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Physical Review Letters

Low-Energy Parametrization of Scattering Observables in n -Dimensional Quantum Systems

D. Bollé, Fritz Gesztesy

Published Apr 23, 1984• 36 citations
Publisher

Abstract

A rigorous theory for low-energy scattering in quantum systems in $n$ dimensions, $n>~2$, with general, possibly long-range, interactions is presented. It gives new insights into lowenergy phenomena; e.g., for $n=2$ the controversy around the existence of scattering parameters is resolved. Furthermore, the important role of a parametrization of scattering observables in the study of spin-polarized quantum systems is illustrated. For $n=3$, an analytic expansion of the phase shift and scattering length for charged, finite-size particle scattering, around their neutral counterparts, is derived.

DOI
10.1103/physrevlett.52.1469

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arXiv:1810.07386•Oct 17, 2018•0 citations
A rigorous theory for low-energy scattering in quantum systems in nnn dimensions, n> 2n>~2n> 2, with general, possibly long-range, interactions is presented. It gives new insights into lowenergy phenomena; e.g., for n=2n=2n=2 the controversy around the existence of scattering parameters is resolved. Furthermore, the important role of a parametrization of scattering observables in the study of spin-polarized quantum systems is illustrated. For n=3n=3n=3, an analytic expansion of the phase shift and scattering length for charged, finite-size particle scattering, around their neutral counterparts, is derived.
A parametrization of low-energy two-dimensional quantum scattering is given which is in the tradition of familiar three-dimensional effective-range theory. A scattering length differing from previous treatments is introduced whose behavior reflects the repulsive or attractive nature of the interaction, and whether or not bound states are present. However its definition is subject to an unknown length parameter. An effective-range parameter is also defined and together with the scattering length explains the nonexistence of the Efimov effect in two dimensions. It is also shown that the Ramsauer–Townsend effect exists in 2D. Application to the case of a square-well potential reveals direct relationships between the unknown length parameter and the effective range to the actual range of the potential.
It is shown how the concepts of scattering length and effective range, previously introduced for low-energy scattering from a potential V(r) in a plane, correspond to the well-known parameters in three dimensions. This is done by considering low-energy scattering in a general dimension n\ensuremath{\ge}2 and subsequently showing that both the n=2 and n=3 cases fit naturally in such a generalized treatment. Furthermore, our previous work is extended to long-range potentials, decreasing faster than 1/rn+1{r}^{n+1}rn+1. The method used is based on the properties of a local scattering length a(r) for the potential V(r) cut off at radius r and an equivalent hard-sphere radius a(r,k) for k\ensuremath{\ne}0. Some applications and illustrative examples are given.
The interaction between atoms behaves as $\ensuremath{-}\ensuremath{\alpha}{/r}^{n}$ at large distances and, owing to the large reduced mass \ensuremath{\mu} of the collision pair, allows a semiclassical treatment within the potential well. As a result, the low-energy scattering is governed by two large parameters: the asymptotic parameter $\ensuremath{\gamma}=\sqrt{2\ensuremath{\mu}\ensuremath{\alpha}}/\ensuremath{\Elzxh}\ensuremath{\gg}{a}_{0}^{(n\ensuremath{-}2)/2}$ (a0{a}_{0}a0​ is the Bohr radius) and the semiclassical zero-energy phase $\ensuremath{\Phi}\ensuremath{\gg}1.$ In our previous work [Phys. Rev. A 48, 546 (1993)] we obtained an analytical expression for the scattering length a,a,a, which showed that it has 75% preference for positive values for n=6,n=6,n=6, characteristic of collisions between ground-state neutral atoms. In this paper we calculate the effective range and show that it is a function of a,a,a, ${r}_{e}{=F}_{n}\ensuremath{-}{G}_{n}{/a+H}_{n}{/a}^{2},$ where Fn,{F}_{n},Fn​, Gn,{G}_{n},Gn​, and Hn{H}_{n}Hn​ depend only on \ensuremath{\gamma}. Thus, we know the sss-phase shift at low momenta $k\ensuremath{\ll}{\ensuremath{\gamma}}^{\ensuremath{-}2/(n\ensuremath{-}2)}$ from the expansion $k\mathrm{cot}{\ensuremath{\delta}}_{0}\ensuremath{\simeq}\ensuremath{-}1/a+\frac{1}{2}{r}_{e}{k}^{2}.