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Physical review. B, Solid state

Tricritical exponents and crossover behavior of a next-nearest-neighbor Ising antiferromagnet

David Paul Landau

Published Nov 1, 1976• 30 citations
Publisher

Abstract

Monte Carlo data for a simple cubic Ising antiferromagnet with nearest- and next-nearest-neighbor interactions reveal asymptotic tricritical behavior of the order parameter which is mean-field-like modified by logarithmic corrections and high-temperature susceptibilities which are mean-field-like without corrections, in agreement with renormalization-group calculations. Crossover between tricritical and critical behavior is observed in the temperature variation of the order parameter and high-temperature susceptibility.

DOI
10.1103/physrevb.14.4054

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Canadian Journal of Physics•Jul 1, 1977•2 citations
Monte Carlo data for a simple cubic Ising antiferromagnet with nearest- and next-nearest-neighbor interactions reveal asymptotic tricritical behavior of the order parameter which is mean-field-like modified by logarithmic corrections and high-temperature susceptibilities which are mean-field-like without corrections, in agreement with renormalization-group calculations. Crossover between tricritical and critical behavior is observed in the temperature variation of the order parameter and high-temperature susceptibility.
The nnn model is an Ising model with nearest-neighbor antiferromagnetic interactions (J1<0{J}_{1}<0J1​<0) but also next-nearest-neighbor ferromagnetic exchange (J2>0{J}_{2}>0J2​>0). This model is analyzed in external magnetic field using the same techniques as applied to the meta model of Paper I. Again, the staggered susceptibility ${\ensuremath{\chi}}_{\mathrm{st}}$ appears to diverge along the critical line in the $H\ensuremath{-}T$ plane with a constant exponent ${\ensuremath{\gamma}}_{\mathrm{st}}=\frac{5}{4}$, consistent with the universality hypothesis. However, in contrast to the meta model, it is found that the direct susceptibility $\ensuremath{\chi}$ diverges at the tricritical point with an exponent $\overline{\ensuremath{\gamma}}\ensuremath{\simeq}\frac{1}{4}$. Implications of the scaling hypothesis at the tricritical point are discussed and the results for both the meta and nnn models are utilized to obtain the scaling power a‾2{\overline{a}}_{2}a2​ corresponding to the "weak" direction (in the sense of Griffiths and Wheeler). Included in this discussion is the double-power-law form, predicted to hold within the crossover region by tricritical-point scaling.
The phase diagrams of Ising antiferromagnets in a magnetic field HHH are investigated for various values of the ratio RRR between nearest- and next-nearest-neighbor interaction. While meanfield approximations and the existing real-space renormalization-group treatments yield phase diagrams which are sometimes even qualitatively incorrect, accurate results are obtained from Monte Carlo calculations. For R<0R<0R<0 only an antiferromagnetically ordered phase exists. Its transition to the disordered phase is first order for temperatures below the tricritical point (Tt{T}_{t}Tt​,Ht{H}_{t}Ht​). For $R\ensuremath{\rightarrow}0$ also ${T}_{t}\ensuremath{\rightarrow}0$. For R=0R=0R=0 we find very good agreement with the results of M\"uller-Hartmann and Zittartz. For R>0R>0R>0 and H1<H<H2{H}_{1}<H<{H}_{2}H1​<H<H2​ a new phase with anomalous high ground-state degeneracy is found (two sublattices have only one-dimensional order). These sublattices undergo order-disorder transitions at T=0T=0T=0, such that for T>0T>0T>0 one is left with a "superantiferromagnetic" phase. At low temperatures in this phase a pronounced tendency is observed to form a simpler (2 \ifmmode\times\else\texttimes\fi{} 2) superstructure but with many antiphase domain boundaries. For $R\ensuremath{\rightarrow}\frac{1}{2}$ and H<H1H<{H}_{1}H<H1​ the regime of the antiferromagnetic phases goes to zero temperature, while for R>12R>\frac{1}{2}R>21​ the superantiferromagnetic phase exists also for H<H1H<{H}_{1}H<H1​. The order-disorder transition associated with this phase seems to have non-Ising critical exponents which vary as a function of RRR and HHH. Estimates for the exponents lead us to suggest that Suzuki's "weak universality" is valid. The behavior of the model at T=0T=0T=0 is related to known results on hard-core lattice gases. It is shown that it is useful to interpret the transitions at T=0T=0T=0 as generalized percolation transitions. Since the model may have applications to adsorbate phases in registered structures at (100) surfaces of cubic crystals, the transcription of our results to temperature-coverage phase diagrams and adsorption isotherms is discussed in detail, and possible experimental applications are mentioned.
The tricritical behavior of a model studied by Harbus and Stanley is reanalyzed. The Harbus-Stanley analysis of the direct susceptibility suggested anomalous (i.e., non-mean-field-like) tricritical exponents. The tricritical point cannot be unambiguously located by present series data. We point out that, if the true tricritical temperature were actually somewhat lower than the Harbus-Stanley value, then standard ratio analysis would give tricritical exponents consistent with the Gaussian-tricritical-fixed-point analysis of Riedel and Wegner. However, the present situation remains inconclusive.
The thermodynamic properties of the antiferromagnetic Ising simple cubic and square lattices with nearest-neighbor and next-nearest-neighbor interactions have been studied using a Monte Carlo technique. Although both systems were found to possess magnetic tricritical points, their behavior in the "tricritical region" differed from that found in He3{\mathrm{He}}^{3}He3-He4{\mathrm{He}}^{4}He4 mixtures.