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New Journal of Physics

Light-mediated quantum phase transition and manipulations of the quantum states of arrayed two-level atoms

Chih-Chun Chang, Lee Lin

Published Jul 10, 2012• 5 citations
Publisher

Abstract

In a quantum electrodynamics (QED) system of arrayed two-level atoms interacting with light, because the energy of the photon is around the spacing between two atomic energy levels, the photon will be absorbed and is not in the propagating mode but the attenuated mode. Our theoretical study shows that coherent phasing of atomic states occurs when the photons are in the attenuated mode. The existence of this ordered state is a result of a quantum phase transition induced by the mediation of the attenuated photonic field. By tuning the intensity of the light, the ordered state can be manipulated so that two-level atoms can be in an arbitrary uniform linear combination of the single-atom ground state and the excited state. Potential applications of this phenomenon are quantum computation, lasing physics, optical lattices and related subjects in nanotechnology. Similar phase transitions induced by the mediation of transmuted intermediate boson-like phonons, magnons or other fields may also occur in condensed-matter systems.

DOI
10.1088/1367-2630/14/7/073018

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In a quantum electrodynamics (QED) system of arrayed two-level atoms interacting with light, because the energy of the photon is around the spacing between two atomic energy levels, the photon will be absorbed and is not in the propagating mode but the attenuated mode. Our theoretical study shows that coherent phasing of atomic states occurs when the photons are in the attenuated mode. The existence of this ordered state is a result of a quantum phase transition induced by the mediation of the attenuated photonic field. By tuning the intensity of the light, the ordered state can be manipulated so that two-level atoms can be in an arbitrary uniform linear combination of the single-atom ground state and the excited state. Potential applications of this phenomenon are quantum computation, lasing physics, optical lattices and related subjects in nanotechnology. Similar phase transitions induced by the mediation of transmuted intermediate boson-like phonons, magnons or other fields may also occur in condensed-matter systems.
In a quantum system of arrayed two-level atoms interacting with light, the interacted (dressed) photon is propagating in a periodic medium and its eigenstate ought to be of Bloch type with lattice symmetry. As the energy of photon is around the spacing between the two atomic energy levels, the photon will be absorbed and is not in the propagating mode but the attenuated mode. Therefore an energy gap exists in the dispersion relation of the photonic Bloch wave of dressed photon in addition to the nonlinear behaviors due to atom-light interactions. There follows several interesting results which are distinct from those obtained through a linear dispersion relation of free photon. For example, slow light can exist, the density of state of dressed photon is non-Lorentzian and is very large around the energy gap; the Rabi oscillations become monotonically decreasing in some cases; and besides the superradiance occurs at long wavelengths, the spontaneous emission is also very strong near the energy gap because of the high density of state.
Coupling between quantum emitters and modes of light is foundational to studies of quantum systems. Coherent interactions between matter and light have greatly advanced the development of quantum technologies. When an ensemble of atoms interacts with light that is confined within a cavity---a resonator for photons---light also mediates atom-atom interactions, leading to collective phenomena that cannot be extrapolated from microscopic behaviors. Understanding how interactions among quantum particles lead to macroscopic phenomena, such as phase transitions and breaking of symmetries, remains a challenge in modern physics. In this dissertation, I present results addressing this challenge in the context of mesoscopic arrays of optical-tweezer-trapped atoms interfaced with a high-finesse optical cavity. In particular, the physics we investigate arises from the collective scattering of light. Utilizing the ability to place atoms with nanometer-scale precision, we engineer superradiant and subradiant states, where control over interference of the emission from multiple atoms leads to collectively enhanced or suppressed amounts of scattered light. Building on this work, we investigate the emergence of optomechanical self-organization, mediated by superradiance in the cavity electromagnetic field. By coupling atoms to the same cavity mode, the atoms exert forces on one another through the exchange of photons, leading them to autonomously order themselves spatially. We characterize mesoscopic fluctuations and their effect on symmetry-breaking dynamics associated with self-organization. Finally, we extend this framework to theoretically investigate how the phase of the atom-cavity coupling can be altered to generate higher symmetries. Our analysis reveals first-order phase transitions and instabilities induced by non-reciprocal forces. Altogether, this work establishes a path towards realizing mesoscopic systems of complex phases of matter in cavity quantum electrodynamics with unprecedented programmability.
The atom - electromagnetic field interaction is studied in the Dicke model, wherein a single field mode is interacting with a collection of two level atoms at thermal equilibrium. It is found that in the superradiant phase of the system, wherein the Bose-Einstein condensation of photons takes place, the notion of photon as an elementary electromagnetic excitation ceases to exist. The phase and intensity excitations of the condensate are found to be the true excitations of electromagnetic field. It is found that in this phase, the atom interacts with these excitations in a distinct coherent transition process, apart from the known stimulated emission/absorption and spontaneous emission processes. In the coherent transition it is found that while the atomic state changes in course of the transition process, the state of electromagnetic field remains unaffected. It is found that the transition probability of such coherent transition process is macroscopically large compared to other stimulated emission/absorption and spontaneous emission processes.
Systems of strongly interacting atoms and photons, which can be realized wiring up individual cavity QED systems into lattices, are perceived as a new platform for quantum simulation. While sharing important properties with other systems of interacting quantum particles, here we argue that the nature of light-matter interaction gives rise to unique features with no analogs in condensed matter or atomic physics setups. By discussing the physics of a lattice model of delocalized photons coupled locally with two-level systems through the elementary light-matter interaction described by the Rabi model, we argue that the inclusion of counterrotating terms, so far neglected, is crucial to stabilize finite-density quantum phases of correlated photons out of the vacuum, with no need for an artificially engineered chemical potential. We show that the competition between photon delocalization and Rabi nonlinearity drives the system across a novel Z(2) parity symmetry-breaking quantum criticality between two gapped phases that share similarities with the Dicke transition of quantum optics and the Ising critical point of quantum magnetism. We discuss the phase diagram as well as the low-energy excitation spectrum and present analytic estimates for critical quantities.
Atom arrays are a new type of quantum light-matter interface.Here we propose to employ one-dimensional ordered arrays as atomic waveguides.These arrays support optical guided modes that do not decay into free space.We show that these modes can be harnessed to mediate tunable, long-range interactions between additional "impurity qubits" coupled to the chain, without need for photonic structures.The efficient coupling between qubits and atomic waveguides enables the realization of tunable qubit-qubit interactions, which can be short or long range, dissipative or coherent, as well as chiral.Moreover, owing to the two-level nature of atoms, these waveguides are intrinsically quantum.In contrast to classical waveguides, where photons do not interact with each other, atomic waveguides display strong nonlinearities, which create a tunable dissipative channel for qubit-qubit interactions, and opens the door to the exploration of many-body physics between guided photons.This physics is universal as it only relies on photon interference and can also be observed with other types of quantum emitters, such as those in molecular or solid-state systems.
We study the quantum phase transition between superfluid and Mott-insulator states for ultracold bosons with two internal states forming two bands of an optical lattice. The two atomic states are resonantly coupled by a coherent field enclosed in a single cavity mode, which mediates transitions between the two bosonic particle modes via absorption or emission of cavity photons. As nonlocal atomic coherence can build up via photon assisted tunneling, this coupling shifts the transition to the Mott-insulator phase toward deeper lattice potentials and stronger on-site interaction. Varying the intra and interband on-site interactions leads to several different atomic phase configurations. There are even parameter regions, where a mean-field approach predicts concurrence of a Mott-insulator state in one band and a superfluid in the other band.