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International Journal of Quantum Chemistry

Nonlinear resonant magneto‐optical effects in alkaline metal vapors in the strong bichromatic laser radiation field

T. Ya. Karagodova, Anna V. Kuptsova

Published May 10, 2004• 2 citations
Publisher

Abstract

Abstract Results of computer simulations of the spectra of magneto‐optical rotation (MOR) of the polarization plane for both components of intense bichromatic laser radiation are presented. Dependences of MOR on light intensity and the external magnetic field strength have been investigated. The simulations are based on the theory and method published earlier. Our results coincide with experimental results known from literature. This suggests that new peculiarities of MOR in alkaline vapors obtained by computer simulations can be observed in the natural experiments. © 2004 Wiley Periodicals, Inc. Int J Quantum Chem, 2004

DOI
10.1002/qua.20046

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Abstract Results of computer simulations of the spectra of magneto‐optical rotation (MOR) of the polarization plane for both components of intense bichromatic laser radiation are presented. Dependences of MOR on light intensity and the external magnetic field strength have been investigated. The simulations are based on the theory and method published earlier. Our results coincide with experimental results known from literature. This suggests that new peculiarities of MOR in alkaline vapors obtained by computer simulations can be observed in the natural experiments. © 2004 Wiley Periodicals, Inc. Int J Quantum Chem, 2004
In the paper there are presented the last results of computer simulations on the spectra of magneto-optical rotation (MOR) of plane of polarization for the both components of intense bichromatic laser radiation. Also the dependences of MOR on light intensity and magnetic field strength are investigated. The calculations are based on the theory and method, published earlier. The agreement of calculations for the cases investigated in the known experiments with experimental results permits to hope that new peculiarities of the MOR in alkaline vapors considered in our paper can be observed in the natural experiments.
The method of computer simulations on nonlinear resonant magneto-optical effects developed for real multi-level atoms in the two laser fields of arbitrary intensity and external magnetic field is applied for the polarization effects of different types calculations and investigations of the dependence of the characteristics of these effects on magnetic field strength, intensities, polarizations and detunings of laser fields for alkaline atoms. The essence of the method consists in simulations and analysis of the plots of dependence of quasienergies on parameters (detunings and intensities of radiation fields, magnetic field strength), which are obtained with the help of sorting subprogram, and selection of suitable algorithms for calculations of characteristics of nonlinear resonant magneto-optical effects. One-photon and two photon resonant effects are investigated for wide range of magnetic field strength from Zeeman to Paschen Back effects. Some new features in the spectra of rotation of plane of polarization and circular dicohroizm of different types are predicted. The results show the agreement with known experiments. Such calculations of nonlinear resonant magneto-optical effects in the intense laser fields resonant to adjacent transitions and magnetic field show the opportunity of investigation the modifications of electronic structure due to intense radiation fields and strong external magnetic field in atomic gases and also may be used for the treatment of new methods of phase-polarization selection of modes of tunable lasers.
The method of computer simulations on nonlinear resonant magnetooptical effects developed for real multi-level atoms in the two laser fields of arbitrary intensity and external magnetic field is applied for the polarization effects of different types calculations and investigations of the dependence of the characteristics of these effects on magnetic field strength, intensities, polarization and detunings of laser fields for alkaline atoms. The essence of the method consists in simulations and analysis of the plots of dependence of quasi energies on parameters, which are obtained with the help of sorting subprogram, and selection of suitable algorithms for calculations of characteristics of nonlinear resonant magnetooptical effects. One photon and two photon resonant effects are investigated for wide range of magnetic field strength from Zeeman to Paschen Back effects. Some new features in the spectra of rotation of plane of polarization and circular dichroism of different types are predicted. The results show the agreement with known experiments. Such calculations of nonlinear resonant magnetooptical effects in the intense laser fields resonant to adjacent transitions and magnetic field show the opportunity of investigation the modifications of electronic structure due to intense radiation fields and strong external magnetic field in atomic gases and also may be used for the treatment of new methods of phase-polarization selection of modes of tunable lasers.
Results of a numerical study of the Faraday effect arising upon propagation of the light beams with the frequencies ω L1 (resonant to the nS 1/2-nP 1/2, 3/2 transitions) and ω L2 (resonant to the nP 1/2, 3/2-(n+2)S 1/2 transitions) through alkali-metal vapors are presented. Characteristics of the magneto-optical rotation spectra at each of the frequencies are strongly affected by the second intense radiation field resonant to the adjacent transition. When the atoms interact with two strong light waves, resonant to adjacent transitions, and with a magnetic field, the shape of the Faraday rotation spectra depends on the energy shifts of the atomic states that arise due to the dynamic Stark effect and the Zeeman effect (the Paschen-Back or an intermediate-type effect), as well as due to the difference of populations of these states caused by the interaction of the atoms with the fields. The results obtained show that in the frequency selection method, based on the resonance Faraday effect, the frequency of the generated narrow-band beam can be tuned by the intensity of the strong wave, resonant to the transition between the excited states.
The numerical analyses of polarization phenomena is developed for the radiation fields resonant with the transitions nS1/2-nP1/2,3/2 and nP1/2,3/2 -- (n+2)S1/2 of alkaline atoms. The method of computer simulation of nonlinear resonant polarization phenomena is used, which is based on the solution of the problem of interaction of the real multilevel atom with two laser fields of arbitrary intensity and polarization and with a constant magnetic field. This method is known to be successful applied for the investigation of the polarization phenomena in the atomic gases of the alkaline atoms Na and K. In present paper the whole alkaline group is considered. The represented spectra of rotation of plane of polarization are appear to be qualitatively different for different atoms since atom fine- structure intervals differ very much from each other. The obtained spectra for Rb are in good agreement with the experimental spectra.