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Physical Review A

Laser cooling at low intensity in a strong magnetic field

P. van der Straten, S-Q. Shang, B. Sheehy, H. Metcalf, Gerard Nienhuis

Published May 1, 1993• 23 citations
Publisher

Abstract

We have studied theoretically and experimentally the effect of a relatively strong magnetic field on sub-Doppler laser cooling in a one-dimensional optical molasses. We used the operator description of laser cooling with the Larmor precession frequency ${\mathrm{\ensuremath{\omega}}}_{\mathit{Z}}$ being much higher than the optical pumping rate. We found velocity-selective resonances (VSR) in the force at velocities ${\mathit{v}}_{\mathit{r}}$=n${\mathrm{\ensuremath{\omega}}}_{\mathit{Z}}$, with n=0,\ifmmode\pm\else\textpm\fi{}1,\ifmmode\pm\else\textpm\fi{}2 for both the scattering and redistribution force operators. These depend on the relative direction of the magnetic field and the polarization vectors of the light beams. Analytical results for the force on the atom are obtained in two cases that illustrate the effect of the VSR on the force. These formulas are compared with numerical calculations of the force. We also discovered a redistribution mechanism that relies on the gradient of the eigenstates of the light-shift operator, with eigenvalues that are independent of position so that a ``Sisyphus cooling'' picture does not apply. The theory is compared with many experimental results and excellent agreement is found. We believe that all essential features of laser cooling at low intensity are well described by this operator theory.

DOI
10.1103/physreva.47.4160

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Journal of Physics B Atomic Molecular and Optical Physics•Sep 28, 1993•16 citations
We have studied theoretically and experimentally the effect of a relatively strong magnetic field on sub-Doppler laser cooling in a one-dimensional optical molasses. We used the operator description of laser cooling with the Larmor precession frequency \ensuremathωZ{\mathrm{\ensuremath{\omega}}}_{\mathit{Z}}\ensuremathωZ​ being much higher than the optical pumping rate. We found velocity-selective resonances (VSR) in the force at velocities vr{\mathit{v}}_{\mathit{r}}vr​=n\ensuremathωZ{\mathrm{\ensuremath{\omega}}}_{\mathit{Z}}\ensuremathωZ​, with n=0,\ifmmode\pm\else\textpm\fi{}1,\ifmmode\pm\else\textpm\fi{}2 for both the scattering and redistribution force operators. These depend on the relative direction of the magnetic field and the polarization vectors of the light beams. Analytical results for the force on the atom are obtained in two cases that illustrate the effect of the VSR on the force. These formulas are compared with numerical calculations of the force. We also discovered a redistribution mechanism that relies on the gradient of the eigenstates of the light-shift operator, with eigenvalues that are independent of position so that a ``Sisyphus cooling'' picture does not apply. The theory is compared with many experimental results and excellent agreement is found. We believe that all essential features of laser cooling at low intensity are well described by this operator theory.
We describe a new sub-Doppler cooling scheme that cools atoms to nonzero velocity vr{\mathit{v}}_{\mathit{r}}vr​. The atomic motion in a combined optical standing wave and constant magnetic field induces a velocity-selective magnetic resonance that produces strong cooling for negative laser detuning to vr{\mathit{v}}_{\mathit{r}}vr​=${\mathrm{\ensuremath{\omega}}}_{\mathit{Z}}$/2k, with ${\mathrm{\ensuremath{\omega}}}_{\mathit{Z}}$ the Larmor frequency. In a one-dimensinal optical molasses transverse to a thermal Rb beam we observe the bunching of the atoms into two peaks corresponding to \ifmmode\pm\else\textpm\fi{}vr{\mathit{v}}_{\mathit{r}}vr​. We present a quantitative comparison between our theory and experiment and suggest some applications.
We present two cooling mechanisms that lead to temperatures well below the Doppler limit. These mechanisms are based on laser polarization gradients and work at low laser power when the optical-pumping time between different ground-state sublevels becomes long. There is then a large time lag between the internal atomic response and the atomic motion, which leads to a large cooling force. In the simple case of one-dimensional molasses, we identify two types of polarization gradient that occur when the two counterpropagating waves have either orthogonal linear polarizations or orthogonal circular polarizations. In the first case, the light shifts of the ground-state Zeeman sublevels are spatially modulated, and optical pumping among them leads to dipole forces and to a Sisyphus effect analogous to the one that occurs in stimulated molasses. In the second case (σ+−σ− configuration), the cooling mechanism is radically different. Even at very low velocity, atomic motion produces a population difference among ground-state sublevels, which gives rise to unbalanced radiation pressures. From semiclassical optical Bloch equations, we derive for the two cases quantitative expressions for friction coefficients and velocity capture ranges. The friction coefficients are shown in both cases to be independent of the laser power, which produces an equilibrium temperature proportional to the laser power. The lowest achievable temperatures then approach the one-photon recoil energy. We briefly outline a full quantum treatment of such a limit.
We describe several one-dimensional sub-Doppler laser-cooling experiments that cool Rb to finite and zero velocities in a magnetic field and polarization gradients. We then present a physical picture that unifies these measurements in terms of coherent two-photon velocity-selective resonances between atomic ground-state sublevels (including Raman resonances). We propose several sub-Doppler cooling schemes without fields or without polarization gradients, based on VSR between nondegenerate ground states.
We investigate the effect of a longitudinal magnetic field on the orientational cooling mechanism that operates both in σ+–σ− optical molasses and in a magneto-optical trap. For an atom with different Landé g factors in its ground and excited states, single-photon scattering and stimulated Raman scattering are resonant at different field-dependent velocities. The sharp polarization-gradient feature in the force-versus-velocity curve may therefore be translated to a velocity at which the Doppler force is dominant. In addition to this, we find that the momentum diffusion coefficient can grow as the field is increased. By numerically solving a semiclassical Fokker–Planck equation, we show that these effects lead to a field-induced inhibition of efficient sub-Doppler cooling for atoms with unequal g factors. Our treatment also enables us to discuss other phenomena that are accessible only if both Doppler and polarization-gradient effects are included in the calculation.
We report a new cooling scheme used to actively collimate an atomic beam of 85Rb^{85}\mathrm{Rb}85Rb with one-dimensional optical molasses. The atoms' transverse velocity is damped by a standing wave of circularly polarized light in a magnetic field of \ensuremath{\sim}20 \ensuremath{\mu}T to 2 cm/s (rms), well below the Doppler velocity vD{v}_{D}vD​=(7\ensuremath{\Elzxh}\ensuremath{\gamma}/20M)1/2{)}^{1/2})1/2\ensuremath{\sim}10 cm/s for one-dimensional optical molasses. The minimum measured velocity is limited only by the experimental geometry. We have developed a model in which the mixing by the field and optical pumping combine to form a cycle that cools below the Doppler limit, in agreement with our measurements.
The force on a multilevel atom in a 1D magneto-optical molasses with imbalanced laser intensities is theoretically investigated. The authors employ a full quantum treatment to obtain the stationary momentum distribution of the atoms, for arbitrary parameters. The force exerted the counterpropagating laser beams balances for a nonzero locking velocity. The dependence of this velocity on the intensity imbalance is found to be reduced by polarization gradient cooling. For certain values of the imbalance there are two stable velocities, and a splitting of the velocity distribution occurs. A small imbalance, or a magnetic field along the laser beams, can cause the subDoppler cooling to be lost. However, by the correct choice of parameters these effects can be made to cancel, and the sub-Doppler cooling is regained.