Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Optics Express

Measuring the dynamics of second-order photon correlation functions inside a pulse with picosecond time resolution

Marc Aßmann, Franziska Veit, Jean-Sebastian Tempel, T. Berstermann, H. Stolz, Mike van der Poel, J. M. Hvam, M. Bayer

Published Sep 8, 2010• 46 citations
Publisher

Abstract

We present a detailed discussion of a recently demonstrated experimental technique capable of measuring the correlation function of a pulsed light source with picosecond time resolution. The measurement involves a streak camera in single photon counting mode, which is modified such that a signal at a fixed repetition rate, and well defined energy, can be monitored after each pulsed laser excitation. The technique provides further insight into the quantum optical properties of pulsed light emission from semiconductor nanostructures, and the dynamics inside a pulse, on the sub-nanosecond time scale.

DOI
10.1364/oe.18.020229

Related papers

Second-order photon correlation measurement with picosecond resolution using frequency upconversion

Aymeric Delteil, Chun Tat Ngai, Thomas Fink +1 more

The second-order correlation function of light g(2)(τ) constitutes a pivotal tool to quantify the quantum behavior of an emitter and in turn its potential for quantum information applications. The experimentally accessible time resolution of g(2)(τ) is usually limited by the jitter of available single-photon detectors. Here, we present a versatile technique allowing g(2)(τ) to be measured from a large variety of light signals with a time resolution given by the pulse length of a mode-locked laser. The technique is based on frequency upconversion in a nonlinear waveguide, and we analyze its properties and limitations by modeling the pulse propagation and the frequency conversion process. We measure g(2)(τ) from various signals including light from a quantum emitter—a confined exciton-polariton structure—revealing its quantum signatures at a scale of a few picoseconds and demonstrating the capability of the technique.

arXiv:1904.02515•Optics Letters•Jul 30, 2019•7 citations

Second-order photon correlation measurement with picosecond resolution using frequency upconversion

Aymeric Delteil, Chun Tat Ngai, Fink, Thomas +1 more

The second-order correlation function of light g2τ constitutes a pivotal tool to quantify the quantum behavior of an emitter and in turn its potential for quantum information applications. The experimentally accessible time resolution of g2τ is usually limited by the jitter of available single-photon detectors. Here, we present a versatile technique allowing g2τ to be measured from a large variety of light signals with a time resolution given by the pulse length of a mode-locked laser. The technique is based on frequency upconversion in a nonlinear waveguide, and we analyze its properties and limitations by modeling the pulse propagation and the frequency conversion process. We measure g2τ from various signals including light from a quantum emitter—a confined exciton-polariton structure—revealing its quantum signatures at a scale of a few picoseconds and demonstrating the capability of the technique.

•Jul 1, 2019•4 citations

Novel technique for photon correlation measurements at high photon rates and resolutions

Dimitar Stoyanov

A novel technique for photon correlation measurements, based on the excitation of a resonant system by photon-detector single pulses, analog/digital sampling, and deconvolution, has been developed and analyzed experimentally and by computer simulations. The measured correlation function is expressed by a convolution of the true photon correlation function of the optical field and a well-defined, noiseless resonator correlation function. The effect of detector statistics is reduced to the contribution of two integral parameters—the total single-pulse charge and the jitter of single-pulse centers. Good performance of this technique is demonstrated at high photon rates and resolutions, where the well-known photon-counting or single-quantum methods are ineffective. The novel technique offers linear recording of photocount time series without dead-time effects. The temporal resolution is defined by the sampling step of the analog/digital converter. The retrieval error does not exceed 1 to 3% at count rates higher than 1 GHz and single-pulse durations larger than the resolution cell. This technique can be effectively applied in photon correlation measurements of high dynamic optical fields.

