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Physical review. B, Condensed matter

Quantum phase transitions and thermodynamics of quantum antiferromagnets with next-nearest-neighbor couplings

Andrei A. Zvyagin, Andreas Klümper

Published Oct 20, 2003• 36 citations
Publisher

Abstract

We study quantum spin models with nearest- and next-nearest-neighbor exchange interactions by means of exact solutions. Depending on the representation, the models can also be viewed as spin ladders with interchain couplings and with ring biquadratic spin-spin interactions. The ground-state phase diagram is constructed as a function of the next-nearest-neighbor couplings and an external magnetic field. Several quantum phase transitions in the ground state, including the possibility of a first-order quantum phase transition, governed by the external magnetic field, are predicted. The low-energy conformal behavior of the low-lying excitations is studied in the commensurate and incommensurate phases. Finally, the properties of the models at finite temperature are studied exactly. A finite set of nonlinear integral equations determining the thermodynamic potential at arbitrary temperature and external magnetic field is derived and solved in several important cases. The results for the magnetic susceptibility and the Sommerfeld coefficient of the specific heat are presented.

DOI
10.1103/physrevb.68.144426

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Several exactly solvable quantum spin models with incommensurate magnetic structures, which manifest quantum phase transitions between incommensurate and commensurate phases, are proposed. The ground-state and thermodynamic characteristics of these quantum spin antiferromagnetic models with the Dzyaloshinsky-Moriya antisymmetric exchange interaction and spin-frustrating next-nearest-neighbor, three-spin, and four-spin (ring exchange) interactions are exactly studied. We investigated the ground state phases of the considered models, as function of the magnetic anisotropy, Dzyaloshinsky-Moriya interaction, next-nearest-neighbor coupling constants, and external magnetic field. Several quantum phase transitions between magnetically incommensurate phases and between incommensurate and ferromagnetic phases are predicted, and the behavior of thermodynamic characteristics of those models at phase transitions is studied. We have shown that for models with chiral three-spin interactions the Dzyaloshinsky-Moriya coupling yields the onset of the weak ferromagnetism, similar to three-dimensional ordered antiferromagnets, but not present in other quantum spin chains with the antisymmetric exchange. Considered models appeared to be important for several quasi-one-dimensional spin systems, studied in recent experiments.
We study the isotropic Heisenberg chain with nearest and next-nearest neighbor interactions. The ground state phase diagram is constructed in dependence on the additional interactions and an external magnetic field. The thermodynamics is studied by the use of finite sets of nonlinear integral equations resulting from integrability. The equations are solved numerically and analytically in suitable limiting cases. We find second- and first-order transition lines. The exponents of the low-temperature asymptotics at the phase transitions are determined.
A one-dimensional spin-1∕2 model in which the alternation of the exchange interactions between neighboring spins is accompanied by the next-nearest-neighbor (NNN) spin exchange (zig-zag spin ladder with alternation) is studied. The thermodynamic characteristics of the model quantum spin chain are obtained in the mean-field-like approximation. Depending on the strength of the NNN interactions, the model manifests either the spin-gapped behavior of low-lying excitations at low magnetic fields, or ferrimagnetic ordering in the ground state with gapless low-lying excitations. The system undergoes second-order or first-order quantum phase transitions, governed by the external magnetic field, NNN coupling strength, and the degree of the alternation. Hence, NNN spin–spin interactions in a dimerized quantum spin chain can produce a spontaneous magnetization. On the other hand, for quantum spin chains with a spontaneous magnetization, caused by NNN spin–spin couplings, the alternation of nearest-neighbor (NN) exchange interactions can cause destruction of that magnetization and the onset of a spin gap for low-lying excitations. Alternating NN interactions produce a spin gap between two branches of low-energy excitations, and the NNN interactions yield asymmetry of the dispersion laws of those excitations, with possible minima corresponding to incommensurate structures in the spin chain.
We study the isotropic Heisenberg chain with nearest and next-nearest neighbor interactions. The ground state phase diagram is constructed in dependence on the additional interactions and an external magnetic field. The thermodynamics is studied by use of finite sets of nonlinear integral equations resulting from integrability. The equations are solved numerically and analytically in suitable limiting cases. We find second and first order transition lines. The exponents of the low-temperature asymptotics at the phase transitions are determined.
We propose an exactly solvable quantum spin model, in which the alternation of the exchange interactions between neighboring spins is accompanied by the multiple spin exchange. The model permits us to obtain exactly thermodynamic characteristics of the considered quantum spin chain. In the ground state, depending on the strength of the three-spin coupling, the model manifests either the spin-gapped behavior of low-lying excitations at low magnetic fields, or the ferrimagnetic ordering with the spontaneous magnetization and with gapless low-lying excitations. The system undergoes second order or first order quantum phase transitions, governed by an external magnetic field and the multiple spin exchange coupling strength. Our exactly solvable quantum spin model demonstrates that multispin interactions in a dimerized quantum spin chain can produce a spontaneous magnetization. On the other hand, for quantum spin chains with a spontaneous magnetization, caused by multispin couplings, the alternation of nearest neighbor exchange interactions can be the reason for destroying of that magnetization and the onset of a spin gap for low-lying excitations.
The behavior in an external magnetic field is studied exactly for a wide class of multichain quantum spin models. It is shown that the magnetic field together with the interchain couplings cause commensurate–incommensurate phase transitions between the gapless phases in the ground state. The conformal limit of these models is studied and it is shown that the low-lying excitations for the incommensurate phases are not independent, because they are governed by the same magnetic field (chemical potential for excitations). A scenario for the transition from one to two space dimensions for the exactly integrable multichain quantum spin models is proposed, and it is shown that the incommensurate phases in an external magnetic field disappear in the limit of an infinite number of coupled spin chains. The similarities in the external field behavior for the quantum multichain spin models and a wide class of quantum field theories are discussed. The scaling exponents for the appearance of the gap in the spectrum of low-lying excitations of the quantum multichain models due to the relevant perturbations of the integrable theories are calculated.