$ At $k\ensuremath{\gg}{\ensuremath{\gamma}}^{\ensuremath{-}2/(n\ensuremath{-}2)}$ the phase shift is obtained semiclassically as ${\ensuremath{\delta}}_{0}=\ensuremath{\Phi}+\ensuremath{\pi}/4\ensuremath{-}{I}_{n}{\ensuremath{\gamma}}^{2/n}{k}^{(n\ensuremath{-}2)/n},$ where ${I}_{n}=[n/(n\ensuremath{-}2)]\ensuremath{\Gamma}((n\ensuremath{-}1)/n)\ensuremath{\Gamma}((n+2)/2n)/\sqrt{\ensuremath{\pi}}.$ Therefore, \ensuremath{\gamma} and \ensuremath{\Phi} determine the sss-wave atomic scattering in a wide range of momenta, as well as the positions of upper bound states of the diatomic molecule.
We study the near-threshold behavior of scattering phase shifts, quantum reflection amplitudes, and quantization functions for systems described by a circularly symmetric potential in two spatial dimensions. In contrast to the three-dimensional case, the centrifugal potential $({m}^{2}\ensuremath{-}\frac{1}{4}){\ensuremath{\hbar}}^{2}∕(2M{r}^{2})$ is nonvanishing and even attractive for sss waves, m=0m=0m=0, and the leading near-threshold energy dependence of phase shifts and amplitudes for scattering and quantum reflection is logarithmic in this case. The near-threshold behavior of the sss-wave phase shifts and amplitudes can nevertheless be characterized by a well-defined scattering length (for potentials falling off faster than 1∕r21∕{r}^{2}1∕r2) and an effective range (for potentials falling off faster than 1∕r41∕{r}^{4}1∕r4). For a potential with a bound state at energy ${E}_{n}=\ensuremath{-}{\ensuremath{\hbar}}^{2}{\ensuremath{\kappa}}_{n}^{2}∕(2M)$ very near threshold, the scattering length obeys $a\stackrel{{\ensuremath{\kappa}}_{n}\ensuremath{\rightarrow}0}{\ensuremath{\sim}}2{e}^{\ensuremath{-}{\ensuremath{\gamma}}_{\mathrm{E}}}∕{\ensuremath{\kappa}}_{n}+O({\ensuremath{\kappa}}_{n})$, with no term of order ${\ensuremath{\kappa}}_{n}^{0}$---in contrast to the three-dimensional case. Analytical results are derived for homogeneous potentials, and the necessary modification of the effective-range expansion is given for potentials proportional to 1∕r41∕{r}^{4}1∕r4. For $m\ensuremath{\ne}0$ we give analytical expressions for the near-threshold behavior of phase shifts as well as scattering and quantum reflection amplitudes, which are generally valid, even when mmm is neither integer nor half-integer.
We study low-dimensional quantum systems with analytical and computational methods. Firstly, the one-dimensional extended ttt-VVV model of fermions with interactions of a finite range is investigated. The model exhibits a phase transition between liquid and insulating regimes. We use various analytical approaches to generalise previous theoretical studies. We devise a strong coupling expansion to go beyond first-order perturbation theory. The method is insensitive to the presence or the lack of integrability of the system. We extract the ground state energy and critical parameters of the model near the Mott insulating commensurate density. We also study the possible charge-density-wave phases that exist when the model is at the critical density. Secondly, we investigate Mott-Wannier complexes of two (excitons), three (trions) and four (biexcitons) charge carriers in two-dimensional semiconductors. Our study also includes impurity-bound complexes. We provide a classification of trions and biexcitons in transition-metal dichalcogenides, which incorporates the difference of spin polarisation between molybdenum- and tungsten-based materials. Using the diffusion Monte Carlo method, which is statistically exact for these systems, we extract binding energies of the complexes for a complete set of parameters of the model. Our results are compared with theoretical and experimental work on transition-metal dichalcogenides. An agreement is found for excitonic and trionic results, but we also observe a large discrepancy in the theoretical biexcitonic binding energies as compared to the experimental values. Possible reasons for this are outlined. We also calculate contact pair densities, which in the future can be used in the determination of the contact interaction.