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Optics and Spectroscopy

Enhancement of electromagnetically induced transparency in room temperature alkali metal vapor

O. S. Mishina, Michael S. Scherman, Pietro Lombardi, J. Ortalo, D. Felinto, A. S. Sheremet, Dmitriy V. Kupriyanov, Julien Laurat, E. Giacobino

Published Oct 1, 2011• 3 citations
Publisher

Abstract

Electromagnetically induced transparency (EIT) has led to several quantum optics effects such as lasing without inversion or squeezed light generation. More recently quantum memories based on EIT have been experimentally implemented in different systems such as alkali metal atoms. In this system the excited state of the optical transition splits into several sublevels due to the hyperfine interaction. However, most of the theoretical models used to describe the experimental results are based on a Λ-system with only one excited state. In this article, we present a theoretical model for the Λ-type interaction of two light, fields and an atomic system with multiple excited state. In particular we show that if the control and probe fields are orthogonally circularly polarized the EIT effect in an alkali-metal vapor can almost disappears. We also identify the reasons of this reduction and propose a method to recover the transparency via velocity selective optical pumping.

DOI
10.1134/s0030400x1111021x

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Electromagnetically induced transparency (EIT) has led to several quantum optics effects such as lasing without inversion or squeezed light generation. More recently quantum memories based on EIT have been experimentally implemented in different systems such as alkali metal atoms. In this system the excited state of the optical transition splits into several sublevels due to the hyperfine interaction. However, most of the theoretical models used to describe the experimental results are based on a system with only one excited state. In this article, we present a theoretical model for the type interaction of two light, fields and an atomic system with multiple excited state. In particular we show that if the control and probe fields are orthogonally circularly polarized the EIT effect in an alkali metal vapor can almost disappears. We also iden tify the reasons of this reduction and propose a method to recover the transparency via velocity selective opti cal pumping. DOI: 10.1134/S0030400X1111021X Λ Λ COHERENT EFFECTS IN OPTICAL AND ATOMIC–MOLECULAR PROCESSES

