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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Dynamics of transient four-wave mixing of laser pulses in a resonant medium

V. V. Kabanov, Alexander S. Rubanov

Published Apr 11, 1996• 0 citations
Publisher

Abstract

The characteristic features of the conjugate wave's formation under transient four-wave mixing in a two-level medium are investigated. The phase modulations of the signal and conjugate waves induced in the four-wave mixing are not mutually conjugate and have the same sign. The fulfillment of the phase-conjugation for the phase modulated signal has been shown in particular to be connected with the envelope's deformation and the spectrum's change of signal pulses. The transient optical bistability connected with the nonlinear absorption's saturation in the quasi-cw four-wave mixing and with the inertia in the short pulse's regime is observed.

DOI
10.1117/12.238058

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The characteristic features of the conjugate wave's formation under transient four-wave mixing in a two-level medium are investigated. The phase modulations of the signal and conjugate waves induced in the four-wave mixing are not mutually conjugate and have the same sign. The fulfillment of the phase-conjugation for the phase modulated signal has been shown in particular to be connected with the envelope's deformation and the spectrum's change of signal pulses. The transient optical bistability connected with the nonlinear absorption's saturation in the quasi-cw four-wave mixing and with the inertia in the short pulse's regime is observed.
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An investigation is reported of the characteristic features of a four-wave mixing of a chirped signal with bandwidth- limited pump waves in a resonant medium modeled by a two- level scheme. Analytic estimates are obtained and a numerical analysis is made of the combined influence of various mechanisms (spatial phase matching, a finite nonlinear response time, and phase cross-modulation) on the spectral composition and on the temporal behavior of the fourth pulse. Conditions are found for achieving, with practically undetectable distortions, phase conjugation of a chirped signal accompanied by shortening of the pulse envelope and narrowing of the spectrum of the phase- conjugate wave.
An investigation is reported of the characteristic features of four-wave interaction of a chirped signal with bandwidth-limited pump waves in a resonant medium modelled by a two-level scheme. Analytic estimates are obtained and a numerical analysis is made of the combined influence of various mechanisms (spatial phase matching, a finite nonlinear response time, and phase cross-modulation) on the spectral composition and on the temporal behaviour of the fourth pulse. Conditions are found for achieving, with practically undetectable distortions, phase conjugation of a chirped signal accompanied by shortening of the pulse envelope and narrowing of the spectrum of the phase-conjugate wave.
The transient behavior of degenerate four-wave mixing (DFWM) in a three-level saturable absorber is analyzed and verified experimentally. A sharp peak of phase-conjugated reflectivity is predicted and observed at high pump intensities for pulsed beams. The influence of the time-dependent behavior of the conjugate wave signal on results of pulsed-beam experiments is studied. It is shown that transient effects could account for discrepancies between previous experimental results and steady-state theory.
A set of coupled equations is derived and used to analyze transient coherent degenerate four-wave mixing (DFWM) in a two-level system. The numerical results show that in the case of near-resonance, intense pumping, and short pulses, the properties of degenerate four-wave mixing have interesting coherent interaction characteristics, such as quasi-periodicity in the pump pulse area, probe pulse areas, and energy reflectivity, oscillatory behavior of the DFWM pulse, and generation of a DFWM signal in the case of delayed incidence, where the three incident pulses do not overlap in the medium.>
Degenerate four-wave mixing (DFWM) and phase conjugation (PC) of pulsed CO2 laser radiation on transient gratings inside its own laser medium have been studied both experimentally and theoretically. The operational mode of the e-beam controlled discharge CO2 laser has been chosen in such a way (CO2:N2:He equals 1:2:4, p equals 0.28 atm, tin equals 30 microsecond(s) ) that the laser pulse length ((tau) out approximately 10 - 20 microsecond(s) ) is comparable with an effective relaxation time of the upper laser level ((tau) rel approximately 15 - 30 microsecond(s) ). The time-history of the CO2 laser and PC signal pulses, and PC reflectivity have been thoroughly investigated for different cavity Q factors and specific electrical energy inputs. It has been shown, that the formation of the PC signal under the intracavity DFWM on gain (amplitude) and thermal (phase) gratings is characterized by a complicated time history that reflects the main relaxation processes taking place inside the inverted medium. A feature of the transient PC process inside the laser active medium is the dependence of the effective relaxation time of the upper laser level on the intensity of pumping waves. PC reflectivity has been obtained by numerical calculations. A comparison of the theoretical and experimental data confirms the contribution of two different mechanisms of grating formation under DFWM inside the active medium of the CO2 laser.