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Journal of Physics D Applied Physics

Interrupted fluorescence, quantum jumps and wavefunction collapse. II

David Thomas Pegg, P. L. Knight

Published Oct 14, 1988• 8 citations
Publisher

Abstract

For pt.I see Phys. Rev. A, vol.37, p.4303 (1988). The principle of wavefunction collapse by non-detection of photons leads to simple but rigorous expressions for the average dark and bright periods, T D and T B , of intermittent quantum jump fluorescence from a V-configuration three-level atom. Here further consequences of this principle are explored, including: the derivation of some new correlation functions which exhibit the physical characteristics of extended dark and bright periods; the expressions for T D and T B when one transition is driven coherently and the other incoherently; and a general expression for the characteristic time to be sure that a quantum jump has occurred for any type of driving field.

DOI
10.1088/0022-3727/21/10s/036

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For pt.I see Phys. Rev. A, vol.37, p.4303 (1988). The principle of wavefunction collapse by non-detection of photons leads to simple but rigorous expressions for the average dark and bright periods, T D and T B , of intermittent quantum jump fluorescence from a V-configuration three-level atom. Here further consequences of this principle are explored, including: the derivation of some new correlation functions which exhibit the physical characteristics of extended dark and bright periods; the expressions for T D and T B when one transition is driven coherently and the other incoherently; and a general expression for the characteristic time to be sure that a quantum jump has occurred for any type of driving field.
The phenomenon of antibunching provides important support for the physical principle of the collapse of the wave function following a detection of a photon. In this paper we show that interrupted fluorescence in a three-level, V-configuration atom, with one transition strongly driven and one weakly driven, can be regarded as evidence supporting the complementary principle of ``collapse by nondetection.'' Use of this principle leads to the immediate deduction of remarkably simple general expressions for the average bright and dark periods, which allows these quantities to be calculated for both coherent and incoherent excitation without the need to solve the density-matrix equations, or even to find their long-term steady-state solutions. Thus the concept of collapse by nondetection appears to be not only valid but is also useful for predicting physically observable phenomena.
In an externally driven multilevel quantum system observation that the NEXT jump has not yet happened affects its future development. In previous work [Phys. Rev. A36, 929 (1987)] it was shown that this class of measurement makes it possible to observe remarkably long dark intervals -- or intermittency -- in the atomic fluorescence of an atom with 3 or more levels. Those calculations were carried out when the driven oscillations or Rabi flopping between the ground state and a strongly fluorescing state were fast compared to its lifetime. In systems with solid state Qubits the accessible parameter space is generally limited to the regime where oscillations are slower than the lifetime. In this paper we evaluate intermittency in atomic transitions, due to measurements with a null result, in this limit. During the dark periods the wave function of the continuously measured multilevel system is coherent.
We apply a general formalism for the separation of rapid and slow time scales in linear evolution equations to three-state atoms with a strong and a weak radiative transition. This leads to an expression for the intensity correlation function that constitutes a good approximation on both time scales. This result can also be translated into an expression for the waiting-time distribution for the next photon emission after a previous one. The slow evolution is expressed in two rate constants, which determine the statistical distribution for dark and bright periods in the fluorescent emission. The result is applied to various configurations of the radiative couplings between the three states.
A theory of the discrete photodetection of quantum jumps on the V configuration of atomic levels has been developed. A three-level source atom is placed in a cavity excited by a resonance fluorescence field. The cavity is tuned to exact resonance with an atomic transition. The cavity mode state is tested by a flux of unexcited (at the entrance) probe atoms passing through the cavity. The energy states of the outgoing probe atoms are detected by ionization chambers, which are assumed ideal. This a posteriori statistical information is indirectly related to the numerical characteristics of a measured quantum system consisting of the source atom and cavity mode. The “tuning” conditions for a discrete photodetector, i.e., the rules for choosing the parameters and durations of the interactions of the cavity mode with the probe and source atoms, intensities of the pump and probe fields that are necessary for observing quantum jumps from the “bright” state to the “dark” one and vice versa, have been determined. A two-state model that describes the dynamics of a quantum jump has been analyzed. The formulas have been obtained for the observable characteristics of quantum jumps: the mean residence time of the quantum system in quasistationary states (durations of the bright and dark periods), probabilities of quantum jumps, mean excitation levels of the quantized cavity mode, etc.
Time correlations in the fluorescence of a multilevel atom are studied in terms of the quantum statistics which describe the emission of the next photon. The next photon equations are substantially simpler than the a photon equations (or so-called optical Bloch equations) yet they contain phase information lost in the averaging procedure that yields the a photon equations. Employing the next photon equations we present a quantum formalism in which the time development of the wave function of the atom is dramatically modified by the observation of a dark period. This ``collapse'' of the quantum state due to measurements with a null result (such as the failure to record events in a photodetector) is the cause of intermittent atomic fluorescence even when the exciting field is arbitrarily coherent. The next photon and a photon formalisms are contrasted and applied to photon antibunching. The phenomenon of photon bunching which characterizes sideband correlations is also calculated. Observable effects particular to the coherent intermittency are emphasized.
Correlations between the emission of photons from an excited three-level atom with one transition more strongly driven than the other are studied. Antibunching, anticorrelation, and superbunching are exhibited in the four possible configurations: ``vee'' (V), ``lambda'' (\ensuremath{\Lambda}), and two cascades with the upper or lower transition strongly driven. We pay particular attention to the projection of the atom into particular states by the measurement of fluorescence, and its significance for detecting quantum jumps in the weak transition by observing the fluorescence from the strong transition. For incoherent excitation we find that cross antibunching (the anticorrelation between emissions of different types of photons) manifests itself as prolonged periods of darkness. For the V and the cascade configuration with a strongly driven lower transition, these periods herald the emission of a weak-transition photon; for the other cascade and the \ensuremath{\Lambda} configuration the periods are heralded by the emission of a weak-transition photon. For on-resonance coherent excitation, dark periods are extremely infrequent for the former two configurations, and are extremely long or infinite for the latter two.