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Optics Communications

The effects of optical pumping on laser enhanced electron impact ionization of atoms

S. M. Park, Gerald J. Diebold

Published Jan 1, 1989• 1 citation
Publisher
DOI
10.1016/0030-4018(89)90110-7

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A review of current work at Manchester is given, with emphasis on low energy electron impact ionization & excitation experiments from laser-prepared targets. Three different methods are considered: super-elastic scattering from targets prepared by laser radiation in an optical enhancement cavity, (e,2e) studies of laser-aligned atoms, and electron impact ionization studies from laser cooled atoms in a new type of atom trap - the AC-MOT. The status of each experimental programme is detailed, and new data presented. Future directions and techniques are then discussed.
The ionization of 6sns1S06sns^{1}S_{0}6sns1S0​ Rydberg states of 138Ba^{138}\mathrm{Ba}138Ba has been investigated by high-resolution electron spectroscopy. The Rydberg states were excited by two cw dye lasers via the 6s6p1P16s6p^{1}P_{1}6s6p1P1​ level. The electron spectra show rich structure between 0.025 and 3 eV, largely attributable to collisional (Penning) ionization, photoionization, and autoionizing transitions. The first process might be interpreted as superelastic scattering of the Rydberg electron by optically pumped Ba(6s6p1P1)\mathrm{Ba}(6s6p^{1}P_{1})Ba(6s6p1P1​) or Ba(6s5d1D2)\mathrm{Ba}(6s5d^{1}D_{2})Ba(6s5d1D2​) atoms.