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Journal of Applied Physics

Deterministic and stochastic spin diffusion in classical Heisenberg magnets

Jianmin Liu, Niraj Srivastava, V. S. Viswanath, Gerhard H. Muller

Published Nov 15, 1991• 11 citations
Publisher

Abstract

This computer simulation study provides further evidence that spin diffusion in the one-dimensional classical Heisenberg model at T=∞ is anomalous: 〈Sj(t)⋅Sj〉 ∼t−α1 withα1 ≳1/2. However, the exponential instability of the numerically integrated phase-space trajectories transforms the deterministic transport of spin fluctuations into a computationally generated stochastic process in which the global conservation laws are still satisfied to high precision. This may cause a crossover in 〈Sj(t)⋅Sj〉 from anomalous spin diffusion (α1 ≳ 1/2) to normal spin diffusion (α1 = 1/2) at some characteristic time lag that depends on the precision of the numerical integration.

DOI
10.1063/1.350037

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This computer simulation study provides further evidence that spin diffusion in the one-dimensional classical Heisenberg model at T=∞ is anomalous: 〈Sj(t)⋅Sj〉 ∼t−α1 withα1 ≳1/2. However, the exponential instability of the numerically integrated phase-space trajectories transforms the deterministic transport of spin fluctuations into a computationally generated stochastic process in which the global conservation laws are still satisfied to high precision. This may cause a crossover in 〈Sj(t)⋅Sj〉 from anomalous spin diffusion (α1 ≳ 1/2) to normal spin diffusion (α1 = 1/2) at some characteristic time lag that depends on the precision of the numerical integration.
The problem of spin diffusion is studied numerically in the one-dimensional classical Heisenberg model using a deterministic odd-even spin precession dynamics. We demonstrate that spin diffusion in this model is normal in the infinite-temperature limit and one obtains a long-time diffusive tail in the decay of the autocorrelation function. Some variations of the model with different coupling schemes and anisotropy are also studied and we find normal diffusion in all of them. A systematic finite-size analysis also suggests normal diffusive spreading of spin fluctuations, contrary to previous claims of anomalous diffusion. We also briefly discuss spin diffusion in this model at finite temperatures.
We report a systematic study of finite-temperature spin transport in quantum and classical one-dimensional magnets with isotropic spin interactions, including both integrable and nonintegrable models. Employing a phenomenological framework based on a generalized Burgers' equation in a time-dependent stochastic environment, we identify four different universality classes of spin fluctuations. These comprise, aside from normal spin diffusion, three types of superdiffusive transport: the Kardar-Parisi-Zhang universality class and two distinct types of anomalous diffusion with multiplicative logarithmic corrections. Our predictions are supported by extensive numerical simulations on various examples of quantum and classical chains. Contrary to common belief, we demonstrate that even nonintegrable spin chains can display a diverging spin diffusion constant at finite temperatures.
The anomalous spin diffusion of the integrable easy-axis Heisenberg chain originates in the ballistic transport of symmetry sectors with nonzero magnetization. Ballistic transport is replaced by normal dissipative transport in all magnetization sectors upon introducing the integrability-breaking perturbations, including external driving. Such behavior implies that the diffusion constant obtained for the integrable model is relevant for the spread of spin excitations but not for the spin conductivity. We present numerical results for closed systems and driven open systems, indicating that the diffusion constant shows a discontinuous variation as the function of perturbation strength.
We have studied the dynamics of the classical Heisenberg chain at finite and infinite temperatures by computer simulation of an array of 4000 spins. The evaluation of the spin-spin and energy-energy wave-vector- and time-dependent correlation functions out to time $10{J}^{\ensuremath{-}1}$ made it possible to determine the spin and energy diffusion constants. At infinite temperature we find ${D}_{S}=(1.33\ifmmode\pm\else\textpm\fi{}0.10)JS{a}^{2}$ and ${D}_{E}=(3\ifmmode\pm\else\textpm\fi{}1)JS{a}^{2}$. Values of DS{D}_{S}DS​ have also been determined, with less precision, for ferromagnetic and antiferromagnetic interactions at temperatures kBT∣J∣=1.0and0.5\frac{{k}_{B}T}{|J|}=1.0 \mathrm{and} 0.5∣J∣kB​T​=1.0and0.5. Our results are compared with various theoretical estimates. In addition, we calculate the time-dependent spin and energy self-correlation functions.
The search for departures from standard hydrodynamics in many-body systems has yielded a number of promising leads, especially in low dimensions. Here, we study one of the simplest classical interacting lattice models, the nearest-neighbor Heisenberg chain, with temperature as the tuning parameter. Our numerics expose strikingly different spin dynamics between the antiferromagnet, where it is largely diffusive, and the ferromagnet, where we observe strong evidence either of spin superdiffusion or an extremely slow crossover to diffusion. This difference also governs the equilibration after a quench, and, remarkably, is apparent even at very high temperatures.
We analytically and numerically study spin transport in a one-dimensional Heisenberg model in linear-response regime at infinite temperature. It is shown that as the anisotropy parameter Δ is varied spin transport changes from ballistic for Δ<1 to anomalous at the isotropic point Δ=1, to diffusive for finite Δ>1, ending up as a perfect isolator in the Ising limit of infinite Δ. Using perturbation theory for large Δ a quantitative prediction is made for the dependence of diffusion constant on Δ.