We present an experimental observation and comprehensive theory that address the effect of interaction on the phase transition in a many-body system, which is far from equilibrium and does not have detailed balance. In the resonantly driven cold atomic trap, we observe kinetic phase transition (KPT) that is manifested by substantial enhancement of fluctuations, similar to the first-order phase transition in thermal equilibrium. Moreover, we can control the attractive interaction between atoms trapped in the coexisting states by adjusting the total number of atoms, which induces shift of the phase boundaries of KPT. The demonstrated effect is the many-body analogue of KPT that was previously predicted and observed in a single-driven oscillator. Our work provides a unique model platform for quantitative study of nonequilibrium nonlinear dynamics in many-body systems.
We present an experimental observation and comprehensive theory that address the effect of interaction on the phase transition in a many-body system, which is far from equilibrium and does not have detailed balance. In the resonantly driven cold atomic trap, we observe kinetic phase transition (KPT) that is manifested by substantial enhancement of fluctuations, similar to the first-order phase transition in thermal equilibrium. Moreover, we can control the attractive interaction between atoms trapped in the coexisting states by adjusting the total number of atoms, which induces shift of the phase boundaries of KPT. The demonstrated effect is the many-body analogue of KPT that was previously predicted and observed in a single-driven oscillator. Our work provides a unique model platform for quantitative study of nonequilibrium nonlinear dynamics in many-body systems.
Atomic ensembles strongly interacting with light constitute rich quantum-optical many-body systems, with the potential for observing cooperative effects and dissipative nonequilibrium phase transitions. We theoretically analyze the conditions under which a driven atomic ensemble in free space, characterized by strong dipole-dipole interactions and large spatial extent, can undergo a superradiant phase transition, also known as cooperative resonance fluorescence. In an atomic array, stationary states that conserve the collective pseudospin exhibit completely cooperative decay and undergo a second-order phase transition in the large atom number limit. In contrast, decay mechanisms on longer timescales that fail to conserve pseudospin can lead to discontinuous first-order phase transition at a critical finite atom number, disrupting cooperation despite sharing many similar observable characteristics. A hallmark of the superradiant phase transition is an abrupt shift from total light reflection off the atoms to rapidly increasing transmission, accompanied by significant quantum fluctuations, as a function of light intensity.
Abstract Far-from equilibrium dynamics that lead to self-organization are highly relevant to complex dynamical systems not only in physics, but also in life-, earth-, and social sciences. It is challenging however to find systems with sufficiently controllable parameters that allow quantitatively modelling of emergent properties. Here, we study a non-equilibrium phase transition and observe signatures of self-organized criticality in a dilute thermal vapour of atoms optically excited to strongly interacting Rydberg states. Electromagnetically induced transparency (EIT) provides excellent control over the population dynamics and enables high-resolution probing of the driven-dissipative dynamics, which also exhibits phase bistability. Increased sensitivity compared to previous work allows us to reconstruct the complete phase diagram including in the vicinity of the critical point. We observe that interaction-induced energy shifts and enhanced decay only occur in one of the phases above a critical Rydberg population. This limits the application of generic mean-field models, however a modified, threshold-dependent approach is in qualitative agreement with experimental data. Near threshold, we observe self-organized dynamics in the form of population jumps that return the density to a critical value.
Far-from-equilibrium dynamics that lead to self-organization are highly relevant to complex dynamical systems not only in physics but also in life, earth, and social sciences.However, it is challenging to find systems with sufficiently controllable parameters that allow quantitatively modeling of emergent properties.Here, we study a nonequilibrium phase transition and observe signatures of self-organized criticality in a dilute thermal vapor of atoms optically excited to strongly interacting Rydberg states.Electromagnetically induced transparency provides excellent control over the population dynamics and enables highresolution probing of the driven-dissipative dynamics, which also exhibits phase bistability.Increased sensitivity compared to previous work allows us to reconstruct the complete phase diagram, including in the vicinity of the critical point.We observe that interaction-induced energy shifts and enhanced decay only occur in one of the phases above a critical Rydberg population.This case limits the application of generic mean-field models; however, a modified, threshold-dependent approach is in qualitative agreement with experimental data.Near threshold, we observe self-organized dynamics in the form of population jumps that return the density to a critical value.
Due to the variety of tools available to control atomic, molecular, and optical (AMO) systems, they provide a versatile platform for studying many-body physics, quantum simulation, and quantum computation. Although extensive efforts are employed to reduce coupling between the system and the environment, the effects of the environment can never fully be avoided, so it is important to develop a comprehensive understanding of open quantum systems. The system-environment coupling often leads to loss via dissipation, which can be countered by a coherent drive. Open quantum systems subject to dissipation and drive are known as driven-dissipative systems, and they provide an excellent platform for studying many-body nonequilibrium physics. The first part of this dissertation will focus on driven-dissipative phase transitions. Despite the nonequilibrium nature of these systems, the corresponding phase transitions tend to exhibit emergent equilibrium behavior. However, we will show that in the vicinity of a multicritical point where multiple phase transitions intersect, genuinely nonequilibrium criticality can emerge, even though the individual phase transitions on their own exhibit equilibrium criticality. These nonequilibrium multicritical points can exhibit a variety of exotic phenomena not possible for their equilibrium counterparts, including the emergence of complex critical exponents, which lead to discrete scale invariance and spiraling phase boundaries. Furthermore, the Liouvillian gap can take on complex values, and the fluctuation-dissipation theorem is violated, corresponding to an effective temperature which gets "hotter" and "hotter" at longer and longer wavelengths. The second part of this dissertation will focus on Rydberg atoms. In particular, we study how the spontaneous generation of contaminant Rydberg states drastically modifies the behavior of a driven-dissipative Rydberg system due to the resultant dipole-dipole interactions. These interactions lead to a complicated competition of both blockade and anti-blockade effects, leading to strongly enhanced Rydberg populations for far-detuned drive and reduced Rydberg populations for resonant drive.
Abstract We report the first experimental observation of dissipation-driven coherent quantum many-body oscillation, and this oscillation is manifested as the coherent exchange of atoms between the thermal and condensate components in a three-dimensional partially condensed Bose gas. Firstly, we observe that the dissipation leads to two different atom loss rates between the thermal and the condensate components, such that the thermal fraction increases as dissipation time increases. Therefore, this dissipation process serves as a tool to uniformly ramp up the system’s temperature without introducing extra density excitation. Subsequently, a coherent pair exchange of atoms between the thermal and the condensate components occurs, resulting in coherent oscillation of atom numbers in both components. This oscillation, permanently embedded in the atom loss process, is revealed clearly when we inset a duration of dissipation-free evolution into the entire dynamics, manifested as an oscillation of total atom number at the end. Finally, we also present a theoretical calculation to support this physical mechanism, which simultaneously includes dissipation, interaction, finite temperature, and harmonic trap effects. Our work introduces a highly controllable dissipation as a new tool to control quantum many-body dynamics.
We discuss an open driven-dissipative many-body system, in which the competition of unitary Hamiltonian and dissipative Liouvillian dynamics leads to a nonequilibrium phase transition. It shares features of a quantum phase transition in that it is interaction driven, and of a classical phase transition, in that the ordered phase is continuously connected to a thermal state. We characterize the phase diagram and the critical behavior at the phase transition approached as a function of time. We find a novel fluctuation induced dynamical instability, which occurs at long wavelength as a consequence of a subtle dissipative renormalization effect on the speed of sound.