Optical Engineering•Jun 1, 1997•3 citations

Ultrafast photonic quantum correlations mediated by individual phonons (Conference Presentation)

Christophe Galland, Santiago Tarrago Velez, Mitchell D. Anderson

We present a new experiment, in which we measure quantum correlations between single photons that are mediated by the exchange of a single phonon. We create and annihilate a single optical phonon in bulk diamond using two ultrashort laser pulses at two different wavelengths, generated by a Ti:Sapph oscillator and a frequency-doubled optical parametric oscillator (APE Berlin). During Stokes Raman scattering, the first pulse creates a photon-phonon pair, while the second pulse convert the same phonon into an anti-Stokes photon. Using spectral filtering and photon counting, we measure the cross-correlations between the Stokes and anti-Stokes photons with a few hundred femtoseconds time resolution. As expected, the non-classical correlation (g(2) much larger than the classical bound) decays within a few picosecond, following to the dynamics of the phonon mode. Our results demonstrate a new source of broadly tunable quantum correlated photons, and can be extended to provide a new way of measuring non-classical dynamics in nanoscale systems — down to individual nanostructures.

SPIE Quantum Technologies•May 29, 2018•0 citations

Dynamics of a pulsed single photon source

Sergey Vladimirovich Polyakov, Edward B. Flagg, Tim O. Thomay +1 more

We propose and demonstrate a method for an independent verification of a degree of single photon purity and coherence applicable for all single-photon emitters used in pulsed mode. Using two-time second-order correlation measurements, we reconstruct the dynamics of the nonclassical photon wavepacket. This reveals the temporal evolution of the photon field during the excitation-relaxation cycle of an emitter. The technique allows for the simultaneous measurement of multiphoton content and decoherence. Here we applied this technique to characterize a nonclassical state produced from a single InAs quantum dot (QD). We experimentally observe variations in the degree of multiphoton content and coherence of the wavepacket. A rate equation is introduced to explain multiphoton variations of our source and is found to describe the observed two-dimensional second-order correlation function accurately.

AIP conference proceedings•Jan 1, 2012•2 citations

Higher-Order Photon Bunching in a Semiconductor Microcavity

Marc Aßmann, Franziska Veit, M. Bayer +2 more

Quantum mechanically indistinguishable particles such as photons may show collective behavior. Therefore, an appropriate description of a light field must consider the properties of an assembly of photons instead of independent particles. We have studied multiphoton correlations up to fourth order in the single-mode emission of a semiconductor microcavity in the weak and strong coupling regimes. The counting statistics of single photons were recorded with picosecond time resolution, allowing quantitative measurement of the few-photon bunching inside light pulses. Our results show bunching behavior in the strong coupling case, which vanishes in the weak coupling regime as the cavity starts lasing. In particular, we verify the n factorial prediction for the zero-delay correlation function of n thermal light photons.

