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Journal of Applied Physics

Decoherence and time reversibility: The role of randomness at interfaces

Jean Michel Sellier, Mihail Nedjalkov, Ivan Dimov, S. Selberherr

Published Nov 1, 2013• 6 citations
Publisher

Abstract

The Wigner formalism is a convenient reformulation of the Schrödinger equation that allows the simulation of transient behavior of quantum systems in the presence of general boundary conditions. Recently, a Wigner Monte Carlo technique, based on particles signs, has been generalized to two-dimensional evolution problems. In this paper, we apply this technique to study the time reversibility of the quantum evolution of a wave packet colliding with a potential wall in the presence of interface roughness, elastic, inelastic, and diffusive interactions with the environment. We show that a wall surface roughness does not necessarily involve time irreversibility. The dynamics of the packet is indeed influenced, but remains coherent, until the boundaries of the system begin to absorb information from the system. Finally, it is shown that in the presence of inelastic scattering or diffusive processes, the time-reversibility of a quantum system is destroyed, whatever the shape of the wall interface is. In particular, we show that the random nature of a process, elastic or inelastic, is responsible for the appearance of quantum decoherence.

DOI
10.1063/1.4828736

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The Wigner formalism is a convenient reformulation of the Schrödinger equation that allows the simulation of transient behavior of quantum systems in the presence of general boundary conditions. Recently, a Wigner Monte Carlo technique, based on particles signs, has been generalized to two-dimensional evolution problems. In this paper, we apply this technique to study the time reversibility of the quantum evolution of a wave packet colliding with a potential wall in the presence of interface roughness, elastic, inelastic, and diffusive interactions with the environment. We show that a wall surface roughness does not necessarily involve time irreversibility. The dynamics of the packet is indeed influenced, but remains coherent, until the boundaries of the system begin to absorb information from the system. Finally, it is shown that in the presence of inelastic scattering or diffusive processes, the time-reversibility of a quantum system is destroyed, whatever the shape of the wall interface is. In particular, we show that the random nature of a process, elastic or inelastic, is responsible for the appearance of quantum decoherence.
This paper examines the phonon-induced electron decoherence in semiconductor nanostructures and nanodevices within the Wigner transport equation, solved using a particle Monte Carlo technique. The Wigner-Boltzmann formalism is first established as a relevant and original approach to modeling electron quantum decoherence in semiconductors. The simulation of the time evolution of a free wave-packet then allows analyzing the competition between decoherence and wave-packet expansion in a semiconductor. It is additionally argued that decoherence occurs faster than in the widely studied case of quantum Brownian motion. The simulation of a wave packet interacting with a tunnel barrier allows studying the electron localization induced by decoherence. The case of a wave packet interacting with a double barrier puts forward the mechanism of decoherence-induced transition from resonant to sequential transport through a bound state. Finally the simulation of resonant tunneling devices shows how these phenomena take place in nanodevices and highlights the transition from the quantum transport regime to the semiclassical transport regime induced by phonon scattering.
The act of measurement on a quantum state is supposed to "dephase" (dephasing refers to the phenomenon that the states lose phase coherence; then the phases get randomized in interaction with a bath of other oscillators, which is referred to as "decoherence"), then "decohere" and "collapse" (or more precisely "register" and "reduce") the state into one of several eigenstates of the operator corresponding to the observable being measured. This measurement process is sometimes described as outside standard quantum-mechanical evolution and not calculable from Schrödinger's equation. Progress has, however, been made in studying this problem with two main calculation tools-one uses a time-independent Hamiltonian, while a rather more general approach proving that decoherence occurs under some generic conditions. The two general approaches to the study of wave-function collapse are as follows. The first approach, called the "consistent" or "decoherent"' histories approach, studies microscopic histories that diverge probabilistically and explains collapse as an event in our particular history. The other, referred to as the "environmental decoherence" approach studies the effect of the environment upon the quantum system, to explain wave-function decoherence which is produced by irreversible effects of various sorts. However, as we know, wave-function collapse is not related to thermal connection with the environment, rather, it is inherent to how measurements are performed by macroscopic apparata. In the "environmental decoherence" approach, one studies decoherence using a Markovian-approximated Master equation to study the time-evolution of the reduced density matrix (post dephasing) and obtains the long-time dependence of the off-diagonal elements of this matrix. The calculation in this paper studies the evolution of a quantum system starting with "dephasing" followed by the effects of the environment with some differences from prior analyses. We start from the Schrödinger equation for the state of the system, with a time-dependent Hamiltonian that reflects the actual microscopic interactions that are occurring. Then we systematically solve (exactly) for the time-evolved state, without invoking a Markovian approximation when writing out the effective time-evolution equation, i.e., keeping the evolution unitary until the end. This approach is useful, and it shows that the system wave-function will explicitly "un-collapse" if the measurement apparatus is sufficiently small. However, in the limit of a macroscopic system, this "dephasing" quickly leads to "decoherence"-collapse is a temporary state that will simply take extremely long (of the order of multiple universe lifetimes) to reverse. This has been attempted previously and our calculation is particularly simple and calculable. We make some connections to the work by Linden et al. while doing so. The calculation in this paper has interesting implications for the interpretation of the Wigner's friend experiment, as well as the Mott experiment, which is explored in "Connection to some general theoretical results" and "Recurrence times" (especially the enumerated points in "Recurrence times"). The upshot is that as long as Wigner's friend is macroscopically large (or uses a macroscopically large measuring instrument), no one needs to worry that Wigner would see something different from his friend. Indeed, Wigner's friend does not even need to be conscious during the measurement that she conducts. It also allows one to reasonably interpret some of the more recent thought experiments proposed. In particular, as a result of the mathematical analysis, the short-time behavior of a collapsing system, at least the one considered in this paper, is not exponential. Instead, it is the usual Fermi-golden rule result. The long-term behavior is, of course, still exponential. This is a second novel feature of the paper-we connect the short-term Fermi-golden rule (quadratic-in-time behavior) transition probability to the exponential long-time behavior of a collapsing wave-function in one continuous mathematical formulation.
Decoherence in quantum systems which are classically chaotic is studied. The Arnold cat map and the quantum kicked rotor are chosen as examples of linear and nonlinear chaotic systems. The Feynman-Vernon influence functional formalism is used to study the effect of the environment on the system. It is well known that quantum coherence can obliterate chaotic behavior in the corresponding classical system. But interaction with an environment can under general circumstances quickly diminish quantum coherence and reenact classical chaotic behavior. How effectively decoherence works to sustain chaos, and how the resultant behavior qualitatively differs from the quantum picture, depending on the coupling of the system with the environment and the spectral density and temperature of the environment. We show how recurrence in the quantum cat map is lost and classical ergodicity is recovered due to the effect of the environment. Quantum coherence and diffusion suppression are instrumental to dynamical localization for the kicked rotor. We show how environment-induced effects can destroy this localization. Such effects can also be understood as resulting from external noises driving the system. Peculiar to decohering chaotic systems is the apparent transition from reversible to irreversible dynamics. We show such transitions in the quantum cat map and the kicked rotor and distinguish it from apparent irreversibility originating from dynamical instability and imprecise measurements. By performing a time reversal on and following the quantum kicked rotor dynamics numerically, we show how the otherwise reversible quantum dynamics acquires an arrow of time upon the introduction of noise or interaction with an environment.
The interaction of a quantum system with a many degree o ff reedom environment entails damping and the loss of quantum coherence. In these two lectures we focus on two aspects of open quantum system dynamics. First, we present decoherence as a dynamical phenomenon and determine the corresponding time scales, discuss an experiment and the nature of robust states, and mention universal properties of short- time decoherence of macroscopic superpositions. Secondly, in analogy to the classical description of open systems in terms of Langevin equations, we present a stochastic approach to open quantum system dynamics in terms of a stochastic Schrodinger equation. We give a microscopic ¨ derivation that allows us to generalize the stochastic approach to non- Markovian situations. We discuss a convolutionless formulation of our theory and finally, we focus on the quantised version of Brownian motion as an often-employed example.
In this paper we reexamine, and analyze solutions to, the recently derived time-independent wave packet-Schrödinger (TIWS) and time-independent wave packet-Lippmann–Schwinger (TIWLS) equations. These equations are so named because they are inhomogeneous, with the inhomogeneity being the initial L2 wave packet from an underlying time-dependent treatment of the dynamics. We explicitly show that a particular solution of the homogeneous Schrödinger equation can be constructed out of two particular solutions of the inhomogeneous TIW equation satisfying causal and anticausal boundary conditions. The structure of this solution of the homogeneous equation is shown to depend sensitively on the nature of the initial wave packet inhomogeneity, but, as we demonstrate, correct scattering information can be obtained even when the initial wave packet is nonzero only in the target region. It thus becomes possible to carry out quantum scattering calculations in which one need not propagate the wave packet from the noninteracting to the interacting region. The method is illustrated by calculations for two 1-D scattering problems, namely the transmission of an electron through a single barrier and through a double barrier. The latter is especially challenging because of the occurrence of long-lived resonances with the electron trapped inside the double barrier. In addition, we show that the method can still make use of absorbing potentials to decrease grid size, and we show how the formalism can be used to treat inelastic and reactive scattering, and radial scattering variables, thereby constituting a general approach to time-independent wave packet quantum scattering.
With a choice of boundary conditions for solutions of the Schrödinger equation, state vectors and density operators even for closed systems evolve asymmetrically in time. For open systems, standard quantum mechanics consequently predicts irreversibility and signatures of the extrinsic arrow of time. The result is a new framework for the treatment of decoherence, not based on a reduced dynamics or a master equation. As an application, using a general model we quantitatively match previously puzzling experimental results and can conclude that they are the measurable consequence of the indistinguishability of separate, uncontrolled interactions between systems and their environment.