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Physical Review Letters

Competition between singlet formation and magnetic ordering in one-dimensional spin systems

Steven P. Strong, Andrew J. Millis

Published Oct 19, 1992• 136 citations
Publisher

Abstract

We use mappings onto soluble models and Abelian bosonization to determine the phase diagram and correlation functions of a model of two coupled spin chains. We find quantum disordered singlet phases and magnetic phases and determine the phase boundaries, universality classes of transitions, and correlation functions. We believe our model captures the essential physics of the interplay between the Kondo effect and magnetic ordering, which may be important for the heavy fermion materials.

DOI
10.1103/physrevlett.69.2419

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We use mappings onto soluble models and Abelian bosonization to determine the phase diagram and correlation functions of a model of two coupled spin chains. We find quantum disordered singlet phases and magnetic phases and determine the phase boundaries, universality classes of transitions, and correlation functions. We believe our model captures the essential physics of the interplay between the Kondo effect and magnetic ordering, which may be important for the heavy fermion materials.
We study the behavior of a model of two XXZ spin chains coupled by an isotropic exchange interaction JK{\mathit{J}}_{\mathit{K}}JK​ as the anisotropies and spin velocities in the individual chains are varied. In the limit of large antiferromagnetic JK{\mathit{J}}_{\mathit{K}}JK​ we map the model's low-energy sector onto an Ising model in a transverse field; in the limit of large ferromagnetic JK{\mathit{J}}_{\mathit{K}}JK​ we map the model's low-energy sector onto that of a single spin-one chain. For small JK{\mathit{J}}_{\mathit{K}}JK​, we study the model perturbatively via Abelian and non-Abelian bosonization. We determine the possible phases, approximate locations of the phase boundaries, universality classes of the transitions, and asymptotic behavior of correlation functions. We believe our model captures the essential physics of the interplay between the compensation of local moments and magnetic ordering, which may be important for the heavy-fermion materials.
Using a non-Abelian density matrix renormalization group method we determine the phase diagram of the Kondo lattice model in one dimension, by directly measuring the magnetization of the ground state. This allowed us to discover a second ferromagnetic phase missed in previous approaches. The phase transitions are found to be continuous. The spin-spin correlation function is studied in detail, and we determine in which regions the large and small Fermi surfaces dominate. The importance of double-exchange ordering and its competition with Kondo singlet formation is emphasized in understanding the complexity of the model.
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We investigate the magnetic order and related strongly correlated effects in a one-dimensional Ising-Kondo lattice with transverse field. This model is the anisotropic limit of the conventional isotropic Kondo lattice model, in the sense that the itinerant electrons interact with the localized magnetic moments via only longitudinal Kondo exchange. Adopting the numerical density-matrix renormalization group method, we map out the ground-state phase diagram in various parameter spaces. Depending on the Kondo coupling and filling number, three distinct phases, including a metallic paramagnetic, a metallic ferromagnetic, and a gapped spin-density wave phase, are obtained. The spin-density wave is characterized by an ordering wave vector, which coincides with the nesting wave vector of the Fermi surface. This makes the corresponding magnetic transition a spin analog of the Peierls transition occurring in the one-dimensional metal. Moreover, by analyzing the momentum distribution function and charge correlation function, the conduction electrons are shown to behave like free spinless fermions in the ferromagnetic phase. We finally discuss the effect of the repulsive Hubbard interaction between conduction electrons. Our paper enriches the Kondo physics and deepens the current understanding of the heavy fermion compounds.
We investigate a model of two Kondo impurities coupled via an Ising interaction. Exploiting the mapping to a generalized single-impurity Anderson model, we establish that the model has a singlet and a (pseudospin) doublet phase separated by a Kosterlitz-Thouless quantum phase transition. Based on a strong-coupling analysis and renormalization-group arguments, we show that at this transition the conductance GGG through the system either displays a zero-bias anomaly, $G\ensuremath{\sim}{\ensuremath{\mid}V\ensuremath{\mid}}^{\ensuremath{-}2(\sqrt{2}\ensuremath{-}1)}$, or takes a universal value, $G=({e}^{2}∕\ensuremath{\pi}\ensuremath{\hbar}){\mathrm{cos}}^{2}(\ensuremath{\pi}∕2\sqrt{2})$, depending on the experimental setup. Close to the Toulouse point of the individual Kondo impurities, the strong-coupling analysis allows us to obtain the location of the phase boundary analytically. For general model parameters, we determine the phase diagram and investigate the thermodynamics using numerical renormalization-group calculations. In the singlet phase close to the quantum phase transition, the entropy is quenched in two steps: first the two Ising-coupled spins form a magnetic minidomain which is, in a second step, screened by a Kondoesque collective resonance in an effective solitonic Fermi sea. In addition, we present a flow-equation analysis which provides a different mapping of the two-impurity model to a generalized single-impurity Anderson model in terms of fully renormalized couplings, which is applicable for the whole range of model parameters.
We discuss models of interacting magnetic impurities coupled to a metallic host, which show one or more boundary quantum phase transitions where the ground-state spin changes as a function of the interimpurity couplings. The simplest example is realized by two spin-12\frac{1}{2}21​ Kondo impurities coupled to a single orbital of the host. We investigate the phase diagram and crossover behavior of this model and present numerical renormalization-group results together with general arguments showing that the singlet-doublet quantum phase transition is either of first order or of the Kosterlitz-Thouless type, depending on the symmetry of the Kondo couplings. Thus we find an exponentially small energy scale within the Kondo regime, and a two-stage Kondo effect, in a single-channel situation. Connections to other models and possible applications are discussed.