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Physical Review Letters

Stopping Light via Hot Atoms

Olga A. Kocharovskaya, Yuri V. Rostovtsev, Marlan O. Scully

Published Jan 22, 2001• 293 citations
Publisher

Abstract

We prove that it is possible to freeze a light pulse (i.e., to bring it to a full stop) or even to make its group velocity negative in a coherently driven Doppler broadened atomic medium via electromagnetically induced transparency (EIT). This remarkable phenomenon of the ultraslow EIT polariton is based on the spatial dispersion of the refraction index n(omega,k), i.e., its wave number dependence, which is due to atomic motion and provides a negative contribution to the group velocity. This is related to, but qualitatively different from, the recently observed light slowing caused by large temporal (frequency) dispersion.

DOI
10.1103/physrevlett.86.628

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Fast light, slow light and left-handed light

The propagation of light in dispersive media is a subject of fundamental as well as practical importance. In recent years attention has focused in particular on how refractive index can vary with frequency in such a way that the group velocities of optical pulses can be much greater or much smaller than the speed of light in vacuum, or in which the refractive index can be negative. Treating these topics at an introductory to intermediate level, Fast Light, Slow Light and Left-Handed Light focuses on the basic theory and describes the significant experimental progress made during the past decade. The book pays considerable attention to the fact that superluminal group velocities are not in conflict with special relativity and to the role of quantum effects in preventing superluminal communication and violations of Einstein causality. It also explores some of the basic physics at the opposite extreme of very slow group velocities as well as stopped and regenerated light, including the concepts of electromagnetically induced transparency and dark-state polaritons. Another very active aspect of the subject discussed concerns the possibility of designing metamaterials in which the refractive index can be negative and propagating light is left-handed in the sense that the phase and group velocities are in opposite directions. The last two chapters are an introduction to some of the basic theory and consequences of negative refractive index, with emphasis on the seminal work carried out since 2000. The possibility that "perfect" lenses can be made from negative-index metamaterials-which has been perhaps the most controversial aspect of the field-is introduced and discussed in some detail.

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We prove that it is possible to freeze a light pulse (i.e., to bring it to a full stop) or even to make its group velocity negative in a coherently driven Doppler broadened atomic medium via electromagnetically induced transparency (EIT). This remarkable phenomenon of the ultraslow EIT polariton is based on the spatial dispersion of the refraction index n(omega,k), i.e., its wave number dependence, which is due to atomic motion and provides a negative contribution to the group velocity. This is related to, but qualitatively different from, the recently observed light slowing caused by large temporal (frequency) dispersion.
Summary form only given. Electromagnetically induced transparency (EIT) has been the subject of many experimental and theoretical studies over recent years. Most recently, substantial experimental and theoretical work in this area has been focused on the use of EIT to give ultraslow group velocities for light in both ultracold atomic gas and hot atomic vapors. Much of this interest is based on the fact that slowing the group velocity of a laser pulse down to the speed of sound in the same material can produce strong coupling between acoustic waves and the electromagnetic field. It has been suggested that a giant nonlinearity obtained by this method might be utilized for efficient multi-wave mixing and quantum nondemolition measurements. Slow light might also allow a very efficient nonlinear interaction between laser pulses of extremely low (down to a single photon) energies. Here, we report the first direct observation of an ultraslow group velocity of light down to 45 m/s in a solid, well below the speed of sound in the medium. This group velocity is fundamentally limited only by the inhomogeneous broadening of the ground state transition. At low coupling beam intensities, the fraction of centers that are pumped into the "dark state" increases with coupling laser power, so that the observed group delay is increasing with coupling beam intensity. At higher intensities, power broadening reduces the sharpness of the dispersive feature and the observed group delay decreases.
A number of experiments have been performed on light slowing and stopping in the electromagnetically induced transparency (EIT) media of hot atomic gases where the Doppler-shift may add detunings to the field frequencies in an inhomogeneous fashion. We provide here a theoretical analysis as to the effect of such a Doppler-broadened environment on the dynamics of the system in comparison to a cold atomic medium. We will show that one of the most critical factors in the formation of a stationary light pulse is the enhancement of the excited-state decay rate caused by the collisions between the atoms of the medium and the molecules of the buffer gas.
The propagation of light in dispersive media is a subject of fundamental as well as practical importance. In recent years attention has focused in particular on how refractive index can vary with frequency in such a way that the group velocities of optical pulses can be much greater or much smaller than the speed of light in vacuum, or in which the refractive index can be negative. Treating these topics at an introductory to intermediate level, Fast Light, Slow Light and Left-Handed Light focuses on the basic theory and describes the significant experimental progress made during the past decade. The book pays considerable attention to the fact that superluminal group velocities are not in conflict with special relativity and to the role of quantum effects in preventing superluminal communication and violations of Einstein causality. It also explores some of the basic physics at the opposite extreme of very slow group velocities as well as stopped and regenerated light, including the concepts of electromagnetically induced transparency and dark-state polaritons. Another very active aspect of the subject discussed concerns the possibility of designing metamaterials in which the refractive index can be negative and propagating light is left-handed in the sense that the phase and group velocities are in opposite directions. The last two chapters are an introduction to some of the basic theory and consequences of negative refractive index, with emphasis on the seminal work carried out since 2000. The possibility that "perfect" lenses can be made from negative-index metamaterials-which has been perhaps the most controversial aspect of the field-is introduced and discussed in some detail.
The propagation of light in dispersive media is a subject of fundamental as well as practical importance. In recent years attention has focused in particular on how refractive index can vary with frequency in such a way that the group velocities of optical pulses can be much greater or much smaller than the speed of light in vacuum, or in which the refractive index can be negative. Treating these topics at an introductory to intermediate level, Fast Light, Slow Light and Left-Handed Light focuses on the basic theory and describes the significant experimental progress made during the past decade. The book pays considerable attention to the fact that superluminal group velocities are not in conflict with special relativity and to the role of quantum effects in preventing superluminal communication and violations of Einstein causality. It also explores some of the basic physics at the opposite extreme of very slow group velocities as well as stopped and regenerated light, including the concepts of electromagnetically induced transparency and dark-state polaritons. Another very active aspect of the subject discussed concerns the possibility of designing metamaterials in which the refractive index can be negative and propagating light is left-handed in the sense that the phase and group velocities are in opposite directions. The last two chapters are an introduction to some of the basic theory and consequences of negative refractive index, with emphasis on the seminal work carried out since 2000. The possibility that "perfect" lenses can be made from negative-index metamaterials-which has been perhaps the most controversial aspect of the field-is introduced and discussed in some detail.