondegenerate states coupled by an interaction with a single mode of the cavity. The Laplace-transformed Schrodinger equation is solved for specified initial conditions of the system. It is found that the interaction with the coherent field modifies the spectral distribution of spontaneous radiation from the atom. For spontaneous transitions involving an atomic state which interacts with the coherent field, the spectral distributions can no longer be described by Lorentzian functions. The new distributions exhibit a broadening and splitting for strong interactions between the atom and the coherent field. It is shown that the qualitative features of these distributions can be predicted from the energy-level diagram of the atom-cavity system. The net probability of the system gaining a coherent or cavity photon is calculated by integrating over the emitted spontaneous frequencies. The equivalence of this approach to the method of computing probabilities by integrating over time is demonstrated by using Parseval's theorem.
Spontaneous and stimulated emission from atoms in a free one-dimensional space is considered from the quantum-mechanical point of view. The resolvent method is used to calculate the field density matrix, average electric field, and electromagnetic field energy density for a spontaneously emitting atom. For an atom emitting in the field of another atom, calculations are made of the electric field of the spontaneous and stimulated radiation. It is shown how the coherence length and coherence time of the spontaneous radiation increase. The application of these results in laser theory to explain the formation of a radiation mode structure and consequent appearance of coherent radiation is discussed.