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Electromagnetically induced transparency (EIT) has led to several quantum optics effects such as lasing without inversion or squeezed light generation. More recently quantum memories based on EIT have been experimentally implemented in different systems such as alkali metal atoms. In this system the excited state of the optical transition splits into several sublevels due to the hyperfine interaction. However, most of the theoretical models used to describe the experimental results are based on a Λ-system with only one excited state. In this article, we present a theoretical model for the Λ-type interaction of two light, fields and an atomic system with multiple excited state. In particular we show that if the control and probe fields are orthogonally circularly polarized the EIT effect in an alkali-metal vapor can almost disappears. We also identify the reasons of this reduction and propose a method to recover the transparency via velocity selective optical pumping.
Electromagnetically induced transparency (EIT) has led to several quantum optics effects such as lasing without inversion or squeezed light generation. More recently quantum memories based on EIT have been experimentally implemented in different systems such as alkali metal atoms. In this system the excited state of the optical transition splits into several sublevels due to the hyperfine interaction. However, most of the theoretical models used to describe the experimental results are based on a system with only one excited state. In this article, we present a theoretical model for the type interaction of two light, fields and an atomic system with multiple excited state. In particular we show that if the control and probe fields are orthogonally circularly polarized the EIT effect in an alkali metal vapor can almost disappears. We also iden tify the reasons of this reduction and propose a method to recover the transparency via velocity selective opti cal pumping. DOI: 10.1134/S0030400X1111021X Λ Λ COHERENT EFFECTS IN OPTICAL AND ATOMIC–MOLECULAR PROCESSES
Electromagnetically induced transparency (EIT) has mainly been modelled for three-level systems. In particular, a considerable interest has been dedicated to the Lambda-configuration, with two ground states and one excited state. However, in the alkali-metal atoms, which are commonly used, hyperfine interaction in the excited state introduces several levels which simultaneously participate in the scattering process. When the Doppler broadening is comparable with the hyperfine splitting in the upper state, the three-level Lambda model does not reproduce the experimental results. Here we theoretically investigate the EIT in a hot vapor of alkali-metal atoms and demonstrate that it can be strongly reduced due to the presence of multiple excited levels. Given this model, we also show that a well-designed optical pumping enables to significantly recover the transparency.
Electromagnetically induced transparency (EIT) has mainly been modeled for three-level systems. In particular, considerable interest has been dedicated to the $\ensuremath{\Lambda}$ configuration, with two ground states and one excited state. However, in the alkali-metal atoms, which are commonly used, the hyperfine interaction in the excited state introduces several levels which simultaneously participate in the scattering process. When the Doppler broadening is comparable with the hyperfine splitting in the upper state, the three-level $\ensuremath{\Lambda}$ model does not reproduce the experimental results. Here we theoretically investigate the EIT in a hot vapor of alkali-metal atoms and demonstrate that it can be strongly reduced by the presence of multiple excited levels. Given this model, we also show that well-designed optical pumping enables us to significantly recover the transparency.
The effect of electromagnetically induced transparency (EIT) has been experimentally implemented for the first time for the (4S 1/2–4P 1/2–4S 1/2) Λ-system of potassium atom levels in a nanocell with a 770-nm-thick column of atomic vapor. It is shown that, at such a small thickness of the vapor column, the EIT resonance can be observed only when the coupling-laser frequency is in exact resonance with the frequency of the corresponding atomic transition. The EIT resonance disappears even if the coupling-laser frequency differs slightly (by ~50 MHz) from that of the corresponding atomic transition, which is due to the high thermal velocity of K atoms. The EIT resonance and related velocity selective optical pumping resonances caused by optical pumping (formed by the coupling) can be simultaneously recorded because of the small (~462 MHz) hyperfine splitting of the lower 4S 1/2 level.
Electromagnetically-induced transparency has become an important tool to control the optical properties of dense media. However, in a broad class of systems, the interplay between inhomogeneous broadening and the existence of several excited levels may lead to a vanishing transparency. Here, by identifying the underlying physical mechanisms resulting in this effect, we show that transparency can be strongly enhanced. We thereby demonstrate a 5-fold enhancement in a room-temperature vapor of alkali-metal atoms via a specific shaping of the atomic velocity distribution.
The behavior of multilevel atomic ensembles (e.g., alkali-metal atoms) can be influenced significantly by the intensity of a driving field (or controlling/coupling field). The phase coherence between two transition pathways driven by a probe light and a driving field can lead to the effect known as electromagnetically induced transparency (EIT). In EIT, the probe light can pass through a three-level alkali-metal atomic vapor without absorption or reflection when two coherent resonances (transition pathways driven by the driving and probe fields) are present and the linewidths of the transparency windows are sufficiently narrow. The optical characteristics of atomic systems can also be affected by the Doppler broadening of the absorption profile in a spectroscope. Our analysis indicates that both broadenings (related to the transitions excited by the driving and probe fields) can be expanded, leading to an increase in the transmittance and reflectance broadenings when a coupling field with adaptive strength is applied; the corresponding temperature would, thus, be implemented and readable. We show that the most suitable preparation for temperature sensing via an EIT vapor is to provide 80 times the spontaneous decay rate (SDR) of the excited atomic levels. This configuration results in reflectance and transmittance values that range between zero and one and cover a temperature range of 0 K to 600 K. As an example, we demonstrate the integration of specialized coating technologies with EIT ensembles for temperature sensing in the range of dozens of kelvins at and above room temperature. A key advantage of this temperature-sensing system is its ability to use adaptive resonant visible light as the probe field. This novel approach may find applications in providing unprecedented levels of precision and control in temperature sensing for coating processes and in the design of other photonic or optical devices. It can also be used to determine the temperature-dependent behavior of the specific heat of alkali-metal solids and gases (including the latent heats of vaporization or sublimation of alkali-metal solids) through the reflection and transmission spectra of the vaporized EIT atomic vapors.