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Optics and Spectroscopy

Modified optical bloch equations in nonlocal systems of two-level atoms interacting with ultrashort light pulses

O. N. Gadomskiĭ, S. N. Ivanyakov

Published Jan 1, 2001• 0 citations
Publisher

Abstract

Modified optical Bloch equations for two-level atoms in the radiation field with the complex polarization vector, the complex amplitude, and the complex wave vector are derived. A specific case is considered in which a field of this kind acts on a separate atom of a nonlocal atomic system. The solution of the modified equations for the interaction of atoms with ultrashort light pulses is obtained.

DOI
10.1134/1.1343538

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Modified optical Bloch equations for two-level atoms in the radiation field with the complex polarization vector, the complex amplitude, and the complex wave vector are derived. A specific case is considered in which a field of this kind acts on a separate atom of a nonlocal atomic system. The solution of the modified equations for the interaction of atoms with ultrashort light pulses is obtained.
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Based on a model of strong coupling for two electrons that are localized inside a quantum dot characterized by only two levels of size quantization, a set of equations is derived, which allows one to describe coherent transient processes in an ensemble of isolated dots. This set of equations is a generalization of the Bloch equations, which are used in studying the processes occurring under the action of ultrashort pulses of electromagnetic interaction. The model obtained is reduced to the model of two-level atoms only if radiation is circularly polarized.
The nine (9) elements of the density matrix of a general three-level atom interacting with a classically described linearly polarized light are parameterized by eight (8) variables related to the populations of the atomic levels, and the coherences (interference effects) between the levels. The dynamical equations of these eight parameters (that is, the optical Bloch equations for a general three-level atom) are derived under the electric dipole as well as the rotating wave approximations, and under the assumption that the matrix elements of the atomic electric dipole are all real. The general optical Bloch equations so derived are shown to contain the well-known optical Bloch equations for three-level atoms in the , and cascade configurations as well as those for two-level atoms as special cases. Expressing the interaction of light with a three-level atom in all possible configurations as well as with a two-level atom by a single set of generalized optical Bloch equations is the main result of this work.
We propose and develop a method for theoretical description of circularly (elliptically) polarized optical pulse resonant coherent interactions with two-level atoms. The method is based on the time-evolution equations of a two-level quantum system in the presence of a time-dependent dipole perturbation for electric dipole transitions between states with total angular-momentum projection difference $(\ensuremath{\Delta}{J}_{z}=\ifmmode\pm\else\textpm\fi{}1)$ excited by a circularly polarized electromagnetic field [Feynman et al., J. Appl. Phys. 28, 49 (1957)]. The adopted real-vector representation approach allows for coupling with the vectorial Maxwell's equations for the optical wave propagation and thus the resulting Maxwell pseudospin equations can be numerically solved in the time domain without any approximations. The model permits a more exact study of the ultrafast coherent pulse propagation effects taking into account the vector nature of the electromagnetic field and hence the polarization state of the optical excitation. We demonstrate self-induced transparency effects and formation of polarized solitons. The model represents a qualitative extension of the well-known optical Maxwell-Bloch equations valid for linearly polarized light and a tool for studying coherent quantum control mechanisms.
We investigate the interaction of a multilevel atom with a short femtosecond optical pulse beyond the scope of the rotating-wave approximation. We consider the behavior of a three-level atom under the action of two optical pulses resonant with two allowed transitions and a two-level atom under the action of a resonant optical pulse. It is shown that the imaginary part of the off-diagonal elements of the density matrix oscillates with high frequency due to the counter-rotating terms. It is shown also that an effective time-dependent addition to the Rabi frequency exists, which is of importance for ultrashort optical pulses.