Science•Jul 16, 2009•115 citations
We present a detailed discussion of a recently demonstrated experimental technique capable of measuring the correlation function of a pulsed light source with picosecond time resolution. The measurement involves a streak camera in single photon counting mode, which is modified such that a signal at a fixed repetition rate, and well defined energy, can be monitored after each pulsed laser excitation. The technique provides further insight into the quantum optical properties of pulsed light emission from semiconductor nanostructures, and the dynamics inside a pulse, on the sub-nanosecond time scale.
The second-order correlation function of light g(2)(τ) constitutes a pivotal tool to quantify the quantum behavior of an emitter and in turn its potential for quantum information applications. The experimentally accessible time resolution of g(2)(τ) is usually limited by the jitter of available single-photon detectors. Here, we present a versatile technique allowing g(2)(τ) to be measured from a large variety of light signals with a time resolution given by the pulse length of a mode-locked laser. The technique is based on frequency upconversion in a nonlinear waveguide, and we analyze its properties and limitations by modeling the pulse propagation and the frequency conversion process. We measure g(2)(τ) from various signals including light from a quantum emitter—a confined exciton-polariton structure—revealing its quantum signatures at a scale of a few picoseconds and demonstrating the capability of the technique.
The second-order correlation function of light g2τ constitutes a pivotal tool to quantify the quantum behavior of an emitter and in turn its potential for quantum information applications. The experimentally accessible time resolution of g2τ is usually limited by the jitter of available single-photon detectors. Here, we present a versatile technique allowing g2τ to be measured from a large variety of light signals with a time resolution given by the pulse length of a mode-locked laser. The technique is based on frequency upconversion in a nonlinear waveguide, and we analyze its properties and limitations by modeling the pulse propagation and the frequency conversion process. We measure g2τ from various signals including light from a quantum emitter—a confined exciton-polariton structure—revealing its quantum signatures at a scale of a few picoseconds and demonstrating the capability of the technique.
A novel technique for photon correlation measurements, based on the excitation of a resonant system by photon-detector single pulses, analog/digital sampling, and deconvolution, has been developed and analyzed experimentally and by computer simulations. The measured correlation function is expressed by a convolution of the true photon correlation function of the optical field and a well-defined, noiseless resonator correlation function. The effect of detector statistics is reduced to the contribution of two integral parameters—the total single-pulse charge and the jitter of single-pulse centers. Good performance of this technique is demonstrated at high photon rates and resolutions, where the well-known photon-counting or single-quantum methods are ineffective. The novel technique offers linear recording of photocount time series without dead-time effects. The temporal resolution is defined by the sampling step of the analog/digital converter. The retrieval error does not exceed 1 to 3% at count rates higher than 1 GHz and single-pulse durations larger than the resolution cell. This technique can be effectively applied in photon correlation measurements of high dynamic optical fields.
We present a new experiment, in which we measure quantum correlations between single photons that are mediated by the exchange of a single phonon. We create and annihilate a single optical phonon in bulk diamond using two ultrashort laser pulses at two different wavelengths, generated by a Ti:Sapph oscillator and a frequency-doubled optical parametric oscillator (APE Berlin). During Stokes Raman scattering, the first pulse creates a photon-phonon pair, while the second pulse convert the same phonon into an anti-Stokes photon. Using spectral filtering and photon counting, we measure the cross-correlations between the Stokes and anti-Stokes photons with a few hundred femtoseconds time resolution. As expected, the non-classical correlation (g(2) much larger than the classical bound) decays within a few picosecond, following to the dynamics of the phonon mode. Our results demonstrate a new source of broadly tunable quantum correlated photons, and can be extended to provide a new way of measuring non-classical dynamics in nanoscale systems — down to individual nanostructures.
We propose and demonstrate a method for an independent verification of a degree of single photon purity and coherence applicable for all single-photon emitters used in pulsed mode. Using two-time second-order correlation measurements, we reconstruct the dynamics of the nonclassical photon wavepacket. This reveals the temporal evolution of the photon field during the excitation-relaxation cycle of an emitter. The technique allows for the simultaneous measurement of multiphoton content and decoherence. Here we applied this technique to characterize a nonclassical state produced from a single InAs quantum dot (QD). We experimentally observe variations in the degree of multiphoton content and coherence of the wavepacket. A rate equation is introduced to explain multiphoton variations of our source and is found to describe the observed two-dimensional second-order correlation function accurately.
Quantum mechanically indistinguishable particles such as photons may show collective behavior. Therefore, an appropriate description of a light field must consider the properties of an assembly of photons instead of independent particles. We have studied multiphoton correlations up to fourth order in the single-mode emission of a semiconductor microcavity in the weak and strong coupling regimes. The counting statistics of single photons were recorded with picosecond time resolution, allowing quantitative measurement of the few-photon bunching inside light pulses. Our results show bunching behavior in the strong coupling case, which vanishes in the weak coupling regime as the cavity starts lasing. In particular, we verify the n factorial prediction for the zero-delay correlation function of n thermal light photons.