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Bulletin of the Russian Academy of Sciences Physics

An atom-photon cluster localized in a microcavity

Ashat M. Basharov

Published Feb 1, 2011• 3 citations
Publisher

Abstract

It is shown that our description of the dynamics of interaction between atoms with microcavity mode quanta and an external electromagnetic field under conditions of two-photon resonance follows from a simple theory of one-photon resonance interaction between two-level atoms and the same external electromagnetic field, if we substitute su (2) algebra elements of the one-photon resonance theory for third-order elements of polynomial algebra. Commutation relations of polynomial algebra determine the features of processes with the participation of a single object, i.e. an atom-photon cluster localized in a microcavity. Its states are the basis for irreducible representations of this polynomial algebra.

DOI
10.3103/s1062873811020067

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It is shown that our description of the dynamics of interaction between atoms with microcavity mode quanta and an external electromagnetic field under conditions of two-photon resonance follows from a simple theory of one-photon resonance interaction between two-level atoms and the same external electromagnetic field, if we substitute su (2) algebra elements of the one-photon resonance theory for third-order elements of polynomial algebra. Commutation relations of polynomial algebra determine the features of processes with the participation of a single object, i.e. an atom-photon cluster localized in a microcavity. Its states are the basis for irreducible representations of this polynomial algebra.
The interaction of an atomic ensemble localized in a microcavity with external electromagnetic fields under Raman resonance conditions with an optically forbidden atomic transition involving photons of the microcavity mode has been described in terms of third-order polynomial algebra. It has been shown that atoms and photons localized in the microcavity under these conditions form a united object, an atom-photon cluster, on the states of which the irreducible representations of polynomial algebra are implemented. Classical coherent and quantum broadband electromagnetic fields are considered as external fields. The effective Hamiltonian, effective dipole moment operator, and relaxation operator of the atom-photon cluster are expressed in terms of the generators of polynomial algebra, which is the algebra of the dynamical symmetry of the problem. The developed mathematical technique has been applied to describe the main radiative processes—spontaneous emission and nutation effect—on atom-photon clusters. All of these effects are peculiar and differ from similar phenomena on two-level atoms, but only simple cases of the mentioned radiative processes have been considered.
Abstract Models of radiative quantum systems were constructed as analogs of multiphoton and Raman resonances of classical field quanta on an atomic system with the participation of cavity mode quanta. A distinctive feature of the models is the description of an atomic ensemble and quanta using either the generators of polynomial algebra or the two-mode Jordan–Schwinger representation of the su(2) algebra, so that one can talk about an atom–photon and/or photon clusters. The arising algebras are mathematically unsolvable, in contrast to the Heisenberg–Weyl algebra. This makes it possible to implement and observe fundamental effects of coherent nonlinear optics, such as photon echo, optical nutation, and superradiance, in ensembles of the described clusters.
We described the constructed models of radiative quantum systems analogous of multiphoton and Raman resonances of classical field quanta on an atomic system with the participation of resonator mode quanta. A distinctive feature of the models is the possibility to describe an atomic ensemble and quanta using either the generators of polynomial algebra or the two-mode Jordan-Schwinger representation of the su(2) algebra, that could point to atomic-photon and/or photon clusters. The algebras are arising that are mathematically insoluble, in contrast to the Heisenberg — Weyl algebra, which makes it possible to implement and observe fundamental effects of coherent nonlinear optics, such as photon echo, optical nutation, and superradiance in ensembles of the described clusters.
The spontaneous emission from an atomic ensemble localized in a microcavity with the participation of microcavity photons and an external broadband quantized electromagnetic field at the Raman resonance of photons with an optically forbidden (two-photon) atomic transition has been studied. The average spontaneous decay intensity has been calculated for simple cases. It is shown that the dynamics of spontaneous emission from this atomic ensemble differs generally from the conventional superradiance (spontaneous emission of an atomic ensemble at a one-photon optically allowed transition from excited to the ground state. When the atomic ensemble is strongly excited, the delay times and the emission pulse shape differ significantly. The parameter ranges where the spontaneous emission from the atomic ensemble under consideration at a two-photon Raman transition can be described as conventional superradiance with renormalized parameters are found. In the case of single excitation the photon emission probability depends on the number of photons and atoms in the microcavity.
The strong resonance interaction of a two-level atom with the continuum of quantized electromagnetic modes falling within the contour of a resonance mode of a dielectric microsphere is considered within the framework of quantum electrodynamics. Analytical solutions are derived. As an initial condition, we consider the case when, at time t = 0, the atom is excited and the resonance modes of the microsphere contain a single-photon wavepacket. It is shown that the properties of the emitted photon pair depend crucially on space-time properties of the photon wavepacket contained in the resonator. When the mean square of the electric field of the photon wavepacket at the initial instant of time at the atom position is close to the vacuum value, the radiation of an atom is similar to a spontaneous one and the emitted photon pair has no correlations. On the contrary, if the mean square of the electric field of the photon wavepacket at the initial instant of time at the atom position is substantially greater than the vacuum value, the radiation of an atom has a stimulated nature and the emitted photon pair has very complicated strong correlations. The relationship between the results obtained and the predictions of the dressed states theory are briefly discussed. The results obtained are of a general character and can be applied to the description of the resonant interaction of an excited atom and an excited resonator of an arbitrary shape.
A chain of N identical two-level atoms coupled with the electromagnetic field, prepared via a single-photon Fock state, is investigated. It is found that, if the interaction between atoms is negligible, than the obtained dynamic equations for the probability amplitudes allow, in a certain sense, an interpretation of the dynamics of states in the classical fashion in terms of a superposition of oscillatory modes of the system under study. The derived equations reveal how a space configuration of the system of atoms affects the dynamics of the atomic states, particularly the “decay” rates of separate atoms and the system as